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arXiv:2111.15647 · PRX Quantum

Dissipative Superradiant Spin Amplifier for Enhanced Quantum Sensing

Martin Koppenhöfer, Peter Groszkowski, Hoi-Kwan Lau, Aashish A. Clerk

Published Aug 30, 2022• 28 citations
arXivHTMLPDF

Abstract

Quantum metrology protocols exploiting ensembles of N two-level systems and Ramsey-style measurements are ubiquitous.However, in many cases excess readout noise severely degrades the measurement sensitivity; in particular in sensors based on ensembles of solid-state defect spins.We present a dissipative "spin-amplification" protocol that allows us to dramatically improve the sensitivity of such schemes, even in the presence of realistic intrinsic dissipation and noise.Our method is based on exploiting collective (i.e., superradiant) spin decay, an effect that is usually seen as a nuisance because it limits spin-squeezing protocols.We show that our approach can allow a system with a highly imperfect spin readout to approach standard-quantum-limit-like scaling in N within a factor of 2, without needing to change the actual readout mechanism.Our ideas are compatible with several state-of-the-art experimental platforms where an ensemble of solid-state spins (NV centers, SiV centers) is coupled to a common microwave or mechanical mode.

DOI
10.1103/prxquantum.3.030330

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Quantum metrology protocols exploiting ensembles of N two-level systems and Ramsey-style measurements are ubiquitous.However, in many cases excess readout noise severely degrades the measurement sensitivity; in particular in sensors based on ensembles of solid-state defect spins.We present a dissipative "spin-amplification" protocol that allows us to dramatically improve the sensitivity of such schemes, even in the presence of realistic intrinsic dissipation and noise.Our method is based on exploiting collective (i.e., superradiant) spin decay, an effect that is usually seen as a nuisance because it limits spin-squeezing protocols.We show that our approach can allow a system with a highly imperfect spin readout to approach standard-quantum-limit-like scaling in N within a factor of 2, without needing to change the actual readout mechanism.Our ideas are compatible with several state-of-the-art experimental platforms where an ensemble of solid-state spins (NV centers, SiV centers) is coupled to a common microwave or mechanical mode.
Quantum metrology protocols using entangled states of large spin ensembles attempt to achieve measurement sensitivities surpassing the standard quantum limit (SQL), but in many cases they are severely limited by even small amounts of technical noise associated with imperfect sensor readout. Amplification strategies based on time-reversed coherent spin-squeezing dynamics have been devised to mitigate this issue, but are unfortunately very sensitive to dissipation, requiring a large single-spin cooperativity to be effective. Here, we propose a new dissipative protocol that combines amplification and squeezed fluctuations. It enables the use of entangled spin states for sensing well beyond the SQL even in the presence of significant readout noise. Further, it has a strong resilience against undesired single-spin dissipation, requiring only a large collective cooperativity to be effective.
Overcoming poor readout is an increasingly urgent challenge for devices based on solid-state spin defects, particularly given their rapid adoption in quantum sensing, quantum information, and tests of fundamental physics. However, in spite of experimental progress in specific systems, solid-state spin sensors still lack a universal, high-fidelity readout technique. Here we demonstrate high-fidelity, room-temperature readout of an ensemble of nitrogen-vacancy centers via strong coupling to a dielectric microwave cavity, building on similar techniques commonly applied in cryogenic circuit cavity quantum electrodynamics. This strong collective interaction allows the spin ensemble's microwave transition to be probed directly, thereby overcoming the optical photon shot noise limitations of conventional fluorescence readout. Applying this technique to magnetometry, we show magnetic sensitivity approaching the Johnson-Nyquist noise limit of the system. Our results pave a clear path to achieve unity readout fidelity of solid-state spin sensors through increased ensemble size, reduced spin-resonance linewidth, or improved cavity quality factor.
We theoretically explore protocols for measuring the spin polarization of an ensemble of solid-state spins, with precision at or below the standard quantum limit. Such measurements in the solid-state are challenging, as standard approaches based on optical fluorescence are often limited by poor readout fidelity. Indirect microwave resonator-mediated measurements provide an attractive alternative, though a full analysis of relevant sources of measurement noise is lacking. In this work we study dispersive readout of an inhomogeneously broadened spin ensemble via coupling to a driven resonator measured via homodyne detection. We derive generic analytic conditions for when the homodyne measurement can be limited by the fundamental spin-projection noise, as opposed to microwave-drive shot noise or resonator phase noise. By studying fluctuations of the measurement record in detail, we also propose an experimental protocol for directly detecting spin squeezing, i.e. a reduction of the spin ensemble's intrinsic projection noise from entanglement. Our protocol provides a method for benchmarking entangled states for quantum-enhanced metrology.
The sensitivity of quantum sensors is fundamentally constrained by the standard quantum limit (SQL) arising from intrinsic quantum fluctuations. While non-classical resources like squeezing or entanglement can surpass this limit, their utility is often restricted by the extreme fragility of entangled states and the complexity of their preparation. Quantum criticality offers a compelling alternative by harnessing divergent susceptibility to amplify signals without requiring fragile non-classical resources. However, the practical benefit of this approach has remained controversial due to the potential for the simultaneous amplification of quantum noise. Here, we demonstrate a universal protocol for noiseless critical sensing by engineering a light-driven atomic ensemble near a dynamical critical point. Analogous to a Kapitza pendulum near its inverted orientation, the spin system enters a non-equilibrium regime where the signal susceptibility diverges while the quantum noise periodically recedes to its coherent baseline. We exploit this ``noise ebbing'' to create a built-in noiseless amplifier, demonstrating a 3.3 dB metrological gain over the SQL in an atomic magnetometer. Our implementation exhibits intrinsic robustness against common experimental imperfections such as detection losses, establishing non-equilibrium critical dynamics as a practical and versatile paradigm for surpassing the fundamental limits of quantum sensing.
Spin squeezing can increase the sensitivity of interferometric measurements of small signals in large spin ensembles beyond the standard quantum limit. In many practical settings, the ideal metrological gain is limited by imperfect readout of the sensor. To overcome this issue, protocols based on time reversal of unitary one-axis-twist (OAT) spin-squeezing dynamics have been proposed. Such protocols mitigate readout noise and, when implemented using cavity feedback, have been argued to also be robust against dissipation as long as the collective cooperativity of the system is sufficiently large [Davis et al., Phys. Rev. Lett. 116, 053601 (2016)]. Here, we perform a careful systematic study of dissipative effects on three different implementations of a OAT twist-untwist sensing scheme (based on symmetric as well as asymmetric cavity feedback and on a Tavis-Cummings interaction). Our full treatment shows that the three approaches have markedly different properties and resilience when subject to dissipation. Moreover, the metrological gain for an implementation using symmetric cavity feedback is more sensitive to undesired dissipation than was previously appreciated.
Solid-state quantum sensors based on ensembles of nitrogen-vacancy (NV) centers in diamond have emerged as powerful platforms for high-precision metrology. Coupling the NV ensemble to a microwave cavity mode in a cavity quantum electrodynamics (cQED) configuration enables spin readout that surpasses the limitations of conventional optical detection, achieving sub-picotesla magnetic sensitivities. However, existing continuous-wave cQED approaches remain far from the intrinsic spin-projection-noise limit due to spin saturation and power broadening. Here, we introduce a dispersive cQED readout technique to overcome these fundamental limitations in NV ensemble sensing. We develop a comprehensive theoretical framework describing the dispersive interaction and analyze the time-domain dynamics of a strongly-coupled NV-cavity system. Our results indicate near-unity inverse readout fidelity and femtotesla-level sensitivity using a commercially available diamond NV ensemble. Importantly, the dispersive readout exhibits a distinct sensitivity scaling that improves as 1/N with increasing number of spins N, providing a practical pathway toward approaching the standard quantum limit for solid-state spin-ensemble sensors.