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arXiv:2202.00797 · Physical Review Research

Proposal for a cavity-induced measurement of the exchange coupling in quantum dots

Florian Ginzel, Guido Burkard

Published Jul 18, 2022• 3 citations
arXivHTMLPDF

Abstract

In spin qubit arrays the exchange coupling can be harnessed to implement two-qubit gates and to realize intermediate-range qubit connectivity along a spin bus. In this work, we propose a scheme to characterize the exchange coupling between electrons in adjacent quantum dots. We investigate theoretically the transmission of a microwave resonator coupled to a triple quantum dot occupied by two electrons. We assume that the right quantum dot (QD) is always occupied by one electron while the second electron can tunnel between the left and center QDs. If the two electrons are in adjacent dots they interact via the exchange coupling. By means of analytical calculations we show that the transmission profile of the resonator directly reveals the value of the exchange coupling strength between two electrons. From perturbation theory up to second order we conclude that the exchange can still be identified in the presence of magnetic gradients. A valley splitting comparable to the interdot tunnel coupling will lead to further modifications of the cavity transmission dips that also depend on the valley phases.

DOI
10.1103/physrevresearch.4.033048

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In spin qubit arrays the exchange coupling can be harnessed to implement two-qubit gates and to realize intermediate-range qubit connectivity along a spin bus. In this work, we propose a scheme to characterize the exchange coupling between electrons in adjacent quantum dots. We investigate theoretically the transmission of a microwave resonator coupled to a triple quantum dot occupied by two electrons. We assume that the right quantum dot (QD) is always occupied by one electron while the second electron can tunnel between the left and center QDs. If the two electrons are in adjacent dots they interact via the exchange coupling. By means of analytical calculations we show that the transmission profile of the resonator directly reveals the value of the exchange coupling strength between two electrons. From perturbation theory up to second order we conclude that the exchange can still be identified in the presence of magnetic gradients. A valley splitting comparable to the interdot tunnel coupling will lead to further modifications of the cavity transmission dips that also depend on the valley phases.
We investigate the behavior of qubits consisting of three electron spins in double and triple quantum dots subject to external electric fields. Our model includes two independent bias parameters, $\ensuremath{\varepsilon}$ and ${\ensuremath{\varepsilon}}_{M}$, which both couple to external electromagnetic fields and can be controlled by gate voltages applied to the quantum dot structures. By varying these parameters, one can switch the qubit type by shifting the energies in the single quantum dots, thus changing the electron occupancy in each dot. Starting from the asymmetric resonant exchange qubit with a (2,0,1) and (1,0,2) charge admixture, one can smoothly cross over to the resonant exchange qubit with a detuned (1,1,1) charge configuration, and to the exchange-only qubit with the same charge configuration but equal energy levels down to the hybrid qubits with (1,2,0) and (0,2,1) charge configurations. Here, (l,m,n)(l,m,n)(l,m,n) describes a configuration with lll electrons in the left dot, mmm electrons in the center dot, and nnn electrons in the right dot. We first focus on random electromagnetic field fluctuations, i.e., ``charge noise,'' at each quantum dot resulting in dephasing of the qubit, and we provide a complete map of the resulting dephasing time as a function of the bias parameters. We pay special attention to the so-called sweet spots and double sweet spots of the system, which are least susceptible to noise. In the second part, we investigate the coupling of the qubit system to the coherent quantized electromagnetic field in a superconducting strip-line cavity, and we also provide a complete map of the coupling strength as a function of the bias parameters. We analyze the asymmetric qubit-cavity coupling via $\ensuremath{\varepsilon}$ and the symmetric coupling via ${\ensuremath{\varepsilon}}_{M}$.
Semiconductor-based spin qubits embedded into a superconducting microwave cavity constitute a fast-progressing and promising platform for realizing fast and fault-tolerant qubit control with long-range two-qubit coupling. The flopping-mode spin qubit consists of a single electron in a double quantum dot; it combines a charge qubit with a spin qubit. With its strong and tunable cavity coupling, the flopping-mode qubit is proven to be well suited for low-power qubit control and cavity-mediated long-range quantum gates. The singlet-triplet (ST) and exchange-only (EO) qubits are multielectron realizations that go without broadband control and are protected from some types of noise, but are challenging to couple to each other and to microwave cavities. We combine the flopping-mode concept with the ST and EO qubits and propose two new flopping-mode qubits that consist of three (four) quantum dots, occupied by two (three) electrons near the ( 1 , 0 , 1 ) ↔ ( 0 , 1 , 1 ) [ ( 1 , 0 , 1 , 1 ) ↔ ( 0 , 1 , 1 , 1 ) ] charge transition. The two-electron system augments the ST 0 spin qubit with a charge qubit that interacts transversally and longitudinally with a cavity. Both couplings are highly tunable, and the longitudinal coupling distinguishes the flopping-mode ST qubit from the regular flopping-mode qubit. The longitudinal coupling allows for nondissipative universal control similar to superconducting transmon qubits. The EO flopping-mode qubit comprises four dots occupied by three electrons and opens a new possibility to perform two-qubit gates for EO qubits that are challenging to perform directly with the exchange coupling. We use input-output theory to provide means of extracting the coupling strengths from cavity transmission data.
Tunneling in a quantum coherent structure is not restricted to only nearest neighbors. Hopping between distant sites is possible via the virtual occupation of otherwise avoided intermediate states. Here we report the observation of long-range transitions in the transport through three quantum dots coupled in series. A single electron is delocalized between the left and right quantum dots, while the center one remains always empty. Superpositions are formed, and both charge and spin are exchanged between the outermost dots. The delocalized electron acts as a quantum bus transferring the spin state from one end to the other. Spin selection is enabled by spin correlations. The process is detected via the observation of narrow resonances which are insensitive to Pauli spin blockade.
In the last years, the electron spin in quantum dots has become a most promising candidate for the realization of qubits, the basic element for quantum computation. In quantum dot spin qubits the exchange interaction implements a fundamental two qubit gate, which originates in the Coulomb interaction and the Pauli principle. Compared to single qubit gates, the exchange based gates are much faster and easier to control locally, motivating the solely exchange energy based quantum computation. The control is based on the exponential sensitivity of the exchange energy on the interparticle distance. Manipulation then can proceed, for example, shifting the single particle states electrically or compressing them magnetically. The practical manipulation schemes require quantitative knowledge of the exchange energy. The spin-orbit interaction plays an important role in this nano-system. Indeed the usual exchange interaction changes its magnitude, while a new term, called anisotropic exchange, appears. In this thesis we propose an accurate effective spin Hamiltonian for modeling spin-orbit-induced spin dynamics in the presence of the magnetic field. We have also performed numerically exact calculations of the isotropic and anisotropic exchange coupling in realistic two-electron GaAs coupled quantum dots in the presence of both Dresselhaus and Bychkov-Rashba spin-orbit interactions. The numerics allow us to establish the goodness of our model and to see the limits of previous statements. Furthermore we find that in zero magnetic field the second-order spin-orbit effects are absent at all interdot couplings.
Both quantum transport measurements in the Pauli blockade regime and microwave cavity transmission measurements are important tools for spin-qubit readout and characterization. Based on a generalized input-output theory we derive a theoretical framework to investigate how a double quantum dot (DQD) in a transport setup interacts with a coupled microwave resonator while the current through the DQD is rectified by Pauli blockade. We show that the output field of the resonator can be used to infer the leakage current and thus obtain insight into the blockade mechanisms. In the case of a silicon DQD, we show how the valley quasidegeneracy can impose limitations on this scheme. We also demonstrate that a large number of unknown DQD parameters including (but not limited to) the valley splitting can be estimated from the resonator response simultaneous to a transport experiment, providing more detailed knowledge about the microscopic environment of the DQD. Furthermore, we describe and quantify a back action of the resonator photons on the steady-state leakage current.
Quantum physics describes the universe on a microscopic scale. Even though this scale is not accessible without complex experimental setups, quantum effects are respon- sible for the properties of matter and in some instances we have learned to exploit them technologically. A modern computer constituted of transistors passively utilizes the quantum nature of charge carriers in the band structure of semiconductors to encode and process information. Although such a classical computer is a formidable tool already, what could be achieved with active control over the quantum states in the computer is an intriguing question. This is the idea of the quantum computer, which offers an entirely new paradigm of computing by encoding information in quantum binary digits (qubits). Indeed, for several applications it has been shown that a quantum computer is superior to its classical counterpart, even though its realization remains elusive up to date. One candidate to host qubits are gate-defined semiconductor quantum dots, confin- ing single or few charge carriers with spin. The spin of a single confined electron is a quantum two-level system which can be manipulated and measured, allowing the storage and processing of quantum information. This thesis can be viewed as part of the endeavor to give birth to quantum computers based on semiconductor spin qubits. It primarily focuses on the challenge to enable scalable architectures of well-characterized qubits. In the first part, spin shuttling is investigated. This denotes the coherent transport of a single spin between spatially separate nodes of a quantum processor, driven by a time-dependent electric potential. The object of study is a minimal version of a bucket- brigade-like spin shuttling between two quantum dots. The probability of maintaining the spin state is identified as figure of merit and the effect of spin-orbit interaction and the Zeeman effect in an inhomogeneous magnetic field is explored with analytical and numerical methods. Special attention is paid to the repercussions of near-degenerate valleys. The second part of the thesis addresses the challenge to probe the microscopic properties of a quantum dot array, which is a crucial first step before any quantum operation can be performed. The transmission of a microwave resonator coupled to a triple quantum dot occupied by two electrons is investigated, and a scheme to infer the exchange interaction between electrons in adjacent quantum dots is proposed. By means of analytical derivations it is shown that the transmission profile of the resonator directly reveals the value of the exchange coupling strength between two electrons. This holds even if magnetic gradients or a valley splitting comparable to the inter-dot tunnel coupling are included. Subsequently, quantum transport measurements in the Pauli blockade regime are modelled in the presence of a microwave resonator, bringing together two powerful techniques to probe quantum dots. Based on generalized input-output theory, a theoretical framework is derived to investigate how a double quantum dot in a transport setup interacts with a coupled microwave resonator while the current through the double qauntum dot is rectified by Pauli blockade. It is shown that the output field of the resonator can be used to infer the leakage current and thus obtain insight into the blockade mechanisms and to estimate a large number of parameters of the quantum dots. Furthermore, the back-action of the resonator photons on the steady state leakage current is described and quantified. In the context of Pauli blockade, the spin and valley physics of bilayer graphene quantum dots in the few-electron regime is touched upon, describing a situation where spin blockade is observed despite the presence of the valleys. In the final part of the thesis, the attention is shifted towards the readout of the spin qubits. A new paradigm of dispersive readout is devised, which is performed while the qubit dephases, implementing a measurement in the x-basis. Laplace transforming the time dependent cavity response allows a separation of contributions from multiple qubits coupled to the same resonator. Thus, they can be read out simultaneously in a single shot. Modelling silicon spin qubits, as an example, results in in a readout time that compares favourably to conventional dispersive readout with comparable fidelity, even for a single qubit. With an auxiliary qubit the readout scheme can be extended to a quantum non-demolition measurement.