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ACS Photonics

Visible-Telecom Entangled-Photon Pair Generation with Integrated Photonics: Guidelines and a Materials Comparison

Liao Duan, Trevor J. Steiner, Paolo Pintus, Lillian Thiel, Joshua E. Castro, John Edward Bowers, Galan Moody

Published Nov 25, 2024• 10 citations
Publisher

Abstract

Correlated photon-pair sources are key components for quantum computing, networking, synchronization, and sensing applications. Integrated photonics has enabled chip-scale sources using nonlinear processes, producing high-rate time-energy and polarization entanglement at telecom wavelengths with sub-100 microwatt pump power. Many quantum systems operate in the visible or near-infrared ranges, necessitating visible-telecom entangled-pair sources for connecting remote systems via entanglement swapping and teleportation. This study evaluates biphoton pair generation and time-energy entanglement through spontaneous four-wave mixing in various nonlinear integrated photonic materials, including silicon nitride, lithium niobate, aluminum gallium arsenide, indium gallium phosphide, and gallium nitride. We demonstrate how geometric dispersion engineering facilitates phase-matching for each platform and reveals unexpected results, such as robust designs to fabrication variations and a Type-1 cross-polarized phase-matching condition for III-V materials that expands the operational wavelength range.

DOI
10.1021/acsphotonics.4c01238

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Correlated photon-pair sources are key components for quantum computing, networking, synchronization, and sensing applications. Integrated photonics has enabled chip-scale sources using nonlinear processes, producing high-rate time-energy and polarization entanglement at telecom wavelengths with sub-100 microwatt pump power. Many quantum systems operate in the visible or near-infrared ranges, necessitating visible-telecom entangled-pair sources for connecting remote systems via entanglement swapping and teleportation. This study evaluates biphoton pair generation and time-energy entanglement through spontaneous four-wave mixing in various nonlinear integrated photonic materials, including silicon nitride, lithium niobate, aluminum gallium arsenide, indium gallium phosphide, and gallium nitride. We demonstrate how geometric dispersion engineering facilitates phase-matching for each platform and reveals unexpected results, such as robust designs to fabrication variations and a Type-1 cross-polarized phase-matching condition for III-V materials that expands the operational wavelength range.
Correlated photon-pair sources are key components for quantum computing, networking, and sensing applications. Integrated photonics has enabled chip-scale sources using nonlinear processes, producing high-rate entanglement with sub-100 microwatt power at telecom wavelengths. Many quantum systems operate in the visible or near-infrared ranges, necessitating broadband visible-telecom entangled-pair sources for connecting remote systems via entanglement swapping and teleportation. This study evaluates broadband entanglement generation through spontaneous four-wave mixing in various nonlinear integrated photonic materials, including silicon nitride, lithium niobate, aluminum gallium arsenide, indium gallium phosphide, and gallium nitride. We demonstrate how geometric dispersion engineering facilitates phase-matching for each platform and reveals unexpected results, such as robust designs to fabrication variations and a Type-1 cross-polarized phase-matching condition for III-V materials that expands the operational bandwidth. With experimentally attainable parameters, integrated photonic microresonators with optimized designs can achieve pair generation rates greater than ~1 THz/mW2^22.
Photon pair sources are fundamental building blocks for quantum entanglement and quantum communication. Recent studies in silicon photonics have documented promising characteristics for photon pair sources within the telecommunications band, including sub-milliwatt optical pump power, high spectral brightness, and high photon purity. However, most quantum systems suitable for local operation (e.g., storage/computation) support optical transitions in the visible or short nearinfrared bands. In comparison to telecommunications wavelengths, the significantly higher optical attenuation in silica at such wavelengths limits the length scale over which optical-fiber-based quantum communication between such local nodes can take place. One approach to connect such systems over fiber is through a photon pair source that can bridge the visible and telecom bands, but an appropriate source, which should produce narrow-band photon pairs with a high signal-to-noise ratio, has not yet been developed in an integrated platform. Here, we demonstrate a nanophotonic visible-telecom photon pair source for the first time, using high quality factor silicon nitride resonators to generate narrow-band photon pairs with unprecedented purity and brightness, with coincidence-toaccidental ratio (CAR) up to 3,780 ± 140 and detected photon-pair flux up to (18,400 ± 1,000) pairs/s. We further demonstrate visible-telecom time-energy entanglement and its distribution over a 20 km fiber, far exceeding the fiber length over which purely visible wavelength quantum light sources can be transmitted. Finally, we show how dispersion engineering of the microresonators enables the connections of different species of trapped atoms/ions, defect centers, and quantum dots to the telecommunications bands for future quantum communication systems.
Quantum state distribution over vast distances is essential for global-scale quantum networks and fundamental test of quantum physics at space scale. While satellite platforms have demonstrated thousand-kilometer entanglement distribution, quantum key distribution and quantum teleportation with ground, future constellations and deep-space missions demand photon sources that are robust, compact, and power-efficient. Integrated photonics offers a scalable solution, yet a critical spectral gap persists. Although telecom-band integrated photon-pair sources are well established, near-visible photons offer distinct advantages for satellite-to-ground links by mitigating diffraction loss and maximizing the collection efficiency of optical telescopes. Scalable integrated sources in this regime have remained elusive due to the fundamental challenge of achieving anomalous dispersion in materials transparent at visible wavelengths. Here we bridge this gap by demonstrating an integrated near-visible photon-pair source based on a wide-bandgap, ultralow-loss, silicon nitride (Si3_33​N4_44​) microresonator. By engineering the dispersion of higher-order waveguide modes, we overcome the intrinsic normal dispersion limit to achieve efficient phase matching. The device exhibits a spectral brightness of 4.87$\times101010^7$ pairs/s/mW2^22/GHz and a narrow photon linewidth of 357 MHz. We report high-purity heralded single-photon generation with a heralding rate up to 2.3 MHz and a second-order correlation function as low as 0.0041. Furthermore, we observe energy-time entanglement with 98.4% interference visibility, violating the CHSH limit even at flux exceeding 40.6 million pairs/s. Combined with the proven radiation hardness of Si3_33​N4_44​, this source constitutes a flight-ready hardware foundation for daylight quantum communications and protocols requiring on-orbit multiphoton interference.
Entangled photons generation is an interesting field of research, since progress in this area will directly affect the development of photonic quantum technologies, including quantum computing, simulation and sensing. Several methods have been sifted to increase the performances of entangled photon sources and the integrated optics approach represents a promising strategy. In particular, integrated waveguide sources represent a robust tool, thanks to their stability and the enhancement of nonlinear light-crystal interaction provided by waveguide field confinement. Here, we show the versatility of a hybrid approach, realizing an integrated optical source for the generation of entangled photon-pairs at telecom wavelength. The nonlinear active medium used is lithium niobate, while the routing and manipulation of the generated signal is performed in aluminum-borosilicate glass photonic circuits. The system is composed of three cascaded devices. First, a balanced directional coupler at the fundamental wavelength equally splits the pump in the lithium niobate waveguides, which generate single-photon pairs through type 0 spontaneous parametric down-conversion process. A third chip, encompassing directional couplers and waveplates, closes the interferometer and recombines the generated photons, thus giving access to different quantum states of light: path-entangled or polarization-entangled states. A thermal phase shifter, which controls the relative phase between the interferometer arms, gives an additional degree of freedom for engineering the output state of the presented photon pairs source. All these components are entirely fabricated by femtosecond laser micromachining, a direct and very versatile technique that allows to process different kind of materials and realize high quality optical circuits.
Quantum networks based on wavelength-multiplexed entanglement enable parallel distribution of quantum correlations, increasing channel capacity for secure communication and distributed quantum information processing. However, broadband integrated sources capable of generating multipartite entanglement beyond photon pairs remain scarce. Here we report on-chip generation of telecom-band four-photon entanglement in a periodically poled thin-film lithium niobate on insulator (LNOI) waveguide. Type-0 spontaneous parametric down-conversion provides a phase-matching bandwidth exceeding 200 nm, enabling spectrally separable generation of multi-photon entanglement across the telecom band. The generated photons are encoded in time bins for robust fiber compatibility, and a coherent interface enabling reversible conversion between time-bin and polarization degrees of freedom allows complete quantum state tomography. We measure two-photon entanglement with a brightness of 6.7 MHz/mW/nm and a fidelity of 0.874±0.0020.874 \pm 0.0020.874±0.002. At a pump power of 0.08 mW, the four-photon state exhibits a fourfold coincidence rate of 1 Hz and a fidelity of 0.74±0.010.74 \pm 0.010.74±0.01, representing a threefold improvement over previous integrated platforms. Our results establish LNOI as a scalable platform for broadband multi-photon entanglement and provide a practical route toward dense wavelength-multiplexed quantum networks.
Generation of entangled photon pairs at telecom wavelength has been garnering a growing interest in the context of quantum communications and quantum computing. Several generation techniques have been proposed, including spontaneous Four-Wave Mixing in resonators or Spontaneous Parametric Down Conversion (SPDC) in Periodically Polled Lithium Niobate (PPLN) waveguides. Large photon pair efficiencies have been demonstrated in particular in PPLN on insulator [3]. However, polarization entangled photon pair generation (Type II phase matching configuration) suffers from a less favourable non-linear coefficient and optical mode birefringence in PPLN.