Subwavelength arrays of quantum emitters offer an efficient free-space approach to coherent light-matter interfacing, using ultracold atoms or two-dimensional solid-state quantum materials. The combination of collectively suppressed photon losses and emerging optical nonlinearities due to strong photon coupling to mesoscopic numbers of emitters holds promise for generating nonclassical light and engineering effective interactions between freely propagating photons. While most studies have thus far relied on numerical simulations, we describe here a diagrammatic Green's function approach that permits analytical investigations of nonlinear processes. We illustrate the method by deriving a simple expression for the scattering matrix that describes photon-photon interactions in an extended two-dimensional array of quantum emitters and reproduces the results of numerical simulations of coherently driven arrays. The approach yields intuitive insights into the nonlinear response of the system and offers a promising framework for the systematic development of a theory for interacting photons and many-body effects on collective radiance in two-dimensional arrays of quantum emitters. Published by the American Physical Society 2024
Subwavelength arrays of quantum emitters offer an efficient free-space approach to coherent light-matter interfacing, using ultracold atoms or two-dimensional solid-state quantum materials. The combination of collectively suppressed photon losses and emerging optical nonlinearities due to strong photon coupling to mesoscopic numbers of emitters holds promise for generating nonclassical light and engineering effective interactions between freely propagating photons. While most studies have thus far relied on numerical simulations, we describe here a diagrammatic Green's function approach that permits analytical investigations of nonlinear processes. We illustrate the method by deriving a simple expression for the scattering matrix that describes photon-photon interactions in an extended two-dimensional array of quantum emitters and reproduces the results of numerical simulations of coherently driven arrays. The approach yields intuitive insights into the nonlinear response of the system and offers a promising framework for the systematic development of a theory for interacting photons and many-body effects on collective radiance in two-dimensional arrays of quantum emitters. Published by the American Physical Society 2024
The interaction between light and matter has captivated physicists for centuries, from early studies of vision and refraction in ancient Greece to the development of quantum mechanics and quantum electrodynamics in the past century. While the response of a single quantum emitter to light is well understood, the radiative properties of an ensemble of closely spaced emitters are far more intricate. Coupling to a shared electromagnetic environment induces coherent and dissipative interactions between emitters, giving rise to a collective response that cannot be captured by treating them independently. In the regime of few excitations, the system hosts delocalized subradiant states, that is, coherent superpositions that are largely decoupled from the electromagnetic field and thus decay at suppressed rates. While this weak coupling makes subradiant states attractive for quantum technologies, it also renders them difficult to manipulate. At higher excitation densities, the intrinsic nonlinearity of emitters and the exponential growth of the Hilbert space make theoretical and numerical descriptions of the system and its dynamics increasingly challenging. This thesis explores two fundamental questions: How can subradiant and dark states be selectively accessed and harnessed for practical applications in quantum technologies? And how can interacting ensembles of quantum emitters be efficiently simulated to uncover their many-body physics? The first part of the thesis develops protocols for controlling and addressing dark states in free-space and waveguide-coupled atomic arrays, demonstrating their utility in quantum storage and the deterministic generation of entangled photonic states. Incorporating atomic motion, we further show that collective subradiant states can enhance cooling in dense atomic arrays, offering new avenues for controlling motional dynamics. In the second part, we introduce cumulant expansions of the equations of motion as a powerful tool to analytically and numerically investigate collective decay in the many-body regime. We first examine the collective decay of fully excited atomic arrays in free space, characterizing the onset and scaling of the superradiant burst across different geometries. In collaboration with experiments on ultracold erbium atoms in optical lattices, we provide the first direct observations of many-body collective effects in free-space ordered arrays, including early-time superradiant bursts, late-time subradiant tails, and the emergence of atomic correlations throughout the dynamics. Finally, we theoretically and numerically explore the transient formation of multi-excitation subradiant states, and demonstrate how the existence of multiple dissipation channels suppresses steady-state superradiance in extended arrays.
We present a method to systematically study multiphoton transmission in one-dimensional systems comprised of correlated quantum emitters coupled to input and output waveguides. Within the Green's function approach of the scattering matrix (S matrix), we develop a diagrammatic technique to analytically obtain the system's scattering amplitudes while at the same time visualize all the possible absorption and emission processes. Our method helps to reduce the significant effort in finding the general response of a many-body bosonic system, particularly the nonlinear response embedded in the Green's functions. We demonstrate our proposal through physically relevant examples involving scattering of multiphoton states from two-level emitters as well as from arrays of correlated Kerr nonlinear resonators in the Bose-Hubbard model.
We consider the coupling of light, via an optical cavity, to two-dimensional atomic arrays whose lattice spacing exceeds the wavelength of the light. Such “superwavelength” spacing is typical of optical tweezer arrays. While subwavelength arrays exhibit strong atom-photon coupling, characterized by high optical reflectivity in free space, the coupling efficiency of superwavelength arrays is reduced due to collective scattering losses to high diffraction orders. We show how a moderate-finesse cavity can overcome these losses. As the scattering losses peak at certain discrete values of the lattice spacing, the spacing can be optimized to achieve efficient atom-photon coupling in the cavity. Our cavity-QED theory properly accounts for collective dipolar interactions mediated by the lossy, non-cavity-confined photon modes and for finite-size effects of both the array and the light field. These findings pave the way to harnessing the versatility of tweezer arrays for efficient atom-photon interfaces in applications of quantum computing, networking, and nonlinear optics. Published by the American Physical Society 2024
We develop a model describing long-range atom-atom interactions in a two-dimensional periodic or a-periodic lattice of optical centers considering spectral and spatial broadening effects. Using both analytical and numerical Green's function techniques, we develop a mathematical framework to describe effective atom-atom interactions and collective behaviors in the presence of disorder. This framework is applicable to a broad range of quantum systems with arbitrary lattice geometries, including cold atoms, solid-state photonics, and superconducting platforms. The model can be used, for example, to scalably design quantum optical elements, e.g. a quantum lens, harnessing atomistic engineering (e.g. via ion implantation) of collective interactions in materials to enhance quantum properties at scale.
The idea of making photons effectively interact has attracted a lot of interest in recent years, for several reasons. Firstly, since photons do not naturally interact with each other, it is of fundamental physical interest to see what kind of medium can mediate interactions between these fundamental and non-interacting particles, and to what extent. Secondly, photonics is a major candidate for future quantum technology, due to the easy manipulation, readout, and transport of photons, which makes them ideal for quantum information processing. Finally, achieving strong and tunable interactions among photons would open up an avenue for exploring the many-body physics of a fluid of light. In this thesis, we will see how a cavity formed of subwavelength lattices of two-level atoms can confine photons to a nonlinear environment for a long time, such that emitted photons have accumulated strong correlations both among their momenta and in their temporal statistics. This speaks of a strong photon-photon interaction within the cavity. The nonlinearity originates in the saturability of individual atoms, and the lattice structure results in a strong and low-loss collective interaction with light. While a single atomic lattice has a largely linear nature, as the effect of individual atoms washes out in the collective response, the confining geometry of the cavity means the photons are exposed to the underlying saturability of the atoms for such a long time that the nonlinearity is revived. We will analyse this system both using a standard input-output formalism, where the nonlinear physics of the system is handled numerically, and a powerful Green's function-based approach that allows for exact analytical results with no additional approximations. This analytical description has the potential to lead to an exact study of the many-body physics of interacting photons in a two-dimensional setting.
Engineering strong photon–photon interactions at the quantum level have been crucial in various areas of research, notably in quantum information processing and quantum simulation. It is often done by coupling matter strongly to light. A promising way to achieve this is via waveguide quantum electrodynamics (QED). Motivated by these advancements, we study few-photon transport in waveguide QED setups. First, we present a diagrammatic technique to systematically study multiphoton scattering based on the scattering formalism and Green’s function approach. We demonstrate our proposal through physically relevant examples involving scattering of few-photon states from two-level emitters as well as from arrays of correlated Kerr nonlinear resonators described by the Bose–Hubbard model. In the second part, we apply the diagrammatic technique that was developed to perform a comprehensive study on a Bose–Hubbard lattice with a quasi-periodic potential. This model exhibits many-body localisation. We compute the two-photon transmission probability and show that it carries signatures of the underlying localisation transition with close agreement to the participation ratio of the eigenstates. The systematic scattering approach provided in this paper provides a foundation for future works at the interface between quantum optics and condensed matter.