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arXiv:2111.03857

Ferromagnetism in tilted fermionic Mott insulators

Kazuaki Takasan, Masaki Tezuka

Published Nov 6, 2021• 0 citations
arXivHTMLPDF

Abstract

We investigate the magnetism in tilted fermionic Mott insulators. With a small tilt, the fermions are still localized and form a Mott-insulating state, where the localized spins interact via antiferromagnetic exchange coupling. While the localized state is naively expected to be broken with a large tilt, in fact, the fermions are still localized under a large tilt due to the Wannier-Stark localization and it can be regarded as a localized spin system. We find that the sign of the exchange coupling is changed and the ferromagnetic interaction is realized under the large tilt. To show this, we employ perturbation theory and real-time numerical simulation of the fermionic Hubbard chain. Our simulation exhibits that it is possible to effectively control the speed and time direction of the dynamics by changing the size of the tilt, which may be useful for experimentally measuring out-of-time-ordered correlators. Finally, we discuss experimental platforms, such as ultracold atoms in an optical lattice, to observe these phenomena.

DOI
10.48550/arxiv.2111.03857

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We investigate the magnetism in tilted fermionic Mott insulators. With a small tilt, the fermions are still localized and form a Mott-insulating state, where the localized spins interact via antiferromagnetic exchange coupling. While the localized state is naively expected to be broken with a large tilt, in fact, the fermions are still localized under a large tilt due to the Wannier-Stark localization and it can be regarded as a localized spin system. We find that the sign of the exchange coupling is changed and the ferromagnetic interaction is realized under the large tilt. To show this, we employ perturbation theory and real-time numerical simulation of the fermionic Hubbard chain. Our simulation exhibits that it is possible to effectively control the speed and time direction of the dynamics by changing the size of the tilt, which may be useful for experimentally measuring out-of-time-ordered correlators. Finally, we discuss experimental platforms, such as ultracold atoms in an optical lattice, to observe these phenomena.
Quantum-mechanical correlations of interacting fermions result in the emergence of exotic phases.Magnetic phases naturally arise in the Mott-insulator regime of the Fermi-Hubbard model, where charges are localized and the spin degree of freedom remains.In this regime, the occurrence of phenomena such as resonating valence bonds, frustrated magnetism, and spin liquids is predicted.Quantum systems with engineered Hamiltonians can be used as simulators of such spin physics to provide insights beyond the capabilities of analytical methods and classical computers.To be useful, methods for the preparation of intricate many-body spin states and access to relevant observables are required.Here, we show the quantum simulation of magnetism in the Mott-insulator regime with a linear quantum-dot array.We characterize the energy spectrum for a Heisenberg spin chain, from which we can identify when the conditions for homogeneous exchange couplings are met.Next, we study the multispin coherence with global exchange oscillations in both the singlet and triplet subspace of the Heisenberg Hamiltonian.Last, we adiabatically prepare the low-energy global singlet of the homogeneous spin chain and probe it with two-spin singlettriplet measurements on each nearest-neighbor pair and the correlations therein.The methods and control presented here open new opportunities for the simulation of quantum magnetism benefiting from the flexibility in tuning and layout of gate-defined quantum-dot arrays.
Abstract A large repulsion between particles in a quantum system can lead to their localization, an effect responsible for the Mott insulator phases in strongly correlated materials. In a system with multiple orbitals, an orbital-selective Mott insulator can form, where electrons in some orbitals are predicted to localize while others remain itinerant. Here we demonstrate a more general version of this phenomenon by observing flavour-selective localization in an atom-based quantum simulator. Our experiment realizes Fermi–Hubbard models with an SU(3) symmetry that can be broken using a tunable coupling between flavours. We observe an enhancement of the localization associated with a selective Mott transition and the emergence of flavour-dependent correlations. Our realization of flavour-selective Mott physics demonstrates the potential of cold atoms to simulate interacting multicomponent materials such as superconductors and topological insulators.
We theoretically investigate, using non-perturbative strong correlation techniques, Mott insulating phases and magnetic ordering of two-component fermions in a two-dimensional double-well optical lattice. At filling of two fermions per site, there are two types of Mott insulators, one of which is characterized by spin-1 antiferromagnetism below the Neel temperature. The super-exchange interaction in this system is induced by the interplay between the inter-band interaction and the spin degree of freedom. A great advantage of the double-well optical lattice is that the magnetic quantum phase diagram and the Neel temperature can be easily controlled by tuning the orbital energy splitting of the two-level system. Particularly, the Neel temperature can be one order of magnitude larger than that in standard optical lattices, facilitating the experimental search for magnetic ordering in optical lattice systems.
Motivated by recent progress in the realization of artificial gauge fields and SU(NNN) Mott insulators using alkaline-earth-like atoms in optical lattices, we develop an unbiased SU(NNN) real-space dynamical mean-field theory approach to study the effect of spin-orbit coupling and on-site Hubbard interaction UUU on SU(3) fermionic systems. We investigate the behavior of the local magnetization, double occupancies, and the triple occupancy versus the Hubbard interaction across the metal to Mott insulator transition. We map out the magnetic phase diagram in the large-UUU limit and show that the spin-orbit coupling can stabilize long-range orders such as ferromagnets, spirals, and stripes with different orientations in SU(3) Mott insulators.
This thesis reports original research on strongly interacting fermions described by Hubbard-like models which can be realized with ultracold atom experiments. In particular, two main directions have been pursued: (i) the control of magnetic and topological properties in a honeycomb lattice through a suitable tuning of the trapping potential, and (ii) the possibility to observe orbital-selective Mott physics in a multicomponent Fermi system where the SU(N) symmetry is broken in a controlled way. The first line of research is based on the idea that increasing the strength of a trapping potential, one can trap a strongly interacting fermions in a limited portion of space, thereby changing their average density and the related magnetic properties. In particular it was demonstrated that this confinement protocol can be used to designeffective “nanoflakes” which are reminiscent of a solid-state proposal [1]. The second step was to extend the same philosophy to the so-called Kane-Mele model, a spinful version of the paradigmatic model proposed by Haldane which presents quantum Hall states. This model can be realized with cold-atom systems using artificial gauge fields. In this thesis we consider a Kane-Mele-Hubbard model where the electronic structure of the Kane-Mele model is supplemented by the onsite Hubbard interaction, allowing us to study the interplay between the correlations and magnetism induced by the repulsion, with the non-trivial topological properties. Also for this model, we follow the strategy discussed above, namely the possibility to engineer an effective “nanoflake” by tuning the lattice potential. The final outcome in this case is even reacher, because it leads, among other results, to a situation where the effective flake hosts an inhomogeneous state which presents at the same time topologically non-trivial properties and magnetism, realizing a spin-Chern insulator [2]. Besides the remarkable application for topological matter, artificial gauge fields, which rely on the coupling of spin states, offer also great insides into mutli-orbital physics. In the second main research line reported in the thesis we study in collaboration with the experimental group of Leonardo Fallani, the controlled symmetry breaking on a 173Yb many-body system, where coupling between spin states is exploited to simulate the mechanism relevant for the physics of multi-orbital materials, such as iron-based superconductors. In order to reveal this mechanism in cold atoms we focus on interacting SU(3) lattice fermions where the SU(3) spin symmetry is explicitly broken by a Raman coupling between the spin states. Combining experiments and theory, we demonstrate that this setup reveals orbital-selective physics and it shows that the SU(3)-symmetry-breaking Raman coupling favours Mott localization and selective properties [3]. Our results show a clear evidence of orbital-selective correlations, which reflect in contrasting transport properties in different orbitals, the extreme case being an orbital-selective Mott state where only some of the orbitals are Mott localized while others remain metallic. Moreover, the coupling between spin states favors Mott localization with respect to the symmetric case, hence it reduces the critical interaction needed for a full Mott localization.
We experimentally study the emergence of antiferromagnetic correlations between ultracold fermionic atoms in a two-dimensional optical lattice with decreasing temperature. We determine the uniform magnetic susceptibility of the two-dimensional Hubbard model from simultaneous measurements of the in situ density distribution of both spin components. At half filling and strong interactions our data approach the Heisenberg model of localized spins with antiferromagnetic correlations. Moreover, we observe a fast decay of magnetic correlations when doping the system away from half filling.