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arXiv:2106.05776 · Physical review. E

Intermediate-times dilemma for open quantum system: Filtered approximation to the refined weak-coupling limit

Marek Winczewski, Antonio Mandarino, Gerardo Suárez, Robert Alicki, Michał Horodecki

Published Aug 5, 2024• 12 citations
arXivHTMLPDF

Abstract

The famous Davies-GKSL secular Markovian master equation is tremendously successful in approximating the evolution of open quantum systems in terms of just a few parameters. However, the fully secular Davies-GKSL equation fails to accurately describe timescales short enough, i.e., comparable to the inverse of differences of frequencies present in the system of interest. A complementary approach that works well for short times but is not suitable after this short interval is known as the quasisecular master equation. Still, both approaches fail to have any faithful dynamics in the intermediate-time interval. Simultaneously, descriptions of dynamics that apply to the aforementioned "gray zone" often are computationally much more complex than master equations or are mathematically not well-structured. The filtered approximation (FA) to the refined weak-coupling limit has the simplistic spirit of the Davies-GKSL equation and allows capturing the dynamics in the intermediate-time regime. At the same time, our non-Markovian equation yields completely positive dynamics. We exemplify the performance of the FA equation in the cases of the spin-boson system and qutrit-boson system in which two distant timescales appear.

DOI
10.1103/physreve.110.024110

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The famous Davies-GKSL secular Markovian master equation is tremendously successful in approximating the evolution of open quantum systems in terms of just a few parameters. However, the fully secular Davies-GKSL equation fails to accurately describe timescales short enough, i.e., comparable to the inverse of differences of frequencies present in the system of interest. A complementary approach that works well for short times but is not suitable after this short interval is known as the quasisecular master equation. Still, both approaches fail to have any faithful dynamics in the intermediate-time interval. Simultaneously, descriptions of dynamics that apply to the aforementioned "gray zone" often are computationally much more complex than master equations or are mathematically not well-structured. The filtered approximation (FA) to the refined weak-coupling limit has the simplistic spirit of the Davies-GKSL equation and allows capturing the dynamics in the intermediate-time regime. At the same time, our non-Markovian equation yields completely positive dynamics. We exemplify the performance of the FA equation in the cases of the spin-boson system and qutrit-boson system in which two distant timescales appear.
In recent years, there has been tremendous focus on identifying whether effective descriptions of open quantum systems such as master equations can accurately describe the dynamics of open quantum systems. One particular question is whether they provide the correct steady state in the long time limit. The transient regime is also of interest. Description of evolution by various master equations---some of them being not completely positive---is benchmarked against exact solutions [see, e.g., R. Hartmann and W. T. Strunz, Phys. Rev. A 101, 012103 (2020)]. An important property of true evolution is its non-Markovian features, which are not captured by the simplest completely positive master equations. In this paper we consider a non-Markovian yet completely positive evolution (known as refined weak coupling or cumulant equation) for the spin-boson model with an overdamped Drude-Lorentz spectral density and arbitrary coupling. We benchmark it against a numerically exact solution, as well as against other master equations, for different coupling strengths and temperatures. We find the cumulant to be a better description in the weak-coupling regime where it is supposed to be valid. For the examples considered it shows superiority at moderate and strong couplings in the low-temperature regime for all examples considered. In the high-temperature regime, however, its advantage vanishes. This indicates that the cumulant equation is a good candidate for simulations at weak to moderate coupling and low temperature. Our calculations are greatly facilitated due to our concise formulation of the cumulant equation by means of representation of the density matrix in the SU(N) basis.
Derivation of a quantum master equation for a system weakly coupled to a bath which takes into account non-secular effects, but, nevertheless, has the mathematically correct Gorini-Kossakowski-Lindblad-Sudarshan (GKLS) form (in particular, preserves positivity of the density operator) and also satisfies the standard thermodynamic properties is a known long-standing problem in theory of open quantum systems. The non-secular terms are important when some energy levels of the system or their differences (Bohr frequencies) are nearly degenerate. We provide a fully rigorous derivation of such equation based on a formalization of the weak-coupling limit for the general case.
Periodically driven open quantum systems are central to quantum thermodynamics and quantum control. These systems are typically described using Floquet-Born-Markov master equations, derived with the use of a full secular approximation, and whose thermodynamic implications are often overlooked. In this context, we show that such a strong secular approximation may lead to unphysical predictions for steady state energy currents. We then demonstrate that a coarse-grained formulation of the master equation can regularize these issues while yielding completely positive dynamics and consistent energy currents. The coarse-graining time has a clear physical interpretation, as it defines the temporal resolution at which a Markovian master equation can describe the evolution of the periodically driven system. We show the consistency and validity of our approach by comparing to an exact non-Markovian simulation in paradigmatic examples: a driven two-level system and a three-level maser coupled to hot and cold thermal reservoirs. Our work provides a practical framework for correctly applying the secular approximation in periodically driven-dissipative systems and for assessing the accuracy of master equations of the GKSL form.
We study the properties of a refined weak-coupling limit that preserves complete positivity in order to describe non-Markovian dynamics in the spin-boson model. With this tool, we show the system presents a rich non-Markovian phenomenology. This implies a dynamical difference between entanglement and coherence: the latter undergoes revivals, whereas the former not, despite the induced dynamics being fully incoherent. In addition, the evolution presents ``quasieternal'' non-Markovianity, becoming nondivisible at any time period where the system evolves qualitatively. Furthermore, the method allows for an exact derivation of a master equation that accounts for a reversible energy exchange between system and environment. Specifically, this is obtained in the form of a time-dependent Lamb shift term.
We develop a framework that allows us to describe the dynamics of the total state of an open quantum system and its bosonic environment in the usual Born (weak coupling) and Markov approximation. By shifting the whole time-dependence into an unnormalized s-operator of the open system, the full dynamics is captured by an s-master equation of similar structure than the well-known Gorini-Kossakowski-Sudarshan-Lindblad (GKSL) master equation for the reduced dynamics. By varying the ordering parameter s (0 ≤ s ≤ 1) we obtain the partial Husimi representation (s = 0) and the partial Glauber-Sudarshan representation (s = 1) for the dynamics of the total state. For the reduced density operator the GKSL master equation can be derived easily. The case of s = 1/2, leading to a partial Wigner representation, is helpful to study the overlap of states in the total Hilbert space of system and environment.
In various fields from quantum physics to biology, the open quantum dynamics of a system consisting of interacting subsystems emphasizes its fundamental functionality. The local approach, deriving a dissipator in a master equation by ignoring the inter-subsystem interaction, has been widely used to describe the reduced dynamics due to its robustness to keep the positivity of a density operator. However, one critique is that a stationary state obtained by the approach in the limit of weak system-environment coupling is written in the form of the Gibbs state for the partial Hamiltonian by excluding the inter-subsystem interaction from the total one of the relevant system. As an alternative, the global approach, deriving a dissipator with including the inter-subsystem interaction, under the Born--Markov and secular approximations has attracted much attention, and there is debate concerning its violation of positivity in the short-term region and/or limited parameter region for the Bohr frequencies of the subsystems. In this study, we present a formalism that leads to the time-convolutionless (time-local) master equation obtained by extending the global approach beyond the Born-Markov and secular approximations. We apply it to the excitation energy transfer between interacting sites in which only the terminal site weakly interacts with a bosonic environment of finite temperature in a manner beyond the rotating-wave approximation. We find that the formulation (1) gives the short-time behavior while preserving positivity, (2) shows the oscillatory features that the secular approximation would obscure, and (3) leads to a stationary state very near to the Gibbs state for the total Hamiltonian of the relevant system.