Abstract Mean‐field treatment (MFT) is frequently applied to approximately predict the dynamics of quantum optics systems. It simplifies the system Hamiltonian by neglecting the quantum statistics of certain modes that are driven strongly by lasers or couple weakly with other modes. However, the neglected quantum correlations between different modes result in unanticipated quantum effects and might lead to significantly distinct system dynamics. Here, a general and systematic theoretical framework based on perturbation theory in company with MFT is provided to capture these quantum effects. The form of nonlinear dissipation and parasitic Hamiltonian as well as their relationship to the nonlinear coupling rate are predicted. Furthermore, the indicator is also proposed as a measure of the accuracy of mean‐field treatment. As an example, this theory is applied to quantum frequency conversion, in which mean‐field treatment is commonly applied, to test its limitation under strong pump and large coupling strength. The analytical results show excellent agreement with the numerical simulations. This work clearly reveals the residual quantum effects neglected by MFT and provides a more precise theoretical framework for nonlinear optics and quantum optics.
Abstract Mean‐field treatment (MFT) is frequently applied to approximately predict the dynamics of quantum optics systems. It simplifies the system Hamiltonian by neglecting the quantum statistics of certain modes that are driven strongly by lasers or couple weakly with other modes. However, the neglected quantum correlations between different modes result in unanticipated quantum effects and might lead to significantly distinct system dynamics. Here, a general and systematic theoretical framework based on perturbation theory in company with MFT is provided to capture these quantum effects. The form of nonlinear dissipation and parasitic Hamiltonian as well as their relationship to the nonlinear coupling rate are predicted. Furthermore, the indicator is also proposed as a measure of the accuracy of mean‐field treatment. As an example, this theory is applied to quantum frequency conversion, in which mean‐field treatment is commonly applied, to test its limitation under strong pump and large coupling strength. The analytical results show excellent agreement with the numerical simulations. This work clearly reveals the residual quantum effects neglected by MFT and provides a more precise theoretical framework for nonlinear optics and quantum optics.
Abstract Optical solitons classically are stationary solutions of the nonlinear Schrödinger equation. We perform a quantum field theoretic treatment by quantising a linearised fluctuation field around the classical soliton solution which can be seen as providing a background spacetime for the field. The linearised fluctuation modifies the soliton background, which is often neglected, reminiscent of the nondepleted-pump approximation. Going beyond this approximation and by using a number-conserving Bogoliubov approach, we find unstable modes that grow as the soliton propagates. Eventually, these unstable modes induce a considerable (backreaction) effect in the soliton. We calculate the backreaction in the classical field fully analytically in the leading second order. The result is a quadratic local decrease of the soliton photon number in propagation due to the backreaction effect of the unstable mode. Provided the initial pulse is close to the classical soliton solution, the unstable mode contributions always become dominant. We also consider practical scenarios for observing this quantum-induced soliton distortion, in the spectral domain. The backreaction, which we expect to be present in bright and dark, discrete and continuous solitons and other nonlinear pulses plays an important role in future optical analogue gravity experiments, for soliton lasers, and optical communications.
The nonlinear dynamics of dissipative quantum systems in incoherent laser fields is studied in the framework of a master equation with the random telegraph model describing the laser noise and the Markovian approximation dealing with the system-bath couplings. Floquet theory and time-dependent perturbation methods are used to facilitate both analytical and numerical solutions. We develop a theoretical formalism that provides a powerful tool for the detailed analysis of the dissipative quantum dynamics of multilevel systems driven by intense stochastic laser fields. It is found that the system relaxes to a steady state from the effect of the laser phase and frequency noise and the kinetics of this relaxation increases with the addition of dissipative terms, introduced by the coupling to the reservoir. Amplitude fluctuations show a different behavior. Other results concerning the destruction of quantum coherence and the dynamical localization will be established and further relaxation mechanisms such as spontaneous emission and the ionization process will also be considered.
We present a systematic theory of Coulomb-induced correlation effects in the nonlinear optical processes within the strong-coupling regime. In this paper, we shall set a dynamics controlled truncation scheme microscopic treatment of nonlinear parametric processes in semiconductor microcavities including the electromagnetic field quantization. It represents the starting point for the microscopic approach to quantum optics experiments in the strong-coupling regime without any assumption on the quantum statistics of electronic excitations (excitons) involved. We exploit a previous technique, which was used in the semiclassical context, which, once applied to four-wave mixing in quantum wells, allowed us to understand a wide range of observed phenomena. We end up with dynamical equations for exciton and photon operators, which extend the usual semiclassical description of Coulomb interaction effects in terms of a mean-field term plus a genuine noninstantaneous four-particle correlation to quantum optical effects.
Open quantum many body systems describe several quantum simulators, ranging from arrays of superconducting circuits hosting correlated states of light, to ultracold atoms in optical lattices in presence of controlled dissipative processes. Their theoretical understanding is hampered by the exponential scaling of their Hilbert space and by their intrinsic nonequilibrium nature, limiting the applicability of many traditional approaches. In this work we extend Dynamical Mean Field Theory (DMFT), a powerful nonperturbative technique developed for strongly correlated quantum many-body systems, to Markovian open quantum systems. Within Open-DMFT, a master equation describing a lattice of bosonic particles is mapped, at large but finite connectivity, onto an impurity problem describing a single site coupled to Markovian and non-Markovian environments, where the latter accounts for quantum fluctuations beyond Gutzwiller mean-field theory. We introduce a new non-perturbative approach to solve the impurity problem, which dresses the impurity, featuring Markovian dissipative channels, with the non-Markovian bath, in a self-consistent scheme based on a resummation of non-crossing diagrams. Finally, we apply our Open-DMFT to solve a driven-dissipative Bose-Hubbard model, which is relevant to current experiments with dissipative ultracold bosons. We show that this model undergoes a dissipative phase transition towards a superfluid phase, which can be equally interpreted as a quantum many-body synchronization transition of an array of quantum van der Pol oscillators. We show how Open-DMFT captures crucial effects due to finite lattice connectivity, such as hopping-induced dissipation and heating, which are completely missed by mean field theories and which lead to a drastic reduction of the broken symmetry phase that we interpret as a desynchronization driven by quantum fluctuations.
Open quantum systems have drawn attention over decades due to its applicability in the foundation of theoretical physics, e.g. statistical mechanics, quantum mechanics and condensed matter physics. The dynamics of open quantum systems has been described as separate entities from their surrounding environment that consists of a very large number of modes, somehow coupled to the mode of the system. Even though the exact solution of the dynamical behavior of the system is impossible to calculate, we obtain a tentative solution using the crucial Markov approximation. The input-output formalism of the quantum Langevin equation (QLE) has been considered as a useful tool which provides a semi-classical description of the dynamics of the system, whereas the master equation provides a complete picture of the dynamics of the system expressed in terms of density matrix. While studying the dynamics of nonlinear system/environment coupling using QLE, we see, for a small value of external field, that the steady state system field does not change much from the steady state field obtained in the absence of nonlinear dissipation. However, in a case where a stronger external field is applied, we see that the deviation becomes substantial from the solution of linear system. We also see that the nonlinear coupling introduces significant difference in the cavity fluctuation spectrum. The description, therefore, provides a potential explanation of parametric effects in terms of nonlinear dissipation phenomena associated with the nonlinear coupling. Even though the theories developed in the context of open quantum systems have proven to be powerful tools, they do not provide a satisfactory platform to be implemented on non-linear Hamiltonians. We often approximate it by linearizing over nonlinear steady state field amplitude, and therefore, the interesting effects are often overlooked. The limitation of the analytics provokes us to simulate open quantum dynamics numerically. The numerical method consists of transformation of the environmental degrees of freedom to a one-dimensional many-body chain, and the computational technique includes numerical diagonalization and renormalization process. The time-adaptive density matrix renormalisation group (t-DMRG) is known as one of the most powerful techniques for the simulation of strongly-correlated many-body quantum systems. In this thesis, along with the theoretical modeling, we implement DMRG numerical scheme for the simulation of canonical S/B model by mapping it to one-dimensional harmonic chain with nearest neighbor interactions, and use the method to investigate the dynamics of the free dissipative system. The thermalization of open quantum systems is also studied by generating minimally entangled typical thermal states (METTS) through imaginary time evolution, and real-time evolving an empty system in the presence of the thermal bath. Further, we simulate coherently driven free dissipative Kerr nonlinear system numerically using Euler's method by solving Heisenberg equation of motion and t-DMRG algorithm, and demonstrate how the numerical results are analogous to classical bistability. By comparing with analytics, we see that the DMRG numerics is analogous to the quantum-mechanical exact solution obtained by mapping the equation of motion of the density matrix of the system to a Fokker-Plank equation. The comparison between two different numerical techniques shows that the semi-classical Euler's method determines the dynamics of the system field of one among two coherent branches, whereas DMRG numerics gives the superposition of both of them. Hence, DMRG-determined time dynamics undergoes generating non-classical states. Our approach of dealing with nonlinearity represents an important contribution in the developments of technique to study the dynamical and steady-state behavior of open quantum systems, which is a fundamental aspect of quantum physics.
We introduce two approaches to modeling the quantum dynamics of optical χ(3) solitons. Taking an open-system viewpoint, we project the underlying quantum field into system (soliton) and residual reservoir components. The reservoir is treated as either (i) a discrete ``Lanczos supermode'' (LSM) expansion which localizes dynamics to a few-supermode basis, or (ii) a non-local environment which can be traced out by deriving a Markovian master equation (ME). Using these methods, we analyze and identify the quantum structure of both the soliton's stability and its hierarchy of perturbations. Through numerical simulations, we confirm both methods effectively capture quantum-induced soliton phase shifts in a concise few-mode (single-mode for ME) basis, and the LSM approach also captures photon loss which arises from non-Markovian dispersive couplings. As neither method is limited to the linearized regime, our approaches provide powerful computational tools to analyze complex non-Gaussian quantum dynamics of solitons where other commonly-used methods fail, providing insight into such non-perturbative regimes. We also investigate radiation that occurs in the presence of higher-order dispersion with ultrashort pulses, deriving a ME that predicts photon loss consistent with classical theory, but find that both classical and ME theory dramatically underestimate the actual amount of dissipation, which we explain in terms of dispersive coupling-induced soliton broadening.