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arXiv:2109.01495 · Physical Review Research

Excited-state quantum phase transitions in spin-orbit-coupled Bose gases

Josep Cabedo, Alessio Celi

Published Dec 27, 2021• 23 citations
arXivHTMLPDF

Abstract

Excited-state quantum phase transitions depend on and reveal the structure of the whole spectrum of many-body systems. While they are theoretically well understood, finding suitable signatures and detecting them in actual experiments remains challenging. For instance, in spinor gases, excited-state phases have been identified and characterized through a topological order parameter that is challenging to measure in experiments. Here we propose the Raman-dressed spin-orbit-coupled gas as a novel platform to explore excited-state quantum phase transitions. In a weakly coupled regime, the dressed system is equivalent to a spinor gas with tunable spin-spin interactions. Through this equivalence we are able to identify excited-state phases in the Raman-dressed Bose gas. The phases are characterized by the behavior of the spatial density modulations, or stripes, induced by spin-orbit coupling, and can in principle be measured in current state-of-the-art experiments with ultracold atoms. Conversely, we show that the properties of the excited phase can be exploited to prepare stripe states with large and stable density modulations.

DOI
10.1103/physrevresearch.3.043215

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•Jan 1, 2018•0 citations
Excited-state quantum phase transitions depend on and reveal the structure of the whole spectrum of many-body systems. While they are theoretically well understood, finding suitable signatures and detecting them in actual experiments remains challenging. For instance, in spinor gases, excited-state phases have been identified and characterized through a topological order parameter that is challenging to measure in experiments. Here we propose the Raman-dressed spin-orbit-coupled gas as a novel platform to explore excited-state quantum phase transitions. In a weakly coupled regime, the dressed system is equivalent to a spinor gas with tunable spin-spin interactions. Through this equivalence we are able to identify excited-state phases in the Raman-dressed Bose gas. The phases are characterized by the behavior of the spatial density modulations, or stripes, induced by spin-orbit coupling, and can in principle be measured in current state-of-the-art experiments with ultracold atoms. Conversely, we show that the properties of the excited phase can be exploited to prepare stripe states with large and stable density modulations.
In spinor Bose-Einstein condensates, spin-changing collisions are a remarkable proxy to coherently realize macroscopic many-body quantum states. These processes have been, e.g., exploited to generate entanglement, to study dynamical quantum phase transitions, and proposed for realizing nematic phases in atomic condensates. In the same systems dressed by Raman beams, the coupling between spin and momentum induces a spin dependence in the scattering processes taking place in the gas. Here we show that, at weak couplings, such modulation of the collisions leads to an effective Hamiltonian which is equivalent to the one of an artificial spinor gas with spin-changing collisions that are tunable with the Raman intensity. By exploiting this dressed-basis description, we propose a robust protocol to coherently drive the spin-orbit-coupled condensate into the ferromagnetic stripe phase via crossing a quantum phase transition of the effective low-energy model in an excited state.
The recently realized spin-orbit-coupled quantum gases [Lin et al., Nature (London) 471, 83 (2011); Wang et al., Phys. Rev. Lett. 109, 095301 (2012); Cheuk et al., Phys. Rev. Lett. 109, 095302 (2012)] mark a breakthrough in the cold atom community. In these experiments, two hyperfine states are selected from a hyperfine manifold to mimic a pseudospin-1/2 spin-orbit-coupled system by the method of Raman dressing, which is applicable to both bosonic and fermionic gases. In this paper, we show that the method used in these experiments can be generalized to create any large pseudospin spin-orbit-coupled gas if more hyperfine states are coupled equally by the Raman lasers. As an example, we study, in detail, a quantum gas with three hyperfine states coupled by the Raman lasers and show, when the state-dependent energy shifts of the three states are comparable, triple-degenerate minima will appear at the bottom of the band dispersions, thus, realizing a spin-1 spin-orbit-coupled quantum gas. A novel feature of this three-minima regime is that there can be two different kinds of stripe phases with different wavelengths, which has an interesting connection to the ferromagnetic and polar phases of spin-1 spinor Bose-Einstein condensates without spin-orbit coupling.
We propose and analyze a quantum interferometry scheme based on a Raman-dressed Bose gas with spin-orbit coupling. In this system, the atom-light coupling mixes spin and momentum degrees of freedom, giving rise, in the low-energy regime, to an effective spinor condensate whose spin-mixing interaction can be tuned independently of the atomic density. This controllability enables a separation between state preparation and phase imprinting, and provides a natural route to echo-type protocols based on effective time reversal. Within this framework, critical regimes of the effective spinor Hamiltonian can be used to generate entanglement and enhance interferometric sensitivity beyond the standard quantum limit. In addition, the spin-momentum locking of the dressed modes gives access to spatial density modulations that provide an alternative readout of the interferometric phase. In particular, phase information can be extracted from the displacement of spin-orbit-induced density stripes even when conventional spin observables are insensitive within the effective spinor description. Our results identify Raman-dressed spinor gases as a flexible platform for nonlinear atomic interferometry, combining controllable spin-mixing dynamics with spatially resolved phase readout.
We study the ground-state phase diagram and the quantum phase transitions in spin-1 Bose gases with Raman-induced spin-orbit coupling. In addition to the Bose-Einstein condensates with uniform density, three types of stripe condensation phases that simultaneously break the U(1) symmetry and the translation symmetry are identified. The transitions between these phases are investigated, and the occurrences of the various tricritical points are predicted. The excitation spectra in the plane-wave phase and the zero-momentum phase show rich roton-maxon structures, and their instabilities indicate the tendency to develop the crystalline order. We propose the atomic gas of 23Na^{23}\mathrm{Na}23Na could be a candidate for observing the stripe condensate with high contrast fringes.
Excited-state quantum phase transitions extend the notion of quantum phase transitions beyond the ground state. They are characterized by closing energy gaps amid the spectrum. Identifying order parameters for excited-state quantum phase transitions poses, however, a major challenge. We introduce a topological order parameter that distinguishes excited-state phases in a large class of mean-field models and can be accessed by interferometry in current experiments with spinor Bose-Einstein condensates. Our work opens a way for the experimental characterization of excited-state quantum phases in atomic many-body systems.
Quantum degenerate gases have provided rich systems to simulate engineered Hamiltonians and to explore quantum many-body problems in laboratory-scale experiments. In this work, I focus on spin-orbit-coupled (SOC) Bose-Einstein condensates (BECs) of Rubidium-87 atoms realized using two-photon Raman coupling in which various novel phases are predicted to exist due to competing energies from the atomic internal structure, coupling strength, and many-body collisions. BECs are observed primarily using the interaction between light and matter, where it is common to probe the atoms with near-resonant light and image their shadow on a camera. This absorption imaging technique measures the integrated column density of the atoms and it is crucial to focus the imaging system. I present a systematic method to bring the ultracold atom systems into an optimal focus using the power spectral density (PSD) of the atomic density-density correlation function. The spatial frequency at which the defocus-induced artifacts first appear in the PSD is maximized at the focus. The focusing process thus identifies the range of spatial frequencies over which the PSD is uncontaminated by finite-thickness effects. Next, I describe magnetic phases which exist in spin-1 spin-orbit-coupled condensates at a near-zero temperature. I observe ferromagnetic and unmagnetized phases which are stabilized by the locking between the spin and linear momentum of the system. Our measurements of both the first- and second-order transitions are in agreement with theory. Finally, I discuss the stripe-ordered phase that occurs in SOC Bose gases favoring the miscibility configuration. The stripe phase is theoretically predicted to have an excitation spectrum analogous to that of a supersolid and to exhibit spatial density modulation within specific regions of parameter space. I used optical Bragg scattering to probe the small density modulation present in the atomic spatial distribution. I present for the very first time observation of the stripe phase in a Raman SOC Bose gas and its phase diagram in various parameter space. Our observations of the phase boundaries are consistent with theory and previous work.