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arXiv:2201.07074 · Scientific Reports

Geometry of rare regions behind Griffiths singularities in random quantum magnets

István A. Kovács, Ferenc Iglói

Published Jan 20, 2022• 3 citations
arXivHTMLPDF

Abstract

In many-body systems with quenched disorder, dynamical observables can be singular not only at the critical point, but in an extended region of the paramagnetic phase as well. These Griffiths singularities are due to rare regions, which are locally in the ordered phase and contribute to a large susceptibility. Here, we study the geometrical properties of rare regions in the transverse Ising model with dilution or with random couplings and transverse fields. In diluted models, the rare regions are percolation clusters, while in random models the ground state consists of a set of spin clusters, which are calculated by the strong disorder renormalization method. We consider the so called energy cluster, which has the smallest excitation energy and calculate its mass and linear extension in one-, two- and three-dimensions. Both average quantities are found to grow logarithmically with the linear size of the sample. Consequently, the energy clusters are not compact: for the diluted model they are isotropic and tree-like, while for the random model they are quasi-one-dimensional.

DOI
10.1038/s41598-022-05096-z

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In many-body systems with quenched disorder, dynamical observables can be singular not only at the critical point, but in an extended region of the paramagnetic phase as well. These Griffiths singularities are due to rare regions, which are locally in the ordered phase and contribute to a large susceptibility. Here, we study the geometrical properties of rare regions in the transverse Ising model with dilution or with random couplings and transverse fields. In diluted models, the rare regions are percolation clusters, while in random models the ground state consists of a set of spin clusters, which are calculated by the strong disorder renormalization method. We consider the so called energy cluster, which has the smallest excitation energy and calculate its mass and linear extension in one-, two- and three-dimensions. Both average quantities are found to grow logarithmically with the linear size of the sample. Consequently, the energy clusters are not compact: for the diluted model they are isotropic and tree-like, while for the random model they are quasi-one-dimensional.
We have developed a very efficient numerical algorithm of the strong disorder renormalization group method to study the critical behaviour of the random transverse field Ising model, which is a prototype of random quantum magnets. With this algorithm we can renormalize an N-site cluster within a time NlogN, independently of the topology of the graph, and we went up to N ∼ 4 × 10(6). We have studied regular lattices with dimension D ≤ 4 as well as Erdős-Rényi random graphs, which are infinite dimensional objects. In all cases the quantum critical behaviour is found to be controlled by an infinite disorder fixed point, in which disorder plays a dominant role over quantum fluctuations. As a consequence the renormalization procedure as well as the obtained critical properties are asymptotically exact for large systems. We have also studied Griffiths singularities in the paramagnetic and ferromagnetic phases and generalized the numerical algorithm for other random quantum systems.
Abstract In crystalline magnets, interaction randomness is usually thought as a negative factor preventing interesting quantum phenomena to occur. However, intriguing interplay between randomness and quantumness can also leads to unique phenomena in the strongly correlated materials. Among others, the random transverse-field Ising spin chain (RTIC) hosts a renowned quantum Griffiths phase. Although the RTIC model has been regarded as a toy model for long, here we materialize this model with the compound PrTiNbO6, which has a disordered ground state with pronounced quantum fluctuations and continuous spin excitations. The observed anomalous spin dynamics of PrTiNbO6 can be accounted by the RTIC model with a consistent set of parameters determined from fitting the thermodynamic data, and it is ascribed to the quantum Griffiths rare regions in the system. Our results provide a concrete example of quantum Griffiths magnet, and offer an ideal experimental platform for investigating the dynamical properties of random many-body system.
We study the ±J transverse-field Ising spin-glass model at zero temperature on d-dimensional hypercubic lattices and in the Sherrington-Kirkpatrick (SK) model, by series expansions around the strong-field limit. In the SK model and in high dimensions our calculated critical properties are in excellent agreement with the exact mean-field results, surprisingly even down to dimension d=6, which is below the upper critical dimension of d=8. In contrast, at lower dimensions we find a rich singular behavior consisting of critical and Griffiths-McCoy singularities. The divergence of the equal-time structure factor allows us to locate the critical coupling where the correlation length diverges, implying the onset of a thermodynamic phase transition. We find that the spin-glass susceptibility as well as various power moments of the local susceptibility become singular in the paramagnetic phase before the critical point. Griffiths-McCoy singularities are very strong in two dimensions but decrease rapidly as the dimension increases. We present evidence that high enough powers of the local susceptibility may become singular at the pure-system critical point.
We use numerical linked cluster expansions (NLCEs) to study the site-diluted transverse-field Ising model on the square lattice at T=0. NLCE with a self-consistent mean field on the boundary of the clusters is used to obtain the ground-state magnetization, susceptibility, and structure factor as a function of transverse field h and exchange constant J. Adding site dilution to the model turns NLCE into a series expansion in the dilution parameter p. Studying the divergence of the structure factor allows us to establish the phase diagram in the h/J and p plane. By studying the magnetization of the system in a longitudinal field, we investigate the Griffiths-McCoy singularities. We find that the magnetization develops nonlinearities in the Griffiths phase with exponents that vary continuously with h. Additionally, the probability distribution of the local susceptibility develops long tails in the Griffiths phase, which is studied in terms of its moments.
In random quantum magnets, like the random transverse Ising chain, low energy excitations are localized in rare regions and there are only weak correlations between them. It is an open question whether these correlations are relevant in the sense of the renormalization group. To answer this question, we calculate the distribution of the excitation energy of the random transverse Ising chain in the disordered Griffiths phase with high numerical precision by the strong disorder renormalization group method and---for shorter chains---by free-fermion techniques. Asymptotically, the two methods give identical results, which are well fitted by the Fr\'echet limit law of the extremes of independent and identically distributed random numbers. Considering the finite size corrections, the two numerical methods give very similar results, but these differ from the correction term for uncorrelated random variables, indicating that the weak correlations between low-energy excitations in random quantum magnets are relevant.
The infinite-disorder fixed point of the random transverse-field Ising model is expected to control the critical behavior of a large class of random quantum and stochastic systems having an order parameter with discrete symmetry. Here we study the model on the square lattice with a very efficient numerical implementation of the strong disorder renormalization group method, which makes us possible to treat finite samples of linear size up to L=2048L=2048L=2048. We have calculated sample dependent pseudocritical points and studied their distribution, which is found to be characterized by the same shift and width exponent: $\ensuremath{\nu}=1.24(2)$. For different types of disorder the infinite-disorder fixed point is shown to be characterized by the same set of critical exponents, for which we have obtained improved estimates: x=0.982(15)x=0.982(15)x=0.982(15) and $\ensuremath{\psi}=0.48(2)$. We have also studied the scaling behavior of the magnetization in the vicinity of the critical point as well as dynamical scaling in the ordered and disordered Griffiths phases.