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arXiv:2203.13378 · Physical review. B./Physical review. B

Magnetic impurity as a local probe of the U (1) quantum spin liquid with spinon Fermi surface

Wen‐Yu He, Patrick A. Lee

Published May 31, 2022• 26 citations
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Abstract

We solve the problem of a magnetic impurity coupled to a $U(1)$ quantum spin liquid with a spinon Fermi surface, and we compute the impurity spectral function. Using the slave rotor mean-field approach combined with gauge field fluctuations, we find that a peak located at the top of the lower Hubbard band and one at the bottom of the upper Hubbard band can emerge in the impurity spectral function. The peaks at the Hubbard band edges arise from the gauge field fluctuation-induced spinon-chargon binding inside the spinon Kondo screening cloud of the magnetic impurity. For a magnetic impurity embedded in a Mott insulator, our findings suggest that the emergence of a pair of peaks at the Hubbard band edges in the impurity density of states spectra provides strong evidence that the host Mott insulator is a $U(1)$ quantum spin liquid with a spinon Fermi surface.

DOI
10.1103/physrevb.105.195156

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We solve the problem of a magnetic impurity coupled to a U(1)U(1)U(1) quantum spin liquid with a spinon Fermi surface, and we compute the impurity spectral function. Using the slave rotor mean-field approach combined with gauge field fluctuations, we find that a peak located at the top of the lower Hubbard band and one at the bottom of the upper Hubbard band can emerge in the impurity spectral function. The peaks at the Hubbard band edges arise from the gauge field fluctuation-induced spinon-chargon binding inside the spinon Kondo screening cloud of the magnetic impurity. For a magnetic impurity embedded in a Mott insulator, our findings suggest that the emergence of a pair of peaks at the Hubbard band edges in the impurity density of states spectra provides strong evidence that the host Mott insulator is a U(1)U(1)U(1) quantum spin liquid with a spinon Fermi surface.
Electronic Density of States of a U(1)U\left(1\right)U(1) Quantum Spin Liquid with Spinon Fermi Surface. I. Orbital Magnetic Field Effects
Quantum spin liquid (QSL) with spinon Fermi surface is an exotic insulator that hosts neutral Fermi surfaces inside the gap. In an external magnetic field, it has been pointed out that the neutral Fermi surfaces are Landau quantized to form Landau levels (LLs) due to the induced emergent gauge magnetic field. In this work, we calculate the electronic density of states (DOS) of the QSL in an orbital magnetic field. We find that the LLs from the neutral Fermi surfaces give rise to a set of steps emerging at the upper and lower Hubbard band edges. Each of the Hubbard band edge steps further develop into a band edge resonance peak when a weak gauge binding from the gauge field fluctuations is taken into account. Importantly, each Hubbard band edge step and its resulting resonance peak in the weak gauge binding are found to have a correspondence LL from the neutral Fermi surfaces, so the Hubbard band edge steps and the band edge resonance peaks are the unique features that characterize the Landau quantization of the in-gap neutral Fermi surfaces. We further consider the strong gauge binding regime where the band edge resonance peaks move into the Mott gap and develop into true in-gap bound states. In the strong gauge binding regime, we solve the bound state LL spectrum. For the bound state with a Mexican hat like band dispersion, we find that the envelop energy to have a state excited from the bound state LL decreases quadratically with the magnetic field. The quadratic decrease behavior of the envelop energy is consistent with the intuition that applying magnetic field localizes the states and energetically promotes the in-gap bound states formation. Finally, we connect our results to the electronic DOS spectra measured in the layered 1T-TaS2_22​. We point out that a QSL with a quasi-bound state in the upper Hubbard band can give the DOS spectra similar to the one measured in the experiment.
Motivated by recent experimental observations of Kondo resonances in cobalt atoms on single layer 1T-TaSe2_{2}2​, we theoretically investigate the effect of coupling a U(1) quantum spin liquid with a spinon Fermi surface to a lattice of Anderson impurities. Within the slave-rotor formalism, we find that above a critical coupling strength between the spin liquid and impurity lattice, the spinons hybridize to form heavy quasiparticles near the Fermi level, realizing a {\it spinon Kondo lattice phase} analogous to heavy fermion materials. Using the Bethe-Salpeter equation and accounting for emergent gauge fluctuations, we compute the spectral density and density of states, revealing the formation of spinon-chargon bound states in the spinon Kondo lattice phase. We characterize the thermodynamic and spectroscopic signatures of this phase, demonstrating specific heat and neutron scattering responses distinct from a pure quantum spin liquid. Our findings establish the spinon Kondo lattice as a framework to study the rich physics of spin liquids.
Motivated by recent experimental observations of Kondo resonances in cobalt atoms on single layer $1T\text{\ensuremath{-}}{\mathrm{TaSe}}_{2}$, we theoretically investigate the effect of coupling a U(1) quantum spin liquid with a spinon Fermi surface to a lattice of Anderson impurities. Within the slave-rotor formalism, we find that above a critical coupling strength between the spin liquid and impurity lattice, the spinons hybridize to form heavy quasiparticles near the Fermi level, realizing a spinon Kondo lattice phase analogous to heavy fermion materials. Using the Bethe-Salpeter equation and accounting for emergent gauge fluctuations, we compute the spectral density and density of states, revealing the formation of spinon-chargon bound states in the spinon Kondo lattice phase. We characterize the thermodynamic and spectroscopic signatures of this phase, demonstrating specific heat and neutron scattering responses distinct from a pure quantum spin liquid. Our findings establish the spinon Kondo lattice as a framework to study the rich physics of spin liquids.
We address the problem of a magnetic impurity in a two-dimensional U(1)U(1)U(1) spin liquid where the spinons have gapless excitations near the Fermi surface and are coupled to an emergent gapless gauge field. Using a large N expansion, we analyze the strong coupling behavior and obtain the Kondo temperature which was found to be the same as for a Fermi liquid. In this approximation, we also study the specific heat and the magnetic susceptibility of the impurity. These quantities present no deviations from the Fermi liquid ones, consistent with the notion that the magnetic impurity is only sensitive to the local density of fermionic states.
The authors study the orbital magnetic field induced Landau quantization of a quantum spin liquid with spinon Fermi surface. In the electronic density of states of the quantum spin liquid, the Landau quantization is found to induce a set of band-edge steps, band-edge resonance peaks, or in-gap bound states when the gauge-field fluctuations are negligible, weak, or strong, respectively. The results indicate that the Landau quantization of the spinon Fermi surface can be detected through scanning tunneling microscope measurements.
This work studies the Zeeman magnetic field effect on a quantum spin liquid with a spinon Fermi surface. In the absence of gauge binding, the quantum spin liquid electronic density of states exhibits no Zeeman shift in the threshold energy. As the gauge binding increases, the band edge resonance peaks exhibit a reduced Zeeman shift and eventually have the Zeeman shift direction reversed for a sufficiently large gauge binding. The authors further suggest to use such anomalous Zeeman response to identify the gapless quantum spin liquid phase.