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arXiv:2203.16321 · Journal of Physics Conference Series

Excitation and transport of bound magnon clusters in frustrated ferromagnetic chain

Hiroaki Onishi

Published Mar 1, 2022• 0 citations
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Abstract

Abstract We investigate magnetic excitations and spin transport properties of a frustrated spin chain with ferromagnetic nearest-neighbor and antiferromagnetic next-nearest-neighbor exchange couplings in a magnetic field by density-matrix renormalization group methods. In the field-induced quadrupole and octupole regimes, the low-energy excitation is governed by two-and three-magnon bound states, respectively, so that bound magnon clusters would contribute to the spin transport. We show that spin current correlations decrease when the system goes from the quadrupole regime into the octupole regime. This indicates that the spin transport is suppressed in the octupole regime, although bound three-magnon clusters carry a larger amount of angular momentum than bound two-magnon clusters.

DOI
10.1088/1742-6596/2207/1/012045

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We study few-magnon excitations in a finite-size spin-SSS chain with ferromagnetic nearest-neighbor (NN) interaction J>0J>0J>0 and antiferromagnetic next-nearest-neighbor (NNN) interaction ${J}^{\ensuremath{'}}<0$, in the presence of the single-ion (SI) anisotropy DDD. We first reveal the condition for the emergence of zero-excitation-energy states. In the isotropic case with $\mathrm{\ensuremath{\Delta}}={\mathrm{\ensuremath{\Delta}}}^{\ensuremath{'}}=1$ ($\mathrm{\ensuremath{\Delta}}$ and ${\mathrm{\ensuremath{\Delta}}}^{\ensuremath{'}}$ are the corresponding anisotropy parameters), a threshold of $J/|{J}^{\ensuremath{'}}|$, above which the ground state is ferromagnetic, is determined by exact diagonalization for short chains up to 12 sites. Using a set of exact two-magnon Bloch states, we then map the two-magnon problem to a single-particle one on an effective open chain with both NN and NNN hoppings. The whole two-magnon excitation spectrum is calculated for large systems, and the commensurate-incommensurate transition in the lowest-lying mode is found to exhibit different behaviors between S=1/2S=1/2S=1/2 and higher spins due to the interplay of the SI anisotropy and the NNN interaction. For the commensurate momentum $k=\ensuremath{-}\ensuremath{\pi}$, the effective lattice is decoupled into two NN open chains that can be exactly solved via a plane-wave ansatz. Based on this, we analytically identify in the ${\mathrm{\ensuremath{\Delta}}}^{\ensuremath{'}}\ensuremath{-}D/|{J}^{\ensuremath{'}}|$ plane the regions supporting the SI or NNN exchange two-magnon bound states near the edge of the band. In particular, we prove that there always exists a lower-lying NN exchange two-magnon bound state near the band edge for arbitrary $S\ensuremath{\ge}1/2$. Finally, we numerically calculate the nnn-magnon spectra for S=1/2S=1/2S=1/2 with $n\ensuremath{\le}5$ by using a spin-operator matrix element method. The corresponding nnn-magnon commensurate instability regions are determined for finite chains, and consistent results with prior literature are observed.
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We investigate the ground-state phase diagram of frustrated mixed-spin (1, 1/2) chains with three-site four-spin interactions employing different approaches, such as cluster mean field theory, cluster variational method, and spin-wave theory. The interplay of next-nearest-neighbor and three-site interactions leads to a plethora of magnetic and nonmagnetic phases in the ground-state phase diagram. We show that aside from the ferromagnetic and Neel orders, the ground state possesses a magnetic phase in which magnon excitations are dispersionless. The emergence of flat-band magnons is a consequence of the inhomogeneity of our frustrated mixed-spin chains and does not occur in similar uniform spin chains. We also demonstrate that the presence of three-site interaction gives rise to various nonmagnetic phases, such as antiferroquadrupole order and quantum spin-liquid phase.