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arXiv:2104.01485 · Physical Review Letters

High Temperature Superconductivity in a Lightly Doped Quantum Spin Liquid

Hong‐Chen Jiang, Steven Allan Kivelson

Published Aug 27, 2021• 86 citations
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Abstract

We have performed density-matrix renormalization group studies of a square lattice $t\text{\ensuremath{-}}J$ model with small hole doping, $\ensuremath{\delta}\ensuremath{\ll}1$, on long four and six-leg cylinders. We include frustration in the form of a second-neighbor exchange coupling, ${J}_{2}={J}_{1}/2$, such that the undoped ($\ensuremath{\delta}=0$) ``parent'' state is a quantum spin liquid. In contrast to the relatively short range superconducting (SC) correlations that have been observed in recent studies of the six-leg cylinder in the absence of frustration, we find power-law SC correlations with a Luttinger exponent, ${K}_{\mathrm{SC}}\ensuremath{\approx}1$, consistent with a strongly diverging SC susceptibility, $\ensuremath{\chi}\ensuremath{\sim}{T}^{\ensuremath{-}(2\ensuremath{-}{K}_{\mathrm{SC}})}$ as the temperature $T\ensuremath{\rightarrow}0$. The spin-spin correlations---as in the undoped state---fall exponentially suggesting that the SC ``pairing'' correlations evolve smoothly from the insulating parent state.

DOI
10.1103/physrevlett.127.097002

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We have performed density-matrix renormalization group studies of a square lattice t\ensuremath-Jt\text{\ensuremath{-}}Jt\ensuremath-J model with small hole doping, \ensuremathδ\ensuremath≪1\ensuremath{\delta}\ensuremath{\ll}1\ensuremathδ\ensuremath≪1, on long four and six-leg cylinders. We include frustration in the form of a second-neighbor exchange coupling, J2=J1/2{J}_{2}={J}_{1}/2J2​=J1​/2, such that the undoped (\ensuremathδ=0\ensuremath{\delta}=0\ensuremathδ=0) parent'' state is a quantum spin liquid. In contrast to the relatively short range superconducting (SC) correlations that have been observed in recent studies of the six-leg cylinder in the absence of frustration, we find power-law SC correlations with a Luttinger exponent, ${K}_{\mathrm{SC}}\ensuremath{\approx}1$, consistent with a strongly diverging SC susceptibility, $\ensuremath{\chi}\ensuremath{\sim}{T}^{\ensuremath{-}(2\ensuremath{-}{K}_{\mathrm{SC}})}$ as the temperature $T\ensuremath{\rightarrow}0$. The spin-spin correlations---as in the undoped state---fall exponentially suggesting that the SC pairing'' correlations evolve smoothly from the insulating parent state.
Abstract Broad interest in quantum spin liquid (QSL) phases was triggered by the notion that they can be viewed as insulating phases with preexisting electron pairs, such that upon light doping they might automatically yield high temperature superconductivity. Yet despite intense experimental and numerical efforts, definitive evidence showing that doping QSLs leads to superconductivity has been lacking. We address the problem of a lightly doped QSL through a large-scale density-matrix renormalization group study of the t-J model on finite-circumference triangular cylinders with a small but nonzero concentration of doped holes. We provide direct evidences that doping QSL can naturally give rise to d-wave superconductivity. Specifically, we find power-law superconducting correlations with a Luttinger exponent, Ksc ≈ 1, which is consistent with a strongly diverging superconducting susceptibility, χsc ∼ T−(2 − Ksc){\chi }_{sc} \,\sim\, {T}^{-(2\,-\,{K}_{sc})}χsc​∼T−(2−Ksc​) χ s c ~ T − ( 2 − K s c ) as the temperature T → 0. The spin–spin correlations—as in the undoped QSL state—fall exponentially which suggests that the superconducting pair-pair correlations evolve smoothly from the insulating parent state.
Superconductivity in doped quantum paramagnets has been a subject of long theoretical inquiry. In this work, we report a density matrix renormalization group study of lightly doped $t\text{\ensuremath{-}}J$ models on the finite-width square lattice (doped hole densities $\ensuremath{\delta}=1/12$ and 1/8) with parameters for which previous studies have suggested that the undoped system in 2D is either a quantum spin liquid or a valence bond crystal. Our studies are performed on cylinders with width up to 8. Ground-state correlations are found to be nearly identical for the ``doped quantum spin liquid'' and ``doped valence bond crystal.'' Upon increasing the cylinder widths from 4 to 8, we observed a significant strengthening of the quasi-long-range superconducting correlations and a dramatic suppression of any ``competing'' charge density wave order. Extrapolating from the observed behavior of the width eight cylinders, we speculate that the system has a nodeless ddd-wave superconducting ground state in the 2D limit.
The authors employ the density-matrix renormalization group to investigate the doped Hubbard model on six-leg square cylinders. It uncovers a rich quantum phase diagram, intricately sensitive to next-nearest-neighbor electron hopping ($t\ensuremath{'}$). The positive-ttt\ensuremath{'} region shows a robust ddd-wave superconducting phase with intertwined superconducting and charge-density-wave orders. In contrast, the negative-ttt\ensuremath{'} side remains insulating, where doped holes form either long-range charge stripe order at small ttt\ensuremath{'} or a holon Wigner crystal with one doped hole per emergent unit cell and short-range spin correlations at larger ttt'.
We report a density-matrix renormalization group study of the lightly doped $t\text{\ensuremath{-}}J$ model on a four-leg cylinder with doped hole concentrations per site $\ensuremath{\delta}=5%\text{--}12.5%$. By keeping an unusually large number of states and long system sizes, we are able to accurately document the interplay between superconductivity, spin, and charge-density-wave orders. The long-distance behavior is consistent with that of a Luther-Emery liquid with a spin gap and power-law charge-density-wave and superconducting correlations. This is the widest $t\text{\ensuremath{-}}J$ or Hubbard system in which power-law superconducting correlations have been established.
We have performed large-scale density-matrix renormalization group studies of the lightly doped Hubbard model on the honeycomb lattice on long three- and four-leg cylinders. We find that the ground state of the system upon lightly doping is consistent with that of a superconducting state with coexisting quasi-long-range superconducting and charge density wave orders. Both the superconducting and charge density wave correlations decay as a power law at long distances with corresponding exponents Ksc<2{K}_{sc}<2Ksc​<2 and Kc<2{K}_{c}<2Kc​<2. On the contrary, the spin-spin and single-particle correlations decay exponentially, although with relatively long correlation lengths.
While the recent discovery of superconductivity in infinite-layer nickelates has drawn considerable attention, a common ingredient of the fundamental building blocks to describe their ground states has been lacking. A series of experimental and theoretical studies have suggested that an effective two-band Hubbard model with Ni 3dx2−y2d_{x^2-y^2}dx2−y2​ and rare-earth (RRR) 5ddd character may describe the low-energy physics. Here, we study the ground state properties of this two-band model on four-leg cylinders using the density-matrix renormalization group (DMRG). At half-filling, the ground state of the system is consistent with a Luttinger liquid, possessing quasi-long-range charge and spin correlations in the RRR layer, but short-range correlations in the Ni layer. At a hole doping concentration of δ=12.5%\delta=12.5\%δ=12.5%, the RRR layer is nearly empty and the ground state of the system is consistent with a Luther-Emery liquid, where we find power-law superconducting and charge density correlations in the Ni layer, but exponentially decaying spin correlations. The consistency of our results with experimental observations may help to reveal the microscopic mechanism for pairing in these nickelates and other unconventional superconductors.