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arXiv:2108.01153 · SciPost Physics Core

Trapping effects in quantum atomic arrays

Pengfei Zhang

Published Mar 7, 2022• 1 citation
arXivHTMLPDF

Abstract

Quantum emitters, particularly atomic arrays with subwavelength lattice constant, have been proposed to be an ideal platform for studying the interplay between photons and electric dipoles. In this work, motivated by the recent experiment [1], we develop a microscopic quantum treatment using annihilation and creation operator of atoms in deep optical lattices. Using a diagrammatic approach on the Keldysh contour, we derive the cooperative scattering of the light and obtain the general formula for the S matrix. We apply our method to study the trapping effect, which is beyond previous treatment with spin operators. If the optical lattices are formed by light fields with magical wavelength, the result matches previous results using spin operators. When there is a mismatch between the trapping potentials for atoms in the ground state and the excited state, atomic mirrors become imperfect, with multiple resonances in the optical response. We further study the effect of recoil for large but finite trapping frequency. Our results are consistent with existing experiments.

DOI
10.21468/scipostphyscore.5.1.010

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Quantum emitters, particularly atomic arrays with subwavelength lattice constant, have been proposed to be an ideal platform for studying the interplay between photons and electric dipoles. In this work, motivated by the recent experiment [1], we develop a microscopic quantum treatment using annihilation and creation operator of atoms in deep optical lattices. Using a diagrammatic approach on the Keldysh contour, we derive the cooperative scattering of the light and obtain the general formula for the S matrix. We apply our method to study the trapping effect, which is beyond previous treatment with spin operators. If the optical lattices are formed by light fields with magical wavelength, the result matches previous results using spin operators. When there is a mismatch between the trapping potentials for atoms in the ground state and the excited state, atomic mirrors become imperfect, with multiple resonances in the optical response. We further study the effect of recoil for large but finite trapping frequency. Our results are consistent with existing experiments.
Quantum emitters, in particular, atomic arrays with subwavelength lattice constant, have been proposed to be an ideal platform for study the interplay between photons and electric dipoles. Previous theoretical studies are based on spin models, where each site is occupied by a point-like atom. In this work, motivated by the recent experiment [1], we develop a full quantum treatment using annihilation and creation operator of atoms in deep optical lattices. We use a diagrammatic approach on the Keldysh contour to derive the cooperative scattering of the light and obtain the general formula for the S matrix. We apply our formulism to study two effects beyond previous treatment with spin-operators, the effect of fractional filling and trapping. Both effects can lead to imperfectness of atomic mirrors. For the fractional filling case, we find the cooperative linewidth is linear in filling fraction n. When there is a mismatch between the trapping potentials for atoms in the ground state and the excited state, multiple resonances can appear in the response function. Our results are consistent with existing experiments.
Subwavelength arrays of atoms trapped in optical lattices or tweezers are inherently susceptible to deformations: Optomechanical forces displace atoms within their trapping potential and produce lattice distortions, which in turn modify the optical response of the array. We show that this optomechanical coupling hybridizes collective atomic excitations (polaritons) with phonons, forming polaron-polaritons -- the fundamental quasiparticles governing light-matter interactions in arrays of trapped atoms. Using analytical polaron theory and numerical simulations, we find that: (1) phonons can strongly enhance the decay of subradiant states, but also enable their efficient excitation; (2) transport of dark excitations remains remarkably robust even at low trap frequencies, except when a polariton can resonantly scatter phonons; and (3) motion reduces the reflectivity of a two-dimensional atomic mirror; by identifying design principles that mitigate this degradation, we recover reflectivity above 99% under realistic conditions. Our findings lay the foundation for analyzing motional effects in key applications and suggest new ways to harness them in state-of-the-art experiments.
We consider light scattering off a two-dimensional (2D) dipolar array and show how it can be tailored by properly choosing the lattice constant of the order of the incident wavelength. In particular, we demonstrate that such arrays can operate as a nearly perfect mirror for a wide range of incident angles and frequencies, and shape the emission pattern from an individual quantum emitter into a well-defined, collimated beam. These results can be understood in terms of the cooperative resonances of the surface modes supported by the 2D array. Experimental realizations are discussed, using ultracold arrays of trapped atoms and excitons in 2D semiconductor materials, as well as potential applications ranging from atomically thin metasurfaces to single photon nonlinear optics and nanomechanics.
The coupling of atomic arrays and one-dimensional subwavelength waveguides gives rise to interesting photon transport properties, such as recent experimental demonstrations of large Bragg reflection, and paves the way for a variety of potential applications in the field of quantum nonlinear optics. Here, we present a theoretical analysis for the process of single-photon scattering in this configuration using a full microscopic approach. Based on this formalism, we analyze the spectral dependencies for different scattering channels from either ordered or disordered arrays. The developed approach is entirely applicable for a single-photon scattering from a quasi-one-dimensional array of multilevel atoms with degenerate ground-state energy structure. Our approach provides an important framework for including not only Rayleigh but also Raman channels in the microscopic description of the cooperative scattering process.
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Quantum cooperativity is evident in light-matter platforms where quantum emitter ensembles are interfaced with confined optical modes and are coupled via the ubiquitous electromagnetic quantum vacuum. Cooperative aspects such as dipole-dipole interactions and subradiance find applications in the design of nanoscale coherent light sources and highly-reflective quantum metasurfaces made up of hundreds of optically trapped atoms, in the implementation of topological quantum optics on subwavelength arrays of emitters, in quantum metrology and quantum information. The quick bursts of radiation from a collection of quasi-indistiguishable emitters provides an alternative approach to standard lasers by introducing superradiant lasers operating at extremely low intracavity power. This tutorial provides a set of theoretical tools to tackle the behavior responsible for the onset of cooperativity in light-matter systems by extending open quantum system dynamics methods, such as the master equation and quantum Langevin equations, to electron-photon interactions in strongly coupled and correlated quantum emitters ensembles. These analytical approaches are then also extended to frequency disordered or vibronically coupled quantum emitter ensembles with wide relevance ranging from atoms in optical lattices, quantum dots in solid state environments or molecular quantum systems.