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arXiv:2107.05034 · Journal of Physics Condensed Matter

Non-Markovian transients in transport across chiral quantum wires using space–time non-equilibrium Green functions

Nikhil Danny Babu, Girish S Setlur

Published Dec 22, 2021• 1 citation
arXivHTMLPDF

Abstract

Abstract We study a system of two non-interacting quantum wires with fermions of opposite chirality with a point contact junction at the origin across which tunneling can take place when an arbitrary time-dependent bias between the wires is applied. We obtain the exact dynamical non-equilibrium Green function by solving Dyson’s equation analytically. Both the space–time dependent two and four-point functions are written down in a closed form in terms of simple functions of position and time. This allows us to obtain, among other things, the I–V characteristics for an arbitrary time-dependent bias. Our method is a superior alternative to competing approaches to non-equilibrium as we are able to account for transient phenomena as well as the steady state. We study the approach to steady state by computing the time evolution of the equal-time one-particle Green function. Our method can be easily applied to the problem of a double barrier contact whose internal properties can be adjusted to induce resonant tunneling leading to a conductance maximum. We then consider the case of a finite bandwidth in the point contact and calculate the non-equilibrium transport properties which exhibit non-Markovian behaviour. When a subsequently constant bias is suddenly switched on, the current shows a transient build up before approaching its steady state value in contrast to the infinite bandwidth case. This transient property is consistent with numerical simulations of lattice systems using time-dependent density matrix renormalization group suggesting thereby that this transient build up is merely due to the presence of a short distance cutoff in the problem description and not on the other details.

DOI
10.1088/1361-648x/ac45b6

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Abstract We study a system of two non-interacting quantum wires with fermions of opposite chirality with a point contact junction at the origin across which tunneling can take place when an arbitrary time-dependent bias between the wires is applied. We obtain the exact dynamical non-equilibrium Green function by solving Dyson’s equation analytically. Both the space–time dependent two and four-point functions are written down in a closed form in terms of simple functions of position and time. This allows us to obtain, among other things, the I–V characteristics for an arbitrary time-dependent bias. Our method is a superior alternative to competing approaches to non-equilibrium as we are able to account for transient phenomena as well as the steady state. We study the approach to steady state by computing the time evolution of the equal-time one-particle Green function. Our method can be easily applied to the problem of a double barrier contact whose internal properties can be adjusted to induce resonant tunneling leading to a conductance maximum. We then consider the case of a finite bandwidth in the point contact and calculate the non-equilibrium transport properties which exhibit non-Markovian behaviour. When a subsequently constant bias is suddenly switched on, the current shows a transient build up before approaching its steady state value in contrast to the infinite bandwidth case. This transient property is consistent with numerical simulations of lattice systems using time-dependent density matrix renormalization group suggesting thereby that this transient build up is merely due to the presence of a short distance cutoff in the problem description and not on the other details.
We study a system of two non-interacting quantum wires with fermions of opposite chirality with a point-contact junction at the origin across which tunneling can take place when an arbitrary time-dependent bias between the wires is applied. We obtain the exact dynamical non-equilibrium Green function by solving Dyson's equation analytically. Both the space-time dependent two and four-point functions are written down in a closed form in term of simple functions of position and time. This allows us to obtain among other things, the I-V characteristics for an arbitrary time-dependent bias. Our method is a superior alternative to competing approaches to non-equilibrium as we are able to account for transient phenomena as well as the steady state. We study the approach to steady state by computing the time-evolution of the equal-time one-particle Green function. We also show how the presence of the point-contact affects the density profile of the electrons by inducing Friedel oscillations in the system and how the presence of a bias influences these oscillations.
Non-chiral bosonization technique adapted to study chiral quantum wires with non-interacting fermions coupled through a point-contact with a constant bias between the wires is introduced and is shown to reproduce the exact Green functions of this system which was previously derived by the present authors analytically using standard methods. The tunneling I-V characteristics are obtained using the bosonized Green functions. The proposed unconventional bosonization scheme is also shown to be internally consistent as the four-point functions evaluated using NCBT are shown to be related to the two-point functions through Wick's theorem as it should be. In equilibrium, the equal space-time NCBT Green functions for an interacting Luttinger liquid with impurities obtained in a previous work shows universal scaling behaviour in accordance with Bethe ansatz and functional renormalization group predictions. We expect to obtain a similar scaling form of the tunneling properties out of equilibrium in presence of interparticle interactions.
We propose a time-dependent many-body approach to study the short-time dynamics of correlated electrons in quantum transport through nanoscale systems contacted to metallic leads. This approach is based on the time propagation of the Kadanoff-Baym equations for the nonequilibrium many-body Green's function of open and interacting systems out of equilibrium. An important feature of the method is that it takes full account of electronic correlations and embedding effects in the presence of time-dependent external fields, while at the same time satisfying the charge conservation law. The method further extends the Meir-Wingreen formula to the time domain for initially correlated states. We study the electron dynamics of a correlated quantum wire attached to two-dimensional leads exposed to a sudden switch on of a bias voltage using conserving many-body approximations at Hartree-Fock, second Born and GW level. We obtain detailed results for the transient currents, dipole moments, spectral functions, charging times, and the many-body screening of the quantum wire as well as for the time-dependent density pattern in the leads, and we show how the time dependence of these observables provides a wealth of information on the energy level structure of the quantum wire out of equilibrium. For moderate interaction strengths the second Born and GW results are in excellent agreement at all times. We find that many-body effects beyond the Hartree-Fock approximation have a large effect on the qualitative behavior of the system and lead to a bias-dependent gap closing and quasiparticle broadening, shortening of the transient times and washing out of the step features in the current-voltage curves.
In this thesis, certain aspects of time-dependent quantum transport properties in nanoscale structures are investigated using the non-equilibrium Green’s function(NEGF). For the transient behaviors of the electric current and heat current after a quantum quench, the exact analytical solution beyond the wide band limit (WBL) is obtained for the first time which paves a way to simulate realistic physical systems. The time-dependent thermoelectric effects are evaluated based on this general solution and it is shown that the time-dependent thermopower is significantly enhanced in the transient regime. By taking initial correlation into account, the combined Caroli and Cini scheme in quantum transport is proposed and its exact solution beyond WBL is derived for the first time as well. Furthermore, besides the average electric current, a current conserving and gauge invariant formalism for the total electric current operator is established at equilibrium state with the help of the electric displacement current operator formulated by taking the Coulomb interaction into account at the operator level. By means of the NEGF and the scattering matrix theory (SMT), a current conserving theory for equilibrium noise power at finite frequencies is obtained which solves one of the fundamental problems in quantum transport. A generalized equilibrium fluctuation-dissipation theorem is presented. Moreover, the entanglement entropy \nfluctuation and its distribution are investigated by introducing the entanglement entropy operator. The essential feature of the entanglement entropy generated by quantum transport is that it is a stochastic quantity whose fluctuation and distribution can be obtained from the generating function (GF). Combining the NEGF with the Grassmann algebras, it is found that the GF of entanglement \nentropy can be expressed in terms of the lesser Green’s function of the subsystem. The general relation connecting the full counting statistics (FCS) of charge transfer with the GF of entanglement entropy is found which indicates that, from the experimental point of view, the entanglement entropy fluctuation can be measured indirectly. As an illustration of the general theoretical framework of entanglement entropy fluctuation, the quantum point contact (QPC) system as well as the quantum dot (QD) system are studied. It is shown that for a QPC under dc bias, the entanglement entropy is maximized and fluctuationless when the transmission coefficient T is one-half. For the quantum dot system, at short times, a universal scaling relation among transient peak values of cumulants of entanglement entropy is shown.
In this review article, we present a non-equilibrium quantum transport theory for transient electron dynamics in nanodevices based on exact Master equation derived with the path integral method in the fermion coherent-state representation. Applying the exact Master equation to nanodevices, we also establish the connection of the reduced density matrix and the transient quantum transport current with the Keldysh nonequilibrium Green functions. The theory enables us to study transient quantum transport in nanostructures with back-reaction effects from the contacts, with non-Markovian dissipation and decoherence being fully taken into account. In applications, we utilize the theory to specific quantum transport systems, a variety of quantum decoherence and quantum transport phenomena involving the non-Markovian memory effect are investigated in both transient and stationary scenarios at arbitrary initial temperatures of the contacts.
In this paper, we present a non-equilibrium quantum theory for transient electron dynamics in nanodevices based on the Feynman–Vernon influence functional. Applying the exact master equation for nanodevices we recently developed to the more general case in which all the constituents of a device vary in time in response to time-dependent external voltages, we obtained non-perturbatively the transient quantum transport theory in terms of the reduced density matrix. The theory enables us to study transient quantum transport in nanostructures with back-reaction effects from the contacts, with non-Markovian dissipation and decoherence being fully taken into account. For a simple illustration, we apply the theory to a single-electron transistor subjected to ac bias voltages. The non-Markovian memory structure and the nonlinear response functions describing transient electron transport are obtained.