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arXiv:2104.10237 · Journal of Physics Communications

Polymer-loaded three dimensional microwave cavities for hybrid quantum systems

Myles Ruether, C. A. Potts, J. P. Davis, Lindsay J. LeBlanc

Published Nov 24, 2021• 5 citations
arXivHTMLPDF

Abstract

Abstract Microwave cavity resonators are crucial components of many quantum technologies and are a promising platform for hybrid quantum systems, as their open architecture enables the integration of multiple subsystems inside the cavity volume. To suspend these subsystems within the centre of a cavity where field strengths are strong and uniform, auxiliary support structures are often required, but the effects of these structures on the microwave cavity mode are difficult to predict due to a lack of a priori knowledge of the materials’ response in the microwave regime. Understanding these effects becomes even more important when frequency matching is critical and tuning is limited, for example, when matching microwave modes to atomic resonances for atomic vapour cells inside enclosed microwave cavities. Here, we study the microwave cavity mode in the presence of three commonly-used machinable polymers, paying particular attention to the change in resonance and the dissipation of energy. We demonstrate how to use the derived dielectric coefficient for cavity design in a test case, wherein we match a polymer-filled 3D microwave cavity to a hyperfine transition in rubidium.

DOI
10.1088/2399-6528/ac3cff

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Abstract Microwave cavity resonators are crucial components of many quantum technologies and are a promising platform for hybrid quantum systems, as their open architecture enables the integration of multiple subsystems inside the cavity volume. To suspend these subsystems within the centre of a cavity where field strengths are strong and uniform, auxiliary support structures are often required, but the effects of these structures on the microwave cavity mode are difficult to predict due to a lack of a priori knowledge of the materials’ response in the microwave regime. Understanding these effects becomes even more important when frequency matching is critical and tuning is limited, for example, when matching microwave modes to atomic resonances for atomic vapour cells inside enclosed microwave cavities. Here, we study the microwave cavity mode in the presence of three commonly-used machinable polymers, paying particular attention to the change in resonance and the dissipation of energy. We demonstrate how to use the derived dielectric coefficient for cavity design in a test case, wherein we match a polymer-filled 3D microwave cavity to a hyperfine transition in rubidium.
Frequency tunability of three dimensional (3D) microwave cavities opens up numerous possibilities for their use in hybrid quantum systems and related technologies. For many applications, it is desirable to tune the resonance at cryogenic temperatures without mechanical actuation. We show that a superconducting 3D microwave cavity can be tuned at the percent level by taking advantage of the dielectric properties of superfluid 4He at millikelvin temperatures, without affecting its intrinsic quality factor—reaching 3 × 105 in the present experiment.
Vapor-cell devices based on microwave interrogation provide a stable frequency reference with a compact and robust setup. Further miniaturization must focus on optimizing the physics package, containing the microwave cavity and atomic reservoir. In this article, we present a compact cavity-cell assembly based on a dielectric-loaded cylindrical resonator. The loaded cavity resonating at 6.83 GHz has an external volume of only 35 cm3and accommodates a vapor cell with 0.9-cm3inner volume. The proposed design aims at strongly reducing the core of the atomic clock, maintaining, at the same time, high-performing short-term stability (σy(τ)≤5×10−13 τ−1/2\sigma _{y}{(}\tau {)} \leq {5}\times {10}^{-{13}} \,\tau ^{-{1}/{2}}σy​(τ)≤5×10−13τ−1/2 standard Allan deviation). The proposed structure is characterized in terms of microwave field uniformity and atom-field coupling with the aid of finite-element calculations. The thermal sensitivity is also analyzed and experimentally characterized. We present preliminary spectroscopy results by integrating the compact cavity within a rubidium clock setup based on the pulsed optically pumping technique. The obtained clock signals are compatible with the targeted performances. The loaded-cavity approach is, thus, a viable design option for miniaturized microwave clocks.
When in a quantum optical system the coupling between matter and cavity mode becomes comparable to the bare excitation frequency, we enter a non-perturbative coupling regime, as perturbation theory fails describing the system’s dynamics. While recent advances in Cavity Quantum Electrodynamics allowed to achieve very high values of the coupling strength, thanks to the resonators properties optimization and the employment of solid-state devices, an ever growing interest has been shown about the possibility of significantly modify materials’ properties. It has been demonstrated that the chemical structure of molecules strongly coupled to a photon mode can be altered, which opens the possibility to manipulate and control chemical reactions. The aim of this thesis is to explore non-perturbative regimes on several quantum systems, and to investigate the effects of the coupling upon their properties, such as internal degrees of freedom or electronic states structure. I first developed a novel theory to determine the polariton spectrum of a dipolar ensamble in which a Ising-like dipole-dipole interaction in the 2 non-perturbative regime is considered. A further important focus is the investigation of the saturation effects due to the inclusion of the inter-dipole interaction, and the interplay between the latter and light-matter coupling strength. I also explored specifically the influence of the coupling on the rotational degrees of freedom of an ensemble of two-dimensional freely rotating dipoles, all coupled to a single cavity mode, finding that they are driven by the collective light-matter coupling to undergo a crossover between an isotropic and an aligned phase. I then investigated the case of cavity-embedded doped quantum wells, demonstrating that not only it is possible to couple a discrete cavity mode and bound-to-continuum transitions, but also that a novel bound exciton state appears, induced by the coupling strength. This results shows how light–matter coupling can be used to tune both optical and electronic properties of semiconductor heterostructures beyond those permitted by mere crystal properties. Finally, I explored the physics of an array of THz metamaterial resonators coupled to cyclotron resonances of a two-dimensional electron gas, developing a multiple-mode theory that takes in account the interaction between multiple photon modes mediated by the electrons. My results show that this cross-interaction, due to the strong two-dimensional geometry of the optically active medium, leads to the hybridization of different uncoupled photon modes, and manifests as a visible change of the distribution of the coupled electromagnetic field.
We report on a technique for applying a DC bias in a 3D microwave cavity. We achieve this by isolating the two halves of the cavity with a dielectric and directly using them as DC electrodes. As a proof of concept, we embed a variable capacitance diode in the cavity and tune the resonant frequency with a DC voltage, demonstrating the incorporation of a DC bias into the 3D cavity with no measurable change in its quality factor at room temperature. We also characterize the architecture at millikelvin temperatures and show that the split cavity design maintains a quality factor Qi ∼ 8.8 × 105, making it promising for future quantum applications.
In the near-concentric regime, the transverse modes of an optical cavity have small mode volumes with a beam waist on the order of the atomic cross section. This shows potential for strong interaction between single atoms and light, which is a key component in distributed quantum computing architectures [1] . Furthermore, with centimetresized near-concentric cavities, the frequency spacing of the transverse modes ranges from tens of MHz to a GHz, matching well with the hyperfine or the Zeeman level splitting of an atom [2] . This near-degeneracy in resonant frequencies close to the critical point allows to explore the physics of atomic nonlinearities with multiple photonic modes strongly coupled to different hyperfine or magnetic energy levels of a quantum emitter.
Harmonic oscillators might be one of the most fundamental entities described by physics. Yet they stay relevant in recent research. The topological properties associated with exceptional points that can occur when two modes interact have generated much interest in recent years. Harmonic oscillators are also at the heart of new quantum technological applications: the long lifetime of high-Q resonators make them advantageous as quantum memories, and they are employed for narrowband processing of quantum signals, as in Josephson parametric amplifiers. The goal of this thesis is to explore different fundamental regimes of two coupled harmonic oscillators using cavity optomechanics as the experimen- tal platform. With consistent progress in attaining ever increasing Q factors, mechanical and electromagnetic resonators realize near-ideal harmonic oscillators. By parametrically modulating the nonlinear optomechanical interaction between them, an effective linear coupling is achieved, which is tunable in strength and in the relative frequencies of the two modes. Thus cavity optomechanics provides a framework with excellent control over system parameters for the study of two coupled harmonic modes. The specific optomechanical implementation employed are superconducting circuits with the vibrating top plate of a capacitor as the mechanical element. Multimode optomechanical circuits are realized, with two microwave modes interacting with one or two mechanical oscillators. The supplementary modes serve either as intermediaries in the relation of the two modes of interest, or as auxiliaries used to control a parameter of the system. Three main experimental results are achieved. First, an auxiliary microwave mode allows the engineering of the effective dissipation rate of a mechanical oscillator. The latter then acts as a reservoir for the main microwave mode with which it interacts. The microwave mode susceptibility can be tuned, resulting in an instability akin to that of a maser and in resonant amplification of incoming microwave signals with an added noise close to the quantum minimum. Second, we study the conditions for a nonreciprocal interaction between two microwave modes, when the information flows in one direction but not in the other. The two modes interact through two mechanical oscillators, leading to frequency conversion between the two cavities. Dissipation in the mechanical modes is essential to the scheme in two ways: it provides a reciprocal phase necessary for the interference and eliminates the unwanted signals. Third, level attraction between a microwave and a mechanical mode is demonstrated, where the eigenfrequencies of the system are drawn closer as the result of interaction, rather distancing themselves as in the more usual case of level repulsion. The phenomenon is theoretically connected to exceptional points, and a general classification of the possible regimes of interaction between two harmonic modes is exposed, including level repulsion and attraction as special cases.