Excited-state quantum phase transitions extend the notion of quantum phase transitions beyond the ground state. They are characterized by closing energy gaps amid the spectrum. Identifying order parameters for excited-state quantum phase transitions poses, however, a major challenge. We introduce a topological order parameter that distinguishes excited-state phases in a large class of mean-field models and can be accessed by interferometry in current experiments with spinor Bose-Einstein condensates. Our work opens a way for the experimental characterization of excited-state quantum phases in atomic many-body systems.
Excited-state quantum phase transitions extend the notion of quantum phase transitions beyond the ground state. They are characterized by closing energy gaps amid the spectrum. Identifying order parameters for excited-state quantum phase transitions poses, however, a major challenge. We introduce a topological order parameter that distinguishes excited-state phases in a large class of mean-field models and can be accessed by interferometry in current experiments with spinor Bose-Einstein condensates. Our work opens a way for the experimental characterization of excited-state quantum phases in atomic many-body systems.
Entanglement lies at the core of emergent quantum technologies such as quantum-enhanced metrology, quantum communication and cryptography, and quantum simulation and computing. Spinor Bose-Einstein condensates (BECs) offer a promising platform for the generation and application of entangled states. For example, a spin-1 BEC has served for the proof-of-principle demonstration of a quantum-enhanced atomic clock. Ferromagnetic spin-1 BECs with zero magnetization exhibit three ground-state quantum phases with different entanglement properties. The control parameter can be tuned by a magnetic field or by microwave dressing. As already experimentally demonstrated, an entangled ground state can be reached from a well accessible, non-entangled one by driving the control parameter across quantum phase transitions (QPTs). We investigate which of the entangled ground states afford quantum-enhanced interferometry. The interferometric usefulness is quantified by the quantum Fisher information (QFI), which we analyze throughout all ground-state phases. A large QFI at about half the Heisenberg limit, and thus far above the standard quantum limit, is attained by the well-known Twin-Fock state and by the central broken-axisymmetry (CBA) state. We detail how the CBA state can be used as a probe for quantum-enhanced interferometry. Furthermore, we observe that the large QFI of the CBA state can be traced back to enclosed macroscopic superposition states (MSSs). Measuring the atom number in one out of three modes generates, with high probability and heralded by the measurement outcome, a MSS similar to a NOON state. Our proposal promises NOON-like MSSs of unprecedentedly many atoms. Both proposed applications of the adiabatically prepared CBA state depend only on existent technology. Our numerical results show that they tolerate a reasonably swift quasiadiabatic passage in the presence of atom loss as well as uncertainties of atom counting. Excited-state quantum phase transitions (ESQPTs) extend the concept of QPTs beyond the ground state. While they have been extensively investigated theoretically, there are only few experimental results. From the perspective of quantum-state engineering, it is furthermore surprising how rarely order parameters of ESQPTs are discussed in the literature. Mean-field models for spinor BECs imply ESQPTs, to which some experimental observations on the mean-field dynamics can be attributed. However, so far, neither theoretical nor experimental studies have specifically addressed ESQPTs in spinor BECs. We extend the ground-state phase diagram of ferromagnetic spin-1 BECs with zero magnetization across the spectrum. There are three excited-state phases, corresponding to one ground-state phase each. The ESQPTs are signaled by a diverging density of states. The mean-field phase-space trajectories can be characterized by a winding number that is in one-to-one correspondence to the excited-state phases. We derive a closely related order parameter encoded in the dynamics of coherent states and discuss how this order parameter can be interferometrically measured in current experiments. Remarkably, the mean-field model governing the ESQPTs in spin-1 BECs with zero magnetization is encountered also, e. g., in molecular and nuclear physics. Because of the superior experimental control, spinor BECs can be considered as simulators of the ESQPTs in those systems. Our results contribute to quantum-state engineering and quantum-enhanced interferometry in spinor BECs and to the characterization of excited-state quantum phases. The latter may, in turn, lead on to applications in quantum-state engineering.
Excited-state quantum phase transitions depend on and reveal the structure of the whole spectrum of many-body systems. While they are theoretically well understood, finding suitable signatures and detecting them in actual experiments remains challenging. For instance, in spinor gases, excited-state phases have been identified and characterized through a topological order parameter that is challenging to measure in experiments. Here we propose the Raman-dressed spin-orbit-coupled gas as a novel platform to explore excited-state quantum phase transitions. In a weakly coupled regime, the dressed system is equivalent to a spinor gas with tunable spin-spin interactions. Through this equivalence we are able to identify excited-state phases in the Raman-dressed Bose gas. The phases are characterized by the behavior of the spatial density modulations, or stripes, induced by spin-orbit coupling, and can in principle be measured in current state-of-the-art experiments with ultracold atoms. Conversely, we show that the properties of the excited phase can be exploited to prepare stripe states with large and stable density modulations.
Quantum phase transitions universally exist in the ground and excited states of quantum many-body systems, and they have a close relationship with the nonequilibrium dynamical phase transitions, which however are challenging to identify. In the system of spin-1 Bose-Einstein condensates, though dynamical phase transitions with correspondence to equilibrium phase transitions in the ground state and uppermost excited state have been probed, those taking place in intermediate excited states remain untouched in experiments thus far. Here we unravel that both the ground- and excited-state quantum phase transitions in spinor condensates can be diagnosed with dynamical phase transitions. A connection between equilibrium phase transitions and nonequilibrium behaviors of the system is disclosed in terms of the quantum Fisher information. We also demonstrate that near the critical points parameter estimation beyond the standard quantum limit can be implemented. This work not only advances the exploration of excited-state quantum phase transitions via a scheme that can immediately be applied to a broad class of few-mode quantum systems, but also provides a new perspective on the relationship between quantum criticality and quantum enhanced sensing.
Out-of-Time-Order Correlator (OTOC) provides a way of quantifying information scrambling in quantum many-body systems and receives increasing attention from different fields. We extend the application of the OTOC to probe the excited-state quantum phase transitions (ESQPT) in spinor Bose–Einstein condensate in an external magnetic field. Using the quantum approach, mean-field theory, and numerical simulations, we have obtained the phase transition points and dynamical properties around them, and have demonstrated that these features can be detected by the OTOC. Our further investigations reveal that the detection efficiency is guaranteed under different magnetization conditions. Our results provide theoretical suggestions for using the OTOCs for experimentally accessing ESQPT in spinor quantum gases and other quantum many-body systems.
Identifying dynamical signatures of excited-state quantum phase transitions (ESQPTs) in experimentally realizable quantum many-body systems is helpful for understanding the dynamical effects of ESQPTs. In such systems, the highly controllable spinor Bose-Einstein condensates (BECs) offer an exceptional platform to study ESQPTs. In this work, we investigate the dynamical characteristics of the ESQPT in spin-1 BEC by means of the Loschmidt echo spectrum. The Loschmidt echo spectrum is an extension of the well-known Loschmidt echo and defined as the overlaps between the evolved state and the excited states of the initial Hamiltonian. We show that both the time-evolved and long-time-averaged Loschmidt echo spectrum undergo a remarkable change as the system passes through the critical point of the ESQPT. Moreover, the particular behavior exhibited by the Loschmidt echo spectrum at the critical point stands as a dynamical detector for probing the ESQPT. We further demonstrate how to capture the features of the ESQPT by using the energy distribution associated with the Loschmidt echo spectrum for time-evolved and long-time-averaged cases, respectively. Our findings contribute to a further verification of the usefulness of the Loschmidt echo spectrum for witnessing various quantum phase transitions in many-body systems and provide a different way to experimentally examine the dynamical consequences of ESQPTs.
We introduce a general scheme for constructing order parameters (OPs) by extracting generic patterns from the dominant Fock states of many-body ground states. While topological phases are traditionally characterized by non-local invariants, we demonstrate that our real-space OPs provide a more refined classification. In the extended Su-Schrieffer-Heeger model, we show that the standard winding number is insufficient to fully distinguish all phases; our OPs reveal a hidden sub-structure where each topological sector splits into two distinct phases. Beyond identifying the phase boundaries, these OPs quantify the depth of a phase, and remain robust in characterizing transitions in disordered systems. Furthermore, our approach provides a practical finite-size diagnostic for the Berezinskii-Kosterlitz-Thouless transition in the interacting spin-1/2 XXZ model. The presented framework offers a broadly applicable tool for uncovering the phase diagrams of diverse interacting and non-interacting quantum many-body systems.