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arXiv:1905.07368 · Physical Review A

Feynman path-integral treatment of the Bose polaron beyond the Fröhlich model

T. Ichmoukhamedov, Jacques Tempere

Published Oct 9, 2019• 36 citations
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Abstract

An impurity immersed in a Bose-Einstein condensate is no longer accurately described by the Fr\"ohlich Hamiltonian as the coupling between the impurity and the boson bath gets stronger. We study the dominant effects of the two-phonon terms beyond the Fr\"ohlich model on the ground-state properties of the polaron using Feynman's variational path-integral approach. The previously reported discrepancy in the effective mass between the renormalization group approach and this theory is shown to be absent in the beyond-Fr\"ohlich model on the positive side of the Feshbach resonance. Self-trapping, characterized by a sharp and dramatic increase of the effective mass, is no longer observed for the repulsive polaron once the two-phonon interactions are included. For the attractive polaron we find a divergence of the ground-state energy and effective mass at weaker couplings than previously observed within the Fr\"ohlich model.

DOI
10.1103/physreva.100.043605

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An impurity immersed in a Bose-Einstein condensate is no longer accurately described by the Fr"ohlich Hamiltonian as the coupling between the impurity and the boson bath gets stronger. We study the dominant effects of the two-phonon terms beyond the Fr"ohlich model on the ground-state properties of the polaron using Feynman's variational path-integral approach. The previously reported discrepancy in the effective mass between the renormalization group approach and this theory is shown to be absent in the beyond-Fr"ohlich model on the positive side of the Feshbach resonance. Self-trapping, characterized by a sharp and dramatic increase of the effective mass, is no longer observed for the repulsive polaron once the two-phonon interactions are included. For the attractive polaron we find a divergence of the ground-state energy and effective mass at weaker couplings than previously observed within the Fr"ohlich model.
The system of a charged impurity in an interacting Bose gas has gained significant attention due to the long-range ion-atom interactions and the study of transport properties. Here, the ground state energy of a charged Bose polaron is calculated within the Bogoliubov approximation for both the Fröhlich and beyond-Fröhlich Hamiltonians using a generalized Feynman variational path-integral approach, which obtained accurate results for other polaron problems. The generalized approach, which was used to improve the energy result for the neutral polaron, has resulted in a minor improvement, indicating that Feynman's approach is sufficient when the impurity-boson interaction is long-range. Beyond-Fröhlich corrections results in the emergence of a divergence in the polaronic energy indicating a transition between the repulsive and attractive polaron regime. The path-integral approach with the beyond-Fröhlich Hamiltonian is also compared to a field-theory calculation from Christensen et al, 2021. The validity of the Bogoliubov approximation is investigated. The optical absorption has also been calculated within the Bogoliubov approximation for weak ion-atom interactions, and the effect of finite temperature has been studied. We show that the coupling of the ion to an oscillating external electric field offers a straigtforward experimental probe for the charged polaron in a Bose gas, different from but complementary to existing spectroscopic techniques.
The description of an impurity atom in a Bose-Einstein condensate can be cast in the form of Fr\"ohlich's polaron Hamiltonian, where the Bogoliubov excitations play the role of the phonons. An expression for the corresponding polaronic coupling strength is derived, relating the coupling strength to the scattering lengths, the trap size and the number of Bose condensed atoms. This allows to identify several approaches to reach the strong-coupling limit for the quantum gas polarons, whereas this limit was hitherto experimentally inaccessible in solids. We apply Feynman's path-integral method to calculate for all coupling strengths the polaronic shift in the free energy and the increase in the effective mass. The effect of temperature on these quantities is included in the description. We find similarities to the acoustic polaron results and indications of a transition between free polarons and self-trapped polarons. The prospects, based on the current theory, of investigating the polaron physics with ultracold gases are discussed for lithium atoms in a sodium condensate.
We use a nonperturbative renormalization group approach to develop a unified picture of the Bose polaron problem, where a mobile impurity is strongly interacting with a surrounding Bose-Einstein condensate (BEC). A detailed theoretical analysis of the phase diagram is presented and the polaron-to-molecule transition is discussed. For attractive polarons we argue that a description in terms of an effective Fr\"ohlich Hamiltonian with renormalized parameters is possible. Its strong-coupling regime is realized close to a Feshbach resonance, where we predict a sharp increase of the effective mass. Already for weaker interactions, before the polaron mass diverges, we predict a transition to a regime where states exist below the polaron energy and the attractive polaron is no longer the ground state. On the repulsive side of the Feshbach resonance we recover the repulsive polaron, which has a finite lifetime because it can decay into low-lying molecular states. We show for the entire range of couplings that the polaron energy has logarithmic corrections in comparison with predictions by the mean-field approach. We demonstrate that they are a consequence of the polaronic mass renormalization which is due to quantum fluctuations of correlated phonons in the polaron cloud.
Mobile impurity atoms immersed in Bose–Einstein condensates provide a new platform for exploring Bose polarons. Recent experimental advances in the field of ultracold atoms make it possible to realize such systems with highly tunable microscopic parameters and to explore equilibrium and dynamical properties of polarons using a rich toolbox of atomic physics. In this paper we present a detailed theoretical analysis of Bose polarons in one-dimensional systems of ultracold atoms. By combining a non-perturbative renormalization group approach with numerically exact diffusion Monte Carlo calculations we obtain not only detailed numerical results over a broad range of parameters but also qualitative understanding of different regimes of the system. We find that an accurate description of Bose polarons requires the inclusion of two-phonon scattering terms which go beyond the commonly used Fröhlich model. Furthermore we show that when the Bose gas is in the strongly interacting regime, one needs to include interactions between the phonon modes. We use several theoretical approaches to calculate the polaron energy and its effective mass. The former can be measured using radio-frequency spectroscopy and the latter can be studied experimentally using impurity oscillations in a harmonic trapping potential. We compare our theoretical results for the effective mass to the experiments by Catani et al (2012 Phys. Rev. A 85 023623). In the weak-to-intermediate coupling regimes we obtain excellent quantitative agreement between theory and experiment, without any free fitting parameter. We supplement our analysis by full dynamical simulations of polaron oscillations in a shallow trapping potential. We also use our renormalization group approach to analyze the full phase diagram and identify regions that support repulsive and attractive polarons, as well as multi-particle bound states.
Mobile impurity atoms immersed in Bose–Einstein condensates provide a new platform for exploring Bose polarons. Recent experimental advances in the field of ultracold atoms make it possible to realize such systems with highly tunable microscopic parameters and to explore equilibrium and dynamical properties of polarons using a rich toolbox of atomic physics. In this paper we present a detailed theoretical analysis of Bose polarons in one-dimensional systems of ultracold atoms. By combining a non-perturbative renormalization group approach with numerically exact diffusion Monte Carlo calculations we obtain not only detailed numerical results over a broad range of parameters but also qualitative understanding of different regimes of the system. We find that an accurate description of Bose polarons requires the inclusion of two-phonon scattering terms which go beyond the commonly used Fröhlich model. Furthermore we show that when the Bose gas is in the strongly interacting regime, one needs to include interactions between the phonon modes. We use several theoretical approaches to calculate the polaron energy and its effective mass. The former can be measured using radio-frequency spectroscopy and the latter can be studied experimentally using impurity oscillations in a harmonic trapping potential. We compare our theoretical results for the effective mass to the experiments by Catani et al (2012 Phys. Rev. A 85 023623). In the weak-to-intermediate coupling regimes we obtain excellent quantitative agreement between theory and experiment, without any free fitting parameter. We supplement our analysis by full dynamical simulations of polaron oscillations in a shallow trapping potential. We also use our renormalization group approach to analyze the full phase diagram and identify regions that support repulsive and attractive polarons, as well as multi-particle bound states.
F. Grusdt et al. [New J. Phys. 19, 103035 (2017)] recently made a renormalization-group study of a one-dimensional Bose polaron in cold atoms. Their study went beyond the usual Fr\"ohlich description, which includes only single-phonon processes, by including two-phonon processes in which two phonons are simultaneously absorbed or emitted during impurity scattering [Y. E. Shchadilova et al., Phys. Rev. Lett. 117, 113002 (2016)]. We study this same beyond-Fr\"ohlich model, but in the static impurity limit where the ground state is described by a multimode squeezed state instead of the multimode coherent state in the static Fr\"ohlich model. We solve the system exactly by applying the generalized Bogoliubov transformation, an approach that can be straightforwardly adapted to higher dimensions. Using our exact solution, we obtain a polaron energy free of infrared divergences and construct analytically the polaron phase diagram. We find that the repulsive polaron is stable on the positive side of the impurity-boson interaction but is always thermodynamically unstable on the negative side of the impurity-boson interaction, featuring a bound state, whose binding energy we obtain analytically. We find that the attractive polaron is always dynamically unstable, featuring a pair of imaginary energies which we obtain analytically. We expect the multimode squeezed state to help with studies that go not only beyond the Fr\"ohlich paradigm but also beyond Bogoliubov theory, just as the multimode coherent state has helped with the study of Fr\"ohlich polarons.