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arXiv:2112.06976 · Physical review. B./Physical review. B

General memory kernels and further corrections to the variational path integral approach for the Bogoliubov-Fröhlich Hamiltonian

T. Ichmoukhamedov, Jacques Tempere

Published Mar 4, 2022• 5 citations
arXivHTMLPDF

Abstract

The celebrated variational path integral approach to the polaron problem shows remarkable discrepancies with diagrammatic Monte Carlo (DiagMC) for the Bogoliubov-Fr\"ohlich Hamiltonian which describes an impurity weakly coupled to a Bose condensed atomic gas. It has been shown both by a renormalization group approach and by the method of correlated Gaussian wave functions that the model has a subtle UV divergence caused by quantum fluctuations, which are not captured within Feynman's approach. In this work we address the issues with Feynman's approach and show that by extending the model action to a more general form, and by considering higher-order corrections beyond the Jensen-Feynman inequality, a good agreement with DiagMC can be obtained.

DOI
10.1103/physrevb.105.104304

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The celebrated variational path integral approach to the polaron problem shows remarkable discrepancies with diagrammatic Monte Carlo (DiagMC) for the Bogoliubov-Fr"ohlich Hamiltonian which describes an impurity weakly coupled to a Bose condensed atomic gas. It has been shown both by a renormalization group approach and by the method of correlated Gaussian wave functions that the model has a subtle UV divergence caused by quantum fluctuations, which are not captured within Feynman's approach. In this work we address the issues with Feynman's approach and show that by extending the model action to a more general form, and by considering higher-order corrections beyond the Jensen-Feynman inequality, a good agreement with DiagMC can be obtained.
The system of a charged impurity in an interacting Bose gas has gained significant attention due to the long-range ion-atom interactions and the study of transport properties. Here, the ground state energy of a charged Bose polaron is calculated within the Bogoliubov approximation for both the Fröhlich and beyond-Fröhlich Hamiltonians using a generalized Feynman variational path-integral approach, which obtained accurate results for other polaron problems. The generalized approach, which was used to improve the energy result for the neutral polaron, has resulted in a minor improvement, indicating that Feynman's approach is sufficient when the impurity-boson interaction is long-range. Beyond-Fröhlich corrections results in the emergence of a divergence in the polaronic energy indicating a transition between the repulsive and attractive polaron regime. The path-integral approach with the beyond-Fröhlich Hamiltonian is also compared to a field-theory calculation from Christensen et al, 2021. The validity of the Bogoliubov approximation is investigated. The optical absorption has also been calculated within the Bogoliubov approximation for weak ion-atom interactions, and the effect of finite temperature has been studied. We show that the coupling of the ion to an oscillating external electric field offers a straigtforward experimental probe for the charged polaron in a Bose gas, different from but complementary to existing spectroscopic techniques.
An impurity immersed in a Bose-Einstein condensate is no longer accurately described by the Fr\"ohlich Hamiltonian as the coupling between the impurity and the boson bath gets stronger. We study the dominant effects of the two-phonon terms beyond the Fr\"ohlich model on the ground-state properties of the polaron using Feynman's variational path-integral approach. The previously reported discrepancy in the effective mass between the renormalization group approach and this theory is shown to be absent in the beyond-Fr\"ohlich model on the positive side of the Feshbach resonance. Self-trapping, characterized by a sharp and dramatic increase of the effective mass, is no longer observed for the repulsive polaron once the two-phonon interactions are included. For the attractive polaron we find a divergence of the ground-state energy and effective mass at weaker couplings than previously observed within the Fr\"ohlich model.
The Fr\"ohlich model describes the interaction of a mobile impurity with a surrounding bath of phonons which leads to the formation of a quasiparticle, the polaron. In this paper an efficient renormalization group approach is presented which provides a description of Fr\"ohlich polarons in all regimes ranging from weak to strong coupling. The extended renormalization group approach introduced here is capable of predicting ground state properties for arbitrarily small impurity masses. This allows us to obtain the full phase diagram of the Fr\"ohlich Hamiltonian, which we present concretely for the Bogoliubov-Fr\"ohlich model originally introduced to describe ultracold impurities in a Bose-Einstein condensate. For this model, whose regime of validity in ultracold quantum gases is the subject of debate, we benchmark our method by comparison of the ground state energy to recent diagrammatic quantum Monte Carlo calculations.
When a mobile impurity interacts with a many-body system, such as a phonon bath, a polaron is formed. Despite the importance of the polaron problem for a wide range of physical systems, a unified theoretical description valid for arbitrary coupling strengths is still lacking. Here we develop a renormalization group approach for analyzing a paradigmatic model of polarons, the so-called Fröhlich model, and apply it to a problem of impurity atoms immersed in a Bose-Einstein condensate of ultra cold atoms. Polaron energies obtained by our method are in excellent agreement with recent diagrammatic Monte Carlo calculations for a wide range of interaction strengths. They are found to be logarithmically divergent with the ultra-violet cut-off, but physically meaningful regularized polaron energies are also presented. Moreover, we calculate the effective mass of polarons and find a smooth crossover from weak to strong coupling regimes. Possible experimental tests of our results in current experiments with ultra cold atoms are discussed.
We consider two large polaron systems that are described by a Fröhlich type of Hamiltonian, namely the Bose–Einstein condensate (BEC) polaron in the continuum and the acoustic polaron in a solid. We present ground-state energies of these two systems calculated with the Diagrammatic Monte Carlo (DiagMC) method and with a Feynman all-coupling approach. The DiagMC method evaluates up to very high order a diagrammatic series for the polaron's self-energy. The Feynman all-coupling approach is a variational method that has been used for a wide range of polaronic problems. For the acoustic and BEC polaron both methods provide remarkably similar non-renormalized ground-state energies that are obtained after introducing a finite momentum cutoff. For the renormalized ground-state energies of the BEC polaron, there are relatively large discrepancies between the DiagMC and the Feynman predictions. These differences can be attributed to the renormalization procedure for the contact interaction.
The description of an impurity atom in a Bose-Einstein condensate can be cast in the form of Fr\"ohlich's polaron Hamiltonian, where the Bogoliubov excitations play the role of the phonons. An expression for the corresponding polaronic coupling strength is derived, relating the coupling strength to the scattering lengths, the trap size and the number of Bose condensed atoms. This allows to identify several approaches to reach the strong-coupling limit for the quantum gas polarons, whereas this limit was hitherto experimentally inaccessible in solids. We apply Feynman's path-integral method to calculate for all coupling strengths the polaronic shift in the free energy and the increase in the effective mass. The effect of temperature on these quantities is included in the description. We find similarities to the acoustic polaron results and indications of a transition between free polarons and self-trapped polarons. The prospects, based on the current theory, of investigating the polaron physics with ultracold gases are discussed for lithium atoms in a sodium condensate.