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arXiv:2110.00354 · Physical Review Letters

Preparation of the Spin-Mott State: A Spinful Mott Insulator of Repulsively Bound Pairs

Julius de Hond, Jinggang Xiang, Woo Chang Chung, Enid Cruz-Colón, Wenlan Chen, William Cody Burton, Colin J. Kennedy, Wolfgang Ketterle

Published Feb 28, 2022• 22 citations
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Abstract

We observe and study a special ground state of bosons with two spin states in an optical lattice: the spin-Mott insulator, a state that consists of repulsively bound pairs that is insulating for both spin and charge transport. Because of the pairing gap created by the interaction anisotropy, it can be prepared with low entropy and can serve as a starting point for adiabatic state preparation. We find that the stability of the spin-Mott state depends on the pairing energy, and observe two qualitatively different decay regimes, one of which exhibits protection by the gap.

DOI
10.1103/physrevlett.128.093401

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We observe and study a special ground state of bosons with two spin states in an optical lattice: the spin-Mott insulator, a state that consists of repulsively bound pairs that is insulating for both spin and charge transport. Because of the pairing gap created by the interaction anisotropy, it can be prepared with low entropy and can serve as a starting point for adiabatic state preparation. We find that the stability of the spin-Mott state depends on the pairing energy, and observe two qualitatively different decay regimes, one of which exhibits protection by the gap.
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We prepare and study a metastable attractive Mott-insulator state formed with bosonic atoms in a three-dimensional optical lattice. Starting from a Mott insulator with Cs atoms at weak repulsive interactions, we use a magnetic Feshbach resonance to tune the interactions to large attractive values and produce a metastable state pinned by attractive interactions with a lifetime on the order of 10 s. We probe the (de)excitation spectrum via lattice modulation spectroscopy, measuring the interaction dependence of two- and three-body bound-state energies. As a result of increased on-site three-body loss we observe resonance broadening and suppression of tunneling processes that produce three-body occupation.
The superfluid--Mott-insulator transition of spin-2 boson atoms with repulsive interaction in an optical lattice in a magnetic field is presented. By using the mean-field theory, the Mott ground states and phase diagrams of the superfluid--Mott-insulator transition at zero temperature are revealed. An applied magnetic field leads to splitting of some phase boundaries. For all the initial Mott ground states containing multiple spin components, different spin components take on different phase boundaries. It is found that in this system phase boundaries with different magnetization can be moved in different ways by changing only the intensity of the applied magnetic field.
We analyze the behavior of cold spin-1 particles with antiferromagnetic interactions in a one-dimensional optical lattice using density matrix renormalization group calculations. Correlation functions and the dimerization are shown and we also present results for the energy gap between ground state and the spin excited states. We confirm the anticipated phase diagram, with Mott-insulating regions of alternating dimerized S=1S=1S=1 chains for odd particle density versus on-site singlets for even density. We find no evidence for any additional ordered phases in the physically accessible region, however for sufficiently large spin interaction, on-site singlet pairs dominate leading, for odd density, to a breakdown of the Mott insulator or, for even density, a real-space singlet superfluid.
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We suggest and analyze a scheme to adiabatically cool bosonic atoms to picokelvin temperatures which should allow the observation of magnetic ordering via superexchange in optical lattices. The starting point is a gapped phase called the spin Mott phase, where each site is occupied by one spin-up and one spin-down atom. An adiabatic ramp leads to an xyxyxy-ferromagnetic phase. We show that the combination of time-dependent density matrix renormalization group methods with quantum trajectories can be used to fully address possible experimental limitations due to decoherence, and demonstrate that the magnetic correlations are robust for experimentally realizable ramp speeds. Using a microscopic master equation treatment of light scattering in the many-particle system, we test the robustness of adiabatic state preparation against decoherence. Due to different ground-state symmetries, we also find a metastable state with xyxyxy-ferromagnetic order if the ramp crosses to regimes where the ground state is a zzz ferromagnet. The bosonic spin Mott phase as the initial gapped state for adiabatic cooling has many features in common with a fermionic band insulator, but the use of bosons should enable experiments with substantially lower initial entropies.