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arXiv:2106.02038 · Physical review. B./Physical review. B

Reentrant Bloch ferromagnetism

DinhDuy Vu, S. Das Sarma

Published Sep 8, 2021• 1 citation
arXivHTMLPDF

Abstract

An interacting electron liquid in two (2D) and three (3D) dimensions may undergo a paramagnetic-to-ferromagnetic quantum spin polarization transition at zero applied magnetic field, driven entirely by exchange interactions, as the system density ($n$) is decreased. This is known as Bloch ferromagnetism. We show theoretically that the application of an external magnetic field ($B$), which directly spin polarizes the system through Zeeman spin splitting, has an interesting effect on Bloch ferromagnetism if the applied field and carrier density are both decreased (from some initial applied high magnetic field at a high carrier density) in a power-law manner, $B\ensuremath{\sim}{n}^{p}$. For $p<{p}_{c}$, with ${p}_{c}=1(2/3)$ in $2(3)\mathrm{D}$, the system remains either fully spin polarized or undergoes a single transition from a partially spin-polarized (with two Fermi surfaces corresponding to spin up and down electrons) to a fully spin-polarized state (with a single Fermi surface of one spin) as the density and field decrease, depending on whether the starting point is partially spin polarized or fully spin polarized. However, for $p>{p}_{c}$, the system may undergo two transitions if starting from the fully spin-polarized state: first, a weak second-order transition at high density and field from the field-induced fully polarized phase to the partially polarized phase; and then, at a lower field and density, a reentrant first-order transition back to the fully spin-polarized phase again with a single Fermi surface.

DOI
10.1103/physrevb.104.l100405

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•Aug 10, 2021•0 citations
An interacting electron liquid in two (2D) and three (3D) dimensions may undergo a paramagnetic-to-ferromagnetic quantum spin polarization transition at zero applied magnetic field, driven entirely by exchange interactions, as the system density (nnn) is decreased. This is known as Bloch ferromagnetism. We show theoretically that the application of an external magnetic field (BBB), which directly spin polarizes the system through Zeeman spin splitting, has an interesting effect on Bloch ferromagnetism if the applied field and carrier density are both decreased (from some initial applied high magnetic field at a high carrier density) in a power-law manner, B\ensuremath∼npB\ensuremath{\sim}{n}^{p}B\ensuremath∼np. For p<pcp<{p}_{c}p<pc​, with pc=1(2/3){p}_{c}=1(2/3)pc​=1(2/3) in 2(3)D2(3)\mathrm{D}2(3)D, the system remains either fully spin polarized or undergoes a single transition from a partially spin-polarized (with two Fermi surfaces corresponding to spin up and down electrons) to a fully spin-polarized state (with a single Fermi surface of one spin) as the density and field decrease, depending on whether the starting point is partially spin polarized or fully spin polarized. However, for p>pcp>{p}_{c}p>pc​, the system may undergo two transitions if starting from the fully spin-polarized state: first, a weak second-order transition at high density and field from the field-induced fully polarized phase to the partially polarized phase; and then, at a lower field and density, a reentrant first-order transition back to the fully spin-polarized phase again with a single Fermi surface.
Magnetic properties of two-dimensional (2D) spin-polarized Fermi gas with dipole-dipole interaction are studied in the presence of external magnetic field at zero temperature. Within perturbation theory and the second quantization formalism, the total energy is explicitly obtained as a function of three dimensionless parameters: the spin polarization, dipolar coupling, and Zeeman parameters. We examine the effects of these agents on the magnetic properties of 2D Fermi gas. The results show that an induced ferromagnetic phase transition is observed only for adequately large values of magnetic field. This paper offers two controllable factors to change the spin polarization of the system.
Alexander Shashkin Institute of Solid State Physics, Chernogolovka, Moscow District 142432, Russia Sergey Kravchenko Physics Department, Northeastern University, Boston, Massachusetts 02115, U.S.A. Two-dimensional (2D) electron systems are realized when the electrons are free to move in a plane but their motion perpendicular to the plane is quantized in a confining potential well. Quantum phase transitions realized experimentally in such systems so far include metal-insulator transitions in perpendicular magnetic fields, metal-insulator transition in zero magnetic field, and a possible transition to a Wigner crystal. The first transition is governed by the externally controlled electron density or magnetic field, while the other two are governed by the electron density. At low electron densities in 2D systems, the strongly-interacting limit is reached because the kinetic energy is overwhelmed by the energy of electron-electron interactions. The interaction strength is characterized by the ratio between the Coulomb energy and the Fermi energy, r∗s = Eee/EF . Assuming that the effective electron mass is equal to the band mass, the interaction parameter r∗s in the single-valley case reduces to the Wigner-Seitz radius, rs = 1/(πns)1/2aB, and therefore increases as the electron density, ns, decreases (here aB is the Bohr radius in the semiconductor). Possible candidates for the ground state of the system include a Wigner crystal characterized by spatial and spin ordering [1], a ferromagnetic Fermi liquid with spontaneous spin ordering [2], a paramagnetic Fermi liquid [3], etc. In the strongly-interacting limit (rs 1), no analytical theory has been developed to date. According to numerical simulations [4], Wigner crystallization is expected in a very dilute regime, when rs reaches approximately 35. Refined numerical simulations [5] have predicted that prior to the crystallization, in the range of the interaction parameter 25 ≤ rs ≤ 35, the ground state of the system is a strongly correlated ferromagnetic Fermi liquid. At higher electron densities, rs ∼ 1, the electron liquid is expected to be paramagnetic, with the effective mass, m, and Lande´ g factor renormalized by interactions. Apart from the ferromagnetic Fermi liquid, other intermediate phases between the Wigner crystal and the paramagnetic Fermi liquid may also exist.
Based on recent experimental evidence for a spin-polarized ground state in the insulating phase of the two-dimensional electron system, we propose that ferromagnetic spin fluctuations lead to an attractive interaction in the triplet channel and cause p-wave pairing in the conducting phase. We use the Landau-Fermi liquid phenomenology to explain how the enhanced spin susceptibility near the critical density yields an attractive potential, in a similar mechanism to superfluidity in 3He.{}^{3}\mathrm{He}.3He. As the density is decreased, the p-wave order parameter undergoes a transition from a unitary to a nonunitary state, in which it coexists with ferromagnetism for a range of densities. As the density is further reduced, the pairing amplitude vanishes and the system is described by a ferromagnetic insulator. Thus, we find two quantum critical points as a function of density associated with the polarization of the paired state and ferromagnetism. We explain the magnetotransport measurements in parallel and perpendicular magnetic fields and propose a shot-noise experiment to measure the pair charge.
The Kitaev model with an applied magnetic field in the [Formula: see text] direction shows two transitions: from a nonabelian gapped quantum spin liquid (QSL) to a gapless QSL at [Formula: see text] and a second transition at a higher field [Formula: see text] to a gapped partially polarized phase, where K is the strength of the Kitaev exchange interaction. We identify the intermediate phase to be a gapless U(1) QSL and determine the spin structure function [Formula: see text] and the Fermi surface [Formula: see text] of the gapless spinons using the density matrix renormalization group (DMRG) method for large honeycomb clusters. Further calculations of static spin-spin correlations, magnetization, spin susceptibility, and finite temperature-specific heat and entropy corroborate the gapped and gapless nature of the different field-dependent phases. In the intermediate phase, the spin-spin correlations decay as a power law with distance, indicative of a gapless phase.
The nature of the ground state of degenerate two dimensional (2D) fermions at zero magnetic field is an outstanding open problem, which has not been deciphered despite decades of research. In the absence of disorder, the ground state is believed to be determined by the interplay between the kinetic energy, E f, and the inter-particle interaction energy, Ec = e2/ica, where a = (nn)~1^ 2 is the typical inter-particle distance, n is the areal particle density, and k is the host dielectric constant. The relative importance of the two energy scales is characterized by rs = a/ao, with ao being the Bohr radius. For electrons in a single band, rs = Ec/ E f while for the (100) surface of silicon rs = Ec/2E p , due to the two-fold valley degeneracy. At very high densities (rs <£ 1) a 2D system approaches the paramagnetic limit of a non-interacting degenerate gas characterized by the Pauli susceptibility, xo • As the density is reduced, the growing ferromagnetic correlations lead to substantial enhancement of the spin susceptibility, The system is predicted to remain paramagnetic up to rs « 20, where numerical calculations [1] find a quantum phase transition to a ferromagnetic liquid phase [2]. At lower density, rs & 37 [3], the Coulomb correlations are predicted to lead to a second phase transition to an anti-ferromagnetic quantum Wigner crystal. The energy balance between the ferro and paramagnetic states is very subtle, therefore the density window where ferromagnetism can take place is small [1].
Quantum Hall systems have a one-body energy spectrum consisting of dispersion-less Landau levels. Electron-electron interactions thus dominate in partially filled Landau levels, which exhibit a myriad of strongly correlated phases such as quantum hall ferromagnets and fractional quantum Hall phases. We study two examples of these phenomena. In the first project, we explore the ground state of a system with an interface between two semi-infinite regions with fillings ν= 4 and ν= 3 respectively. The width of the interface can be controlled by varying the background potential, which provides an additional tuning parameter. For a certain range of interaction strengths, the ν= 4 bulk is unpolarized whereas the ν= 3 bulk is fully polarized. In the parameter space spanned by the interaction strength and width of the interface, we find two phases at the interface. Phase A has spin as a good quantum number, and the long-wavelength spin edge excitations are gapped. In phase B, spin rotation symmetry is spontaneously broken at the mean-field level. Using symmetry arguments we find the effective theory near the interface of phase B. This effective theory is known to have gapless long-wavelength spin excitations. In the second project, we study the ground state of a tunnel-decoupled double-layer graphene system when both layers are undoped. We find a simple Hamiltonian in the continuum limit from symmetries of the system. Using the Hartree-Fock approximation we find a state with inter-layer coherence with broken layer U(1) symmetry. This phase becomes magnetized in presence of a non-zero Zeeman field. A first-order phase transition can be driven from the ferromagnetic phase to the magnetized inter-layer coherent phase by increasing the Zeeman field. We predict the number of gapless modes in the bulk.