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arXiv:2203.04584 · Physical Review Letters

Resonant Control of Elastic Collisions between Na23K40 Molecules and K40 Atoms

Zhen Su, Huan Yang, Jin Cao, Xinyao Wang, Jun Rui, Bo Zhao, Jian-Wei Pan

Published Jul 13, 2022• 18 citations
arXivHTMLPDF

Abstract

We have demonstrated the resonant control of the elastic scattering cross sections in the vicinity of Feshbach resonances between ^{23}Na^{40}K molecules and ^{40}K atoms by studying the thermalization between them. The elastic scattering cross sections vary by more than 2 orders of magnitude close to the resonance, and can be well described by an asymmetric Fano profile. The parameters that characterize the magnetically tunable s-wave scattering length are determined from the elastic scattering cross sections. The observation of resonantly controlled elastic scattering cross sections opens up the possibility to study strongly interacting atom-molecule mixtures and improve our understanding of the complex atom-molecule Feshbach resonances.

DOI
10.1103/physrevlett.129.033401

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We have demonstrated the resonant control of the elastic scattering cross sections in the vicinity of Feshbach resonances between ^{23}Na^{40}K molecules and ^{40}K atoms by studying the thermalization between them. The elastic scattering cross sections vary by more than 2 orders of magnitude close to the resonance, and can be well described by an asymmetric Fano profile. The parameters that characterize the magnetically tunable s-wave scattering length are determined from the elastic scattering cross sections. The observation of resonantly controlled elastic scattering cross sections opens up the possibility to study strongly interacting atom-molecule mixtures and improve our understanding of the complex atom-molecule Feshbach resonances.
We report the observation of a broad magnetic Feshbach resonance with a large background scattering length in an ultracold fermionic mixture of ^{23}Na^{40}K molecules and ^{40}K atoms, with both species prepared in their lowest hyperfine states. The Feshbach resonance is characterized by measuring resonantly enhanced loss rates and elastic scattering cross sections via cross-species thermalization. The large background scattering length can drive the atom-molecule mixture into the hydrodynamic regime when the magnetic field is far from the resonance. We observe that the center-of-mass motions of the atoms and molecules are phase locked and oscillate with a common frequency due to hydrodynamic drag effects. This broad atom-molecule Feshbach resonance with its large background scattering length opens up a new avenue toward studying strongly interacting fermionic gases with mass imbalance.
In this work we investigate the potential of controlling cold (O(K)−mK) and ultracold (mK-μK) atom-molecule collisions by tuning scattering states across Feshbach resonances using magnetic fields. We are interested in particular in the prospect of suppressing the often undesirable inelastic collisions. The He-O_2 system provides the vehicle for our study. We calculate bound and quasi-bound states of several isotopic combinations, including their Zeeman structure, to reveal the underlaying pattern for easier characterization of quasi-bound states in terms of rigorous and approximately good quantum numbers. These calculations also help us locate the fields at which zero-energy resonances will occur. Scattering calculations are then performed for collisions of 3^He and 4^He with {16}^O_2 at fixed (1 μK) energy but varying magnetic field. The field is varied to sweep the scattering state across resonance. At low and ultralow energies we enter the Wigner threshold regime where the S-partial wave dominates the wavefunction. The cross sections, and the real and imaginary parts of the scattering length, vary dramatically across resonance. Their profiles are used to analyze the resonances. In a highlight of our results we show that dramatic suppression of inelastic cross sections occur for 4^He-{16}^O_2 . The resonances are relatively wide (of order 100 Gauss), with suppression of inelastic scattering over a similarly wide range of fields and for temperatures ranging from 10 mK down to 1 μK. We conclude that under certain conditions it is possible to almost completely eliminate inelastic collisions. This is potentially very important for cooling techniques, such as evaporative and sympathetic cooling, that require efficient elastic cross sections. Suppression of inelastic collisions can not only increase thermalization efficiency but it can also result in longer trap-lifetimes by reducing transitions to untrapable states.
In the absence of inelastic scattering, Feshbach resonances produce poles in scattering lengths and very large peaks in elastic cross-sections. However, inelastic scattering removes the poles. Whenever the resonant state is coupled comparably to the elastic and inelastic channels, the scattering length exhibits only a small oscillation and peaks in cross-sections are significantly suppressed. A resonant scattering length is defined to characterize the amplitude of the oscillation, and is shown to be small for many collisions of ultracold molecules. The results suggest that cross-sections for some ultracold collision processes will be much less sensitive to details of the potential than has been expected.
The s-wave scattering length for elastic collisions between 87Rb{}^{87}\mathrm{Rb}87Rb atoms in the state ∣f,mf〉=∣1,1〉|{f,m}_{f}〉=|1,1〉∣f,mf​〉=∣1,1〉 is measured in the vicinity of a Feshbach resonance near 1007 G. Experimentally, the scattering length is determined from the mean-field-driven expansion of a Bose-Einstein condensate in a homogeneous magnetic field. The scattering length is measured as a function of the magnetic field and agrees with the theoretical expectation. The width of the resonance is determined to be 0.20(3) G, the position of the zero crossing of the scattering length is found at 1007.60(3) G.
We study elastic collisions in an optically trapped spin mixture of fermionic lithium atoms in the presence of magnetic fields up to 1.5 kG by measuring evaporative loss. Our experiments confirm the expected magnetic tunability of the scattering length by showing the main features of elastic scattering according to recent calculations. We measure the zero crossing of the scattering length at 530(3) G which is associated with a predicted Feshbach resonance at approximately 850 G. Beyond the resonance we observe the expected large cross section in the triplet scattering regime.
A modified static exchange model is introduced, it could be useful to control the elastic s-wave scattering length in studying cold-atomic interaction. The theory includes the long-range van der Waals interaction in addition to short-range exchange force. The model is applied on Ps-H system to study the Feshbach resonances e.g. the s-wave elastic phase shifts and the corresponding cross sections at ultracold energies. These are compared with the data obtained using the static exchange model. A very interesting features are observed when we vary the interatomic separation i.e. the strength of dipole-dipole interaction.