The Kitaev model is a fascinating example of an exactly solvable model displaying a spin-liquid ground state in two dimensions. However, deviations from the original Kitaev model are expected to appear in real materials. In this Letter, we investigate the fate of Kitaev's spin liquid in the presence of disorder-bond defects or vacancies-for an extended version of the model. Considering static flux backgrounds, we observe a power-law divergence in the low-energy limit of the density of states with a nonuniversal exponent. We link this power-law distribution of energy scales to weakly coupled droplets inside the bulk, in an uncanny similarity to the Griffiths phase often present in the vicinity of disordered quantum phase transitions. If time-reversal symmetry is broken, we find that power-law singularities are tied to the destruction of the topological phase of the Kitaev model in the presence of bond disorder alone. However, there is a transition from this topologically trivial phase with power-law singularities to a topologically nontrivial one for weak to moderate site dilution. Therefore, diluted Kitaev materials are potential candidates to host Kitaev's chiral spin-liquid phase.
The Kitaev model is a fascinating example of an exactly solvable model displaying a spin-liquid ground state in two dimensions. However, deviations from the original Kitaev model are expected to appear in real materials. In this Letter, we investigate the fate of Kitaev's spin liquid in the presence of disorder-bond defects or vacancies-for an extended version of the model. Considering static flux backgrounds, we observe a power-law divergence in the low-energy limit of the density of states with a nonuniversal exponent. We link this power-law distribution of energy scales to weakly coupled droplets inside the bulk, in an uncanny similarity to the Griffiths phase often present in the vicinity of disordered quantum phase transitions. If time-reversal symmetry is broken, we find that power-law singularities are tied to the destruction of the topological phase of the Kitaev model in the presence of bond disorder alone. However, there is a transition from this topologically trivial phase with power-law singularities to a topologically nontrivial one for weak to moderate site dilution. Therefore, diluted Kitaev materials are potential candidates to host Kitaev's chiral spin-liquid phase.
Frustrated magnetism is a very active research topic in condensed matter physics. The competition between different ground states often leads to a suppression of the ordering temperature and opens up the possibility that novel states emerge. One state of particular interest are the spin liquids, for which we find no broken symmetry down to T —› 0, where T is the temperature. Moreover, theses states show topological order and are notable for their peculiar features, such as long-range entanglement and the emergence of fractionalized excitations. The Kitaev model is a fascinating example of an exactly solvable model displaying a spin-liquid ground state in two dimensions. In real materials, however, deviations from the original Kitaev model are expected to appear, and we discuss relevant perturbations here. In this work, we investigate the fate of Kitaevs spin-liquid in the presence of disorder bond defects or vacancies for an extended version of the model. Considering static flux backgrounds, we observe a power-law divergence in the low-energy limit of the density of states, with a non-universal exponent. We link this power-law distribution of energy scales to weakly coupled droplets inside the bulk, in an uncanny similarity to the Griffiths phase often present in the vicinity of disordered quantum phase transitions. If time-reversal symmetry is broken, we find that power-law singularities are tied to the destruction of the topological phase of the Kitaev model in the presence of bond disorder alone. For weak to moderate site dilution, there is a transition from this topologically trivial phase with power-law singularities to a topologically non-trivial one. Therefore, diluted Kitaev materials are potential candidates to host Kitaevs chiral spin-liquid phase.
We investigate the properties of the Kitaev honeycomb model with both site dilution and exchange randomness. Embarking on this work, we review disorder in some strongly correlated electron systems, including spin-½ and spin-1 Heisenberg antiferromagnetic chains, two dimensional Heisenberg antiferromagnets, the cuprates and graphene. We outline some aspects of resonating valence bond phases, valence bond solids, spin liquids and quantum computation that are pertinent to an understanding of the Kitaev model. The properties of the Kitaev model without disorder are discussed and it is found to be a critical spin liquid, with algebraic correlations in two spin operators sigma^{alpha}_{i}sigma^{alpha}_{j}, where i and j are either end of a link of type alpha = x, y or z on the honeycomb lattice. The Kitaev model is exactly solvable and we show that this remains so in the presence of site dilution and exchange randomness. We find that vacancies bind a flux. In the gapped phase, a vacancy forms an effective paramagnetic moment. With two or more vacancies we describe the interaction of their effective moments and show that a finite density of vacancies leads to a divergent macroscopic susceptibility at small fields. In the gapless phase the effective moment has a susceptibility that is, to leading order at small fields, chi(h)~log(1/h). Interaction between the moments from two vacancies on opposite sublattices cuts off this divergence in susceptibility at a large but finite constant. Two vacancies on the same sublattice behave quite differently and we find the combined susceptibility is parametrically larger than that of an isolated vacancy, chi(h)sim [h(log(1/h))^{3/2}]^{-1}. We also investigate the effects of slowly varying, quenched disorder in exchange coupling. We demonstrate that this does not qualitatively affect the susceptibility but show that the heat capacity C ~ T^{2/z}, where z is a measure of the disorder and increases from one with increasing disorder strength.
We investigate the properties of the Kitaev honeycomb model with both site dilution
and exchange randomness. Embarking on this work, we review disorder in some strongly correlated electron systems, including spin-½ and spin-1 Heisenberg antiferromagnetic chains, two dimensional Heisenberg antiferromagnets, the cuprates and graphene. We outline some aspects of resonating valence bond phases, valence bond solids, spin liquids and quantum computation that are pertinent to an understanding of the Kitaev model. The properties of the Kitaev model without disorder are discussed and it is found to be a critical spin liquid, with algebraic correlations in two spin operators sigma^{alpha}_{i}sigma^{alpha}_{j}, where i and j,/em> are either end of a link of type alpha = x, y or z on the honeycomb lattice.
The Kitaev model is exactly solvable and we show that this remains so in the presence of site dilution and exchange randomness. We find that vacancies bind a flux. In the gapped phase, a vacancy forms an effective paramagnetic moment. With two or more vacancies we describe the interaction of their effective moments and show that a finite density of vacancies leads to a divergent macroscopic susceptibility at small fields.
In the gapless phase the effective moment has a susceptibility that is, to leading order at small fields, chi(h)~log(1/h). Interaction between the moments from two vacancies on opposite sublattices cuts off this divergence in susceptibility at a large but finite constant. Two vacancies on the same sublattice behave quite differently and we find the combined susceptibility is parametrically larger than that of an isolated vacancy, chi(h)sim [h(log(1/h))^{3/2}]^{-1}.
We also investigate the effects of slowly varying, quenched disorder in exchange coupling. We demonstrate that this does not qualitatively affect the susceptibility but show that the heat capacity C ~ T^{2/z}, where z is a measure of the disorder and increases from one with increasing disorder strength.
A quantum spin liquid is a magnetic phase of matter that is remarkable for its ground state long-range entanglement and fractional excitations. A quantum spin liquid appears in the well-known Kitaev honeycomb spin-half model. In a magnetic field, there is a phase transition to a topological phase with an energy gap in the bulk and chiral Majorana fermions at the edge. However, recent nuclear magnetic resonance experiments suggest excitations without a gap in this phase, signalled by the cubic temperature dependence of the spin-lattice relaxation rate at low temperatures. In this work, I propose a mechanism to account for this experimental result. I use the localization of chiral Majorana modes in defects to explain the presence of gapless modes in the bulk. Treating the weak interaction between the chiral modes in the defects within a mean-field approximation, I find that these modes remain gapless when the interaction is below a critical value that depends on the magnetic field strength. I used the effective low-energy theory to calculate the spin-lattice relaxation rate and found a behavior that agrees with the experimental result.
The Kitaev honeycomb model supports gapless and gapped quantum spin liquid phases. Its exact solvability relies on extensively many locally conserved quantities. Any real-world manifestation of these phases would include imperfections in the form of disorder and interactions that break integrability. We show that the latter qualitatively alters the properties of vacancies in the gapless Kitaev spin liquid: (i) Isolated vacancies carry a magnetic moment, which is absent in the exactly solvable case. (ii) Pairs of vacancies on even or opposite sublattices gap each other with distinct power laws that reveal the presence of emergent gauge flux.
The Kitaev spin liquid, stabilized as the ground state of the Kitaev honeycomb model, is a paradigmatic example of a topological Z2 quantum spin liquid. The fate of the Kitaev spin liquid in presence of an external magnetic field is at present, a subject of intense scrutiny due to recent experimental signatures pointing to a Z2 topological phase in certain materials, as well as theoretical studies predicting the emergence of a quantum spin liquid phase of debated nature. In this work, we employ hierarchical mean-field theory, a method based on the use of clusters preserving relevant symmetries and short-range quantum correlations, to investigate the quantum phase diagram of the antiferromagnetic Kitaev's model in a [111] magnetic field. By using clusters of 24 sites, we predict that the Kitaev spin liquid transits through two intermediate phases, characterized by emerging stripe and chiral orders, respectively, before entering the trivial partially polarized phase, differing from previous studies. We assess our results by performing exact diagonalization and computing the scaling of different observables, including the many-body Chern number and other topological quantities, thus establishing hierarchical mean-field theory as a method to study models of frustrated quantum magnetism potentially hosting topological quantum spin liquids.