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arXiv:2003.01104 · Nature Communications

Cavity-enhanced microwave readout of a solid-state spin sensor

Erik R. Eisenach, John F. Barry, Michael F. O’Keeffe, Jennifer M. Schloss, Matthew Steinecker, Dirk Englund, Danielle Braje

Published Mar 1, 2021• 71 citations
arXivHTMLPDF

Abstract

Overcoming poor readout is an increasingly urgent challenge for devices based on solid-state spin defects, particularly given their rapid adoption in quantum sensing, quantum information, and tests of fundamental physics. However, in spite of experimental progress in specific systems, solid-state spin sensors still lack a universal, high-fidelity readout technique. Here we demonstrate high-fidelity, room-temperature readout of an ensemble of nitrogen-vacancy centers via strong coupling to a dielectric microwave cavity, building on similar techniques commonly applied in cryogenic circuit cavity quantum electrodynamics. This strong collective interaction allows the spin ensemble's microwave transition to be probed directly, thereby overcoming the optical photon shot noise limitations of conventional fluorescence readout. Applying this technique to magnetometry, we show magnetic sensitivity approaching the Johnson-Nyquist noise limit of the system. Our results pave a clear path to achieve unity readout fidelity of solid-state spin sensors through increased ensemble size, reduced spin-resonance linewidth, or improved cavity quality factor.

DOI
10.1038/s41467-021-21256-7

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Overcoming poor readout is an increasingly urgent challenge for devices based on solid-state spin defects, particularly given their rapid adoption in quantum sensing, quantum information, and tests of fundamental physics. However, in spite of experimental progress in specific systems, solid-state spin sensors still lack a universal, high-fidelity readout technique. Here we demonstrate high-fidelity, room-temperature readout of an ensemble of nitrogen-vacancy centers via strong coupling to a dielectric microwave cavity, building on similar techniques commonly applied in cryogenic circuit cavity quantum electrodynamics. This strong collective interaction allows the spin ensemble's microwave transition to be probed directly, thereby overcoming the optical photon shot noise limitations of conventional fluorescence readout. Applying this technique to magnetometry, we show magnetic sensitivity approaching the Johnson-Nyquist noise limit of the system. Our results pave a clear path to achieve unity readout fidelity of solid-state spin sensors through increased ensemble size, reduced spin-resonance linewidth, or improved cavity quality factor.
Solid-state quantum sensors based on ensembles of nitrogen-vacancy (NV) centers in diamond have emerged as powerful platforms for high-precision metrology. Coupling the NV ensemble to a microwave cavity mode in a cavity quantum electrodynamics (cQED) configuration enables spin readout that surpasses the limitations of conventional optical detection, achieving sub-picotesla magnetic sensitivities. However, existing continuous-wave cQED approaches remain far from the intrinsic spin-projection-noise limit due to spin saturation and power broadening. Here, we introduce a dispersive cQED readout technique to overcome these fundamental limitations in NV ensemble sensing. We develop a comprehensive theoretical framework describing the dispersive interaction and analyze the time-domain dynamics of a strongly-coupled NV-cavity system. Our results indicate near-unity inverse readout fidelity and femtotesla-level sensitivity using a commercially available diamond NV ensemble. Importantly, the dispersive readout exhibits a distinct sensitivity scaling that improves as 1/N with increasing number of spins N, providing a practical pathway toward approaching the standard quantum limit for solid-state spin-ensemble sensors.
Abstract Quantum sensors based on solid-state defects, in particular nitrogen-vacancy (NV) centers in diamond, enable precise measurement of magnetic fields, temperature, rotation, and electric fields. Cavity quantum electrodynamic (cQED) readout, in which an NV ensemble is hybridized with a microwave mode, can overcome limitations in optical spin detection and has resulted in leading magnetic sensitivities at the pT-level. This approach, however, remains far from the intrinsic spin-projection noise limit due to thermal Johnson-Nyquist noise and spin saturation effects. Here we tackle these challenges by combining recently demonstrated spin refrigeration techniques with comprehensive nonlinear modeling of the cQED sensor operation. We demonstrate that the optically-polarized NV ensemble simultaneously provides magnetic sensitivity and acts as a heat sink for the deleterious thermal microwave noise background, even when actively probed by a microwave field. Optimizing the NV-cQED system, we demonstrate a broadband sensitivity of 576 ± 6 fT/ Hz\sqrt{{{{\rm{Hz}}}}}Hz​ Hz around 15 kHz in ambient conditions. We then discuss the implications of this approach for the design of future magnetometers, including near-projection-limited devices approaching 3 fT/ Hz\sqrt{{{{\rm{Hz}}}}}Hz​ Hz sensitivity enabled by spin refrigeration.
Quantum sensors have the potential to operate at fundamental physical performance limits. Among various quantum sensing platforms, solid-state spin emitters stand out due to advantageous characteristics such as room-temperature spin polarization and readout, atomic-scale spatial resolution, and extended coherence times. Despite these strengths, traditional optical detection methods exhibit low readout fidelity in solid-state ensembles, severely limiting their achievable sensitivity. This thesis addresses this limitation by coupling a solid-state emitter ensemble to a microwave cavity, forming a cavity quantum electrodynamics system. Our approach eliminates the need for photon collection required by conventional optical readout methods, and the resulting strongly coupled system allows efficient cavity-based probing of the solid-state spin ensemble. By exploiting the hybrid quantum system with cavity quantum electrodynamics, we achieve record-high sensitivity for solid-state quantum sensors, representing a substantial advancement toward achieving fundamental sensing limits.
We demonstrate 4π4π4π-steradian vector magnetic field sensing using an ensemble of nitrogen-vacancy (NV) centers in a single-crystal diamond coupled to a microwave (MW) cavity. The MW cavity enhances the spin-photon coupling which enables efficient, high-contrast spin-state readout via MW interrogation and removes the need for bulky optical collection components. An applied AC bias magnetic field lifts the zero-field degeneracy of the four crystallographic NV orientations, allowing each orientation to be individually addressed and used for vector reconstruction of the magnetic field. The resulting magnetometer has a 40\% contrast (20x higher than typical for optical spin-ensemble readout) and achieves a single-axis sensitivity of 250 pT/Hz\sqrt{\mathrm{Hz}}Hz​ which is flat from DC to 1 kHz. Noise models of the composite spin-cavity system establish MW amplitude noise as the dominant noise source and predict a thermal noise limit of 2 pT/Hz\sqrt{\mathrm{Hz}}Hz​.
Nitrogen vacancy centers in diamond have established themselves as good sensing element for various type of sensors. In particular magnetometers based on diamond impurities are quickly developing and are already on the market. Yet, optical readout in these systems complicates system design. Recently schemes of dispersive readout of nitrogen vacancy spin state using high finesse dielectric cavities for microwave field were proposed, which do not use the optical readout scheme. However, only shot noise based estimates were so far done for sensitivity of these devices. Here we provide detailed analysis of various practically relevant noise and loss sources for such a system. Furthermore, we consider the possibility of using the squeezing quantum state of the probing microwave field and show it allows to improve the device performance even at room temperature.
Abstract We demonstrate dispersive readout of the spin of an ensemble of nitrogen-vacancy centers in a high-quality dielectric microwave resonator at room temperature. The spin state is inferred from the reflection phase of a microwave signal probing the resonator. Time-dependent tracking of the spin state is demonstrated, and is employed to measure the T 1 relaxation time of the spin ensemble. Dispersive readout provides a microwave interface to solid state spins, translating a spin signal into a microwave phase shift. We estimate that its sensitivity can outperform optical readout schemes, owing to the high accuracy achievable in a measurement of phase. The scheme is moreover applicable to optically inactive spin defects and it is non-destructive, which renders it insensitive to several systematic errors of optical readout and enables the use of quantum feedback.