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arXiv:2104.05760 · New Journal of Physics

Preparation of one 87Rb and one 133Cs atom in a single optical tweezer

R V Brooks, S Spence, A Guttridge, Alexandros C Alampounti, A Rakonjac, L A McArd, Jeremy M. Hutson, Simon L. Cornish

Published May 11, 2021• 25 citations
arXivHTMLPDF

Abstract

Abstract We report the preparation of exactly one 87Rb atom and one 133Cs atom in the same optical tweezer as the essential first step towards the construction of a tweezer array of individually trapped 87Rb133Cs molecules. Through careful selection of the tweezer wavelengths, we show how to engineer species-selective trapping potentials suitable for high-fidelity preparation of Rb + Cs atom pairs. Using a wavelength of 814 nm to trap Rb and 938 nm to trap Cs, we achieve loading probabilities of 0.508(6) for Rb and 0.547(6) for Cs using standard red-detuned molasses cooling. Loading the traps sequentially yields exactly one Rb and one Cs atom in 28.4(6)% of experimental runs. Using a combination of an acousto-optic deflector and a piezo-controlled mirror to control the relative position of the tweezers, we merge the two tweezers, retaining the atom pair with a probability of 0.9 9 ( − 0.02 ) ( + 0.01 ) . We use this capability to study hyperfine-state-dependent collisions of Rb and Cs in the combined tweezer and compare the measured two-body loss rates with coupled-channel quantum scattering calculations.

DOI
10.1088/1367-2630/ac0000

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Qubits encoded in the electronic states of single atoms trapped in arrays of optical tweezers are a promising platform for a universal quantum computer. These qubits can be prepared in a well-defined quantum state, coherently manipulated using a nearresonant driving field, and their state detected with high fidelity. The most promising aspect of this platform is the large scalability, with arrays of up to 6100 qubits demonstrated[62].We present our progress in developing such a system with an array of single 85Rbatoms. We provide an overview of the experimental setup constructed for this purpose. Typically 50 atoms are loaded from a MOT into a 10×10 array of optical tweezers with sub-micrometer waists, with only a single atom present in a tweezer. The occupation of the tweezers is determined using a fluorescence image. We provide a characterisation of the trapping potentials experienced by the atoms. 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•Oct 28, 2025•0 citations
Abstract We report the preparation of exactly one 87Rb atom and one 133Cs atom in the same optical tweezer as the essential first step towards the construction of a tweezer array of individually trapped 87Rb133Cs molecules. Through careful selection of the tweezer wavelengths, we show how to engineer species-selective trapping potentials suitable for high-fidelity preparation of Rb + Cs atom pairs. Using a wavelength of 814 nm to trap Rb and 938 nm to trap Cs, we achieve loading probabilities of 0.508(6) for Rb and 0.547(6) for Cs using standard red-detuned molasses cooling. Loading the traps sequentially yields exactly one Rb and one Cs atom in 28.4(6)% of experimental runs. Using a combination of an acousto-optic deflector and a piezo-controlled mirror to control the relative position of the tweezers, we merge the two tweezers, retaining the atom pair with a probability of 0.9 9 ( − 0.02 ) ( + 0.01 ) . We use this capability to study hyperfine-state-dependent collisions of Rb and Cs in the combined tweezer and compare the measured two-body loss rates with coupled-channel quantum scattering calculations.
Abstract We report simultaneous Raman sideband cooling of a single 87Rb atom and a single 133Cs atom held in separate optical tweezers at 814 nm and 938 nm, respectively. Starting from outside the Lamb-Dicke regime, after 45 ms of cooling we measure probabilities to occupy the three-dimensional motional ground state of 0.8 6 − 0.04 + 0.03 for Rb and 0.9 5 − 0.04 + 0.03 for Cs. Our setup overlaps the Raman laser beams used to cool Rb and Cs, reducing hardware requirements by sharing equipment along the same beam path. The cooling protocol is scalable, and we demonstrate cooling of single Rb atoms in an array of four tweezers. After motional ground-state cooling, a 938 nm tweezer is translated to overlap with a 814 nm tweezer so that a single Rb and a single Cs atom can be transferred into a common 1064 nm trap. By minimising the heating during the merging and transfer, we prepare the atoms in the relative motional ground state with an efficiency of 0.8 1 − 0.08 + 0.08 . This is a crucial step towards the formation of single RbCs molecules confined in optical tweezer arrays.
We report on the realization of a platform for trapping and manipulating individual 88Sr atoms in optical tweezers. A first cooling stage based on a blue shielded magneto-optical trap (MOT) operating on the |1S0⟩→|1P1⟩ transition at 461 nm enables us to trap approximately 4 × 106 atoms at a temperature of 6.8 mK. Further cooling is achieved in a narrow-line red MOT using the |1S0⟩→|3P1⟩ intercombination transition at 689 nm, bringing 5 × 105 atoms down to 5μK and reaching a density of 4 × 1010 cm3. Atoms are then loaded into 813 nm tweezer arrays generated by crossed acousto-optic deflectors and tightly focused onto the atoms with a high-numerical-aperture objective. Through light-assisted collision processes we achieve the collisional blockade, which leads to single-atom occupancy with a probability of about 50%. The trapped atoms are detected via fluorescence imaging with a fidelity of 99.986(6)%, while maintaining a survival probability of 97(2)%. The release-and-recapture measurement provides a temperature of 12.92(5)μK for the atoms in the tweezers, and the ultra-high-vacuum environment ensures a vacuum lifetime higher than 7 min. These results demonstrate a robust alkaline-earth tweezer platform that combines efficient loading, cooling, and high-fidelity detection, providing the essential building blocks for scalable quantum simulation and quantum information processing with Sr atoms.
We demonstrate the formation of a single RbCs molecule during the merging of two optical tweezers, one containing a single Rb atom and the other a single Cs atom. Both atoms are initially predominantly in the motional ground states of their respective tweezers. We confirm molecule formation and establish the state of the molecule formed by measuring its binding energy. We find that the probability of molecule formation can be controlled by tuning the confinement of the traps during the merging process, in good agreement with coupled-channel calculations. We show that the conversion efficiency from atoms to molecules using this technique is comparable to magnetoassociation.
The optical tweezer experiment with neutral atoms is a focal topic in cold-atom physics due to its significant potential in quantum computing and simulation. Here we present the realization of a dual-species optical tweezer for both Rb and K atoms, taking a step towards creating a polar-molecule optical tweezer array. Initially, Rb and K atoms are collected using a dual magneto-optical trap and further cooled to $7\phantom{\rule{0.28em}{0ex}}\textmu{}\mathrm{K}$ for Rb and $10\phantom{\rule{0.28em}{0ex}}\textmu{}\mathrm{K}$ for K. By employing 850-nm tweezer beams, we demonstrate the ability to capture individual Rb or K atoms. The filling ratios of Rb and K can be finely adjusted by controlling the atomic densities of both species. Utilizing the postselection technique, we can create a deterministic array of two-species atoms, paving the way for future polar-molecule array formation.
We present a new approach to investigating Rydberg molecules by demonstrating the formation and characterization of individual Rb^{*}Cs Rydberg molecules using optical tweezers. By employing single-atom detection of Rb and Cs, we observe molecule formation via correlated loss of both species and study the formation dynamics with single-particle resolution. We control the interatomic distances by manipulating the relative wave function of atom pairs using the tweezer intensity, optimizing the coupling to molecular states and exploring the effect of the tweezer on these states. Additionally, we demonstrate molecule association with atoms trapped in separate tweezers, paving the way for state-selective assembly of polyatomic molecules. The observed binding energies, molecular alignment, and bond lengths are in good agreement with theory. Our approach is broadly applicable to Rydberg tweezer platforms, expanding the range of available molecular systems and enabling the integration of Rydberg molecules into existing quantum science platforms.
Qubits encoded in the electronic states of single atoms trapped in arrays of optical tweezers are a promising platform for a universal quantum computer. These qubits can be prepared in a well-defined quantum state, coherently manipulated using a nearresonant driving field, and their state detected with high fidelity. The most promising aspect of this platform is the large scalability, with arrays of up to 6100 qubits demonstrated[62].We present our progress in developing such a system with an array of single 85Rbatoms. We provide an overview of the experimental setup constructed for this purpose. Typically 50 atoms are loaded from a MOT into a 10×10 array of optical tweezers with sub-micrometer waists, with only a single atom present in a tweezer. The occupation of the tweezers is determined using a fluorescence image. We provide a characterisation of the trapping potentials experienced by the atoms. This characterisation is performed by measuring properties of the atoms in the tweezers, allowing for an in situ characterisation. In particular, the trap depth and trap frequencies were characterised. The temperature of the atoms after the initial fluorescence image was determined using the release and recapture technique [101] and the trapping lifetime of the atom was measured. With the ability to prepare, manipulate, and read out the electronic state of the atoms, an array of hyperfine qubits has been created. The qubits are encoded in the hyperfine clock states as |0⟩ := 52S1/2 |F = 2,mF = 0⟩ and |1⟩ := 52S1/2 |F = 3,mF = 0⟩. These long-lived first-order Zeeman shift insensitive states exhibit good coherence times, which we have characterized as T1=205 ± 3 ms , T2* = 2.01 ± 0.02 ms, andT2 echo = 67.1 ± 0.1 ms. State preparation is achieved by repetitions of optical and microwave pulses, to which the |0⟩ state is dark, allowing for population to accumulate in this state. The coherent evolution of the qubits have been performed using 3.035 GHz microwave radiation. The antenna used to produce this radiation is a home-built fullwave loop antenna. The antenna has allowed for addressing the qubits with Rabi frequencies up to Ω/2π ≈ 160 kHz. We have implemented the single-qubit Clifford gates using the global microwave drive. We determine using randomized benchmarking an166 Summary average gate fidelity of 0.99949(3), limited by Rabi frequency inhomogeneity over the array. To combat this fidelity limitation, we repeated the randomized benchmarking using the pulse length error robust SCROFULOUS pulses [135], which resulted in an increased gate fidelity of 0.999653(5). As a further extension of the capabilities of the system, we demonstrated a preliminary implementation of addressing a single atom int he array by applying a local Rz rotation to the selected qubit using a Stark shifting laser. The high level of control of the microwave radiation has allowed for an experimental verification of control noise-fidelity relations proposed by [115]. We have found good agreement between the experimentally measured fidelities and the proposed analytical relations developed using the stochastic Schrödinger equation. As a preliminary step towards implementing a two-qubit gate, we have performed coherent excitation of the |1⟩ state to the |r ⟩ :=602S1/2 |mJ = −1/2> Rydberg state using an off-resonant two-photon excitation. The low contrast of the Rabi oscillations on the |1⟩↔|r ⟩ transition was investigated using a simple Lindblad master equation based model. The largest contributors to the reduced contrast is SPAM error, intermediate state scattering and laser phase noise. Since Rydberg atoms interact via the van der Waals interaction, the spacing between atoms must be deterministically controlled. For this purpose, we have used an additional optical tweezer which can be dynamically moved using an acousto-optic deflector to rearrange the stochastically filled array into a desired configuration. By placing 2 atoms a distance ≈ 5 μm apart, we have demonstrated the p2 enhancement of the Rabi oscillation on the |1⟩↔|r ⟩ transition, a required first step towards implementing an entangling gate between the hyperfine qubits. To extend the temperature-limited T2* coherence time, we have implemented Λ-enhanced gray molasses cooling. We have opted to perform this cooling on the D2line as it is experimentally convenient to use this transition. Because using this transition for this purpose has not been reported in this isotope of Rb, we studied the efficacy of this cooling scheme under these circumstances. The reduced excited state hyperfine splitting of 85Rb compared to 87Rb has allowed for the study of the efficacy of this technique in the presence of additional transitions that may inhibit the cooling performance. Despite the challenges of the smaller hyperfine splitting, we have cooled the atoms to4.0±0.2 μK. This additional cooling is partially negated by the heating from the qubit state preparation procedure, but the additional cooling has allowed for the average T2*to be extended from ⟨T2*⟩ = 3.4 ± 0.1 ms to ⟨T2*⟩ = 5.3 ± 0.2 ms.