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arXiv:2202.09751 · Physical Review A

Floquet analysis of extended Rabi models based on high-frequency expansion

Yibo Liu, Lijun Mao, Yunbo Zhang

Published May 20, 2022• 5 citations
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Abstract

The extended quantum Rabi models make a significant contribution to understanding of the quantum nature of the atom-light interaction. We transform two kinds of extended quantum Rabi model, the anisotropic Rabi model and the asymmetric Rabi model, into the rotating frame and regard them as periodically driven quantum systems. The analytical solutions of the quasienergy spectrum as well as the Floquet modes for both models are constructed by applying the Floquet theory and the high-frequency expansion, which is applied to the nonstroboscopic dynamics of physical observables such as atomic inversion, transverse magnetization, and atom-field correlation. For the anisotropic Rabi model, the quasienergy fits well with the numerical results even when the rotating-wave coupling is in the deep strong-coupling regime $g\ensuremath{\simeq}\ensuremath{\hbar}\ensuremath{\omega}$ if the counter-rotating term is small enough compared to the driving frequency. Avoided level crossing may occur for quasienergy with the same parity when the positive branch spectrum lines for the total excitation number $N$ cross the negative branch lines for $N+2$, while the high-frequency expansion fails to predict this due to the conservation of the total excitation number. Furthermore, we present analytical and numerical studies of the long-time evolution of population and conclude that the analytical method is credible for the population dynamics. For the asymmetric Rabi model, we find that the external bias field which breaks the parity symmetry of the total excitation number tends to cluster the upper and lower branches into two bundles, and the detuning induced gap in the first temporal Brillouin zone shows a quadratic dependence on the bias. Fourier analysis is applied to extract the frequency composition and two-frequency driving behavior is revealed. Varying the bias strength will change the time-averaged value of the oscillation, which shows how the bias competes with the detuning and atom-field coupling in the driving dynamics. Both models prove that treating the Hamiltonian in the rotating frame by Floquet theory gives an alternative tool in the study of interaction between atom and light.

DOI
10.1103/physreva.105.053717

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The Jaynes–Cummings model with or without rotating-wave approximation plays a major role to study the interaction between atom and light. We investigate the Jaynes–Cummings model beyond the rotating-wave approximation. Treating the counter-rotating terms as periodic drivings, we solve the model in the extended Floquet space. It is found that the full energy spectrum folded in the quasi-energy bands can be described by an effective Hamiltonian derived in the high-frequency regime. In contrast to the Z 2 symmetry of the original model, the effective Hamiltonian bears an enlarged U(1) symmetry with a unique photon-dependent atom-light detuning and coupling strength. We further analyze the energy spectrum, eigenstate fidelity and mean photon number of the resultant polaritons, which are shown to be in accordance with the numerical simulations in the extended Floquet space up to an ultra-strong coupling regime and are not altered significantly for a finite atom-light detuning. Our results suggest that the effective model provides a good starting point to investigate the rich physics brought by counter-rotating terms in the frame of Floquet theory.
We construct a systematic high-frequency expansion for periodically driven quantum systems based on the Brillouin-Wigner (BW) perturbation theory, which generates an effective Hamiltonian on the projected zero-photon subspace in the Floquet theory, reproducing the quasienergies and eigenstates of the original Floquet Hamiltonian up to desired order in $1/\ensuremath{\omega}$, with $\ensuremath{\omega}$ being the frequency of the drive. The advantage of the BW method is that it is not only efficient in deriving higher-order terms, but even enables us to write down the whole infinite series expansion, as compared to the van Vleck degenerate perturbation theory. The expansion is also free from a spurious dependence on the driving phase, which has been an obstacle in the Floquet-Magnus expansion. We apply the BW expansion to various models of noninteracting electrons driven by circularly polarized light. As the amplitude of the light is increased, the system undergoes a series of Floquet topological-to-topological phase transitions, whose phase boundary in the high-frequency regime is well explained by the BW expansion. As the frequency is lowered, the high-frequency expansion breaks down at some point due to band touching with nonzero-photon sectors, where we find numerically even more intricate and richer Floquet topological phases spring out. We have then analyzed, with the Floquet dynamical mean-field theory, the effects of electron-electron interaction and energy dissipation. We have specifically revealed that phase transitions from Floquet-topological to Mott insulators emerge, where the phase boundaries can again be captured with the high-frequency expansion.
The PT -symmetric semiclassical Rabi model explores the fundamental interaction between a two-level atom and a classical field, revealing novel phenomena in open systems through the inclusion of non-Hermitian terms. We propose a single similarity transformation that yields an effective Hamiltonian in rotating-wave approximation, enabling an analytical solution. The phase boundary of the PT -broken phase, derived from the analytical eigenvalues, closely matches the numerically exact one over a wide range of atomic frequencies, demonstrating the effectiveness of the analytical approach, especially at the main resonance. The Floquet parity operator is also introduced, providing a deeper physical understanding of the emergence of the PT -broken phase. Furthermore, by analyzing the dynamics of excited-state population, we observe several stable oscillations in the Fourier spectrum, demonstrating the applicability of the analytical method beyond the single-photon resonance region. The Bloch-Siegert shift is also discussed, and surprisingly, resembles its Hermitian counterpart, except for the higher-order terms in the coupling strength. The present analytical treatment provides a concise and accurate description of the main physics of this non-Hermitian atom-field interaction system.
We theoretically study the dynamics and resonance shift of the Rabi model with frequency modulation, i.e., the Rabi model driven additionally by a slow longitudinal field, by using the counterrotating-hybridized rotating-wave (CHRW) method, aiming to illustrate the effects of the counterrotating (CR) terms of the transverse field. The CHRW method is based on a unitary transformation and reduces the aperiodic Hamiltonian to an effective periodic Hamiltonian that can be efficiently treated by Floquet theory. The validity of the effective Hamiltonian and widely used rotating-wave approximation (RWA) Hamiltonian is carefully examined compared to the numerically exact results over a wide parameter range. It is found that the effective Hamiltonian gives a correct description, while the RWA breaks down in the strong driving regime. Interestingly, we show that under certain conditions the longitudinal field can be used to modify resonance widths such that resonance widths can be comparable to the magnitude of the Bloch-Siegert (BS) shift, which in turn makes the CR-induced BS shift significant and leads to the complete breakdown of the RWA even in a moderately strong driving regime (in which the RWA holds for the Rabi model without frequency modulation). In addition, by using the effective Hamiltonian, we can efficiently access resonance positions for the bichromatically driven qubit and study how the resonance shifts due to the combined effects of the CR terms and frequency modulation. For a weak longitudinal field, we show that resonance positions can be analytically calculated from the effective Rabi frequency for the effective Hamiltonian, which are in excellent agreement with the numerically exact results.
Strong periodic driving of cavity-quantum electrodynamics (QED) in the ultrastrong-coupling regime creates nonequilibrium states whose dissipation is governed by Floquet quasienergies rather than undriven dressed resonances. However, modeling such a regime is a significant theoretical challenge, including a number of subtle problems such as the need to ensure gauge invariance for truncated matter-cavity systems with time-dependent driving. To fill this theoretical gap, we introduce a nonsecular Floquet generalized master equation framework for strongly driven open cavity-QED systems, formulated in the dressed basis of the quantum Rabi model and applicable to structured reservoirs without rotating-wave approximations. Our theory can thus model Floquet-driven dynamics in open ultrastrong-coupling cavity-QED, and demonstrates a wide range of quantum state control. Using strong optical pumping and parametric mechanical modulation, we compute long-time populations, fluorescence spectra, and the Floquet-Liouville eigenspectra, resolving observable resonances into hybridized quasienergy channels and decay rates. By systematically comparing with conventional time-independent dressed-basis generalized master equations, we show that static approaches only reproduce steady-state populations in restricted excitation regimes, and fail for frequency-resolved observables and break down under appropriate Floquet engineering, surprisingly, even for spectrally flat baths. Structured environments, such as Lorentzian-Ohmic reservoirs, further amplify these discrepancies through sideband-selective decay. Our results demonstrate that dissipation in driven ultrastrong cavity-QED is intrinsically quasienergy resolved and we establish Floquet-dissipative theory as an accurate and powerful framework for predicting spectra, controlling decay pathways, and engineering nonequilibrium quantum states and reservoirs.