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arXiv:2103.10421 · Nature

Realizing the symmetry-protected Haldane phase in Fermi–Hubbard ladders

Pimonpan Sompet, Sarah Hirthe, Dominik Bourgund, Thomas Chalopin, Julian Bibo, Joannis Koepsell, Petar Bojović, Ruben Verresen, Frank Pollmann, Guillaume Salomon, Christian Groß, Timon Hilker, Immanuel Bloch

Published Jun 1, 2022• 138 citations

Abstract

Abstract Topology in quantum many-body systems has profoundly changed our understanding of quantum phases of matter. The model that has played an instrumental role in elucidating these effects is the antiferromagnetic spin-1 Haldane chain 1,2 . Its ground state is a disordered state, with symmetry-protected fourfold-degenerate edge states due to fractional spin excitations. In the bulk, it is characterized by vanishing two-point spin correlations, gapped excitations and a characteristic non-local order parameter 3,4 . More recently it has been understood that the Haldane chain forms a specific example of a more general classification scheme of symmetry-protected topological phases of matter, which is based on ideas connected to quantum information and entanglement 5–7 . Here, we realize a finite-temperature version of such a topological Haldane phase with Fermi–Hubbard ladders in an ultracold-atom quantum simulator. We directly reveal both edge and bulk properties of the system through the use of single-site and particle-resolved measurements, as well as non-local correlation functions. Continuously changing the Hubbard interaction strength of the system enables us to investigate the robustness of the phase to charge (density) fluctuations far from the regime of the Heisenberg model, using a novel correlator.

DOI: 10.1038/s41586-022-04688-z

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Abstract Topology in quantum many-body systems has profoundly changed our understanding of quantum phases of matter. The model that has played an instrumental role in elucidating these effects is the antiferromagnetic spin-1 Haldane chain 1,2 . Its ground state is a disordered state, with symmetry-protected fourfold-degenerate edge states due to fractional spin excitations. In the bulk, it is characterized by vanishing two-point spin correlations, gapped excitations and a characteristic non-local order parameter 3,4 . More recently it has been understood that the Haldane chain forms a specific example of a more general classification scheme of symmetry-protected topological phases of matter, which is based on ideas connected to quantum information and entanglement 5–7 . Here, we realize a finite-temperature version of such a topological Haldane phase with Fermi–Hubbard ladders in an ultracold-atom quantum simulator. We directly reveal both edge and bulk properties of the system through the use of single-site and particle-resolved measurements, as well as non-local correlation functions. Continuously changing the Hubbard interaction strength of the system enables us to investigate the robustness of the phase to charge (density) fluctuations far from the regime of the Heisenberg model, using a novel correlator.

We systematically investigate the stability of the symmetry-protected topological (SPT) Haldane phase in spin- 1 2 Heisenberg and half-filled Hubbard ladders coupled by ferromagnetic Hund's interactions. Using the density-matrix renormalization group method, we analyze key signatures of the Haldane phase: long-range string order, finite spin gap, and characteristic entanglement spectrum degeneracies. In spin-only Heisenberg ladders, we find immediate onset and continuous strengthening of the Haldane phase with increasing Hund's coupling. In contrast, the inclusion of charge fluctuations in Hubbard ladders leads to a nontrivial stability regime, revealing a robust yet bounded region where SPT order persists despite significant charge fluctuations. We identify distinct boundaries separating a trivial insulating phase from the Haldane SPT phase, governed by both Coulomb repulsion and Hund's coupling. Our results highlight the subtle interplay of spin and charge degrees of freedom in correlated itinerant systems and establish essential criteria for observing Haldane physics experimentally in fermionic ladder materials.

The Haldane phase for antiferromagnetic spin-1 chains is a celebrated topological state of matter, featuring gapped excitations and fractional spin-1/2 edge states. Here, we provide numerical evidence that this phase can be realized with a Hubbard model at half filling, where each

s=1

spin is stored in a four-site fermionic structure. We find that the noninteracting limit of our proposed model describes a one-dimensional topological insulator, and we conjecture it to be adiabatically connected to the Haldane phase. Our work suggests a route to build spin-1 networks using Hubbard model quantum simulators.

The Haldane phase for antiferromagnetic spin-1 chains is a celebrated topological state of matter, featuring gapped excitations and fractional spin-1/2 edge states. Here we provide numerical evidence that this phase can be realized with a Hubbard model at half-filling, where each

s = 1

spin is stored in a four-site fermionic structure. We find that the noninteracting limit of our proposed parent model describes a one-dimensional topological insulator, adiabatically connected to the Haldane phase. Our work suggests a route to build spin-1 networks using Hubbard model quantum simulators.

The vast majority of symmetry-protected topological (SPT) states are difficult to detect, which often leads to their misidentification as ordinary or topologically trivial phases. In this work, we propose a general framework for detecting these hidden topological states. We distinguish the ordinary matter state from the topological phase by exploiting the boundary effects in space (via surface behaviors on engineered edge) and time (via strange correlators) according to the principle of bulk-edge correspondence. As a concrete example, we study the dimerized spin-1/2 Heisenberg model on a square lattice using quantum Monte Carlo simulations, focusing on its paramagnetic dimer phase and edge states. The dimer phase has been widely regarded as topologically trivial due to its gapped edge state on conventional edges. However, the model can also be viewed as two-dimensional antiferromagnetically (AF) coupled usual ladders, which suggests an SPT state adiabatically connected to the one-dimensional Haldane phase. We resolve this puzzle and demonstrate that the dimer phase is indeed a quasi-one-dimensional SPT state by measuring generalized strange correlators introduced in this work and by showing that the nontrivial gapless edge state on a zigzag edge is ferromagnetically ordered, resulting from effective ferromagnetic interactions between degenerate spinons liberated on each side of the cut. Furthermore, we show that the ordered edge state gives rise to an extraordinary surface critical behavior at the (2+1)-dimensional O(3) bulk critical points of the model, which contradicts theoretical predictions based on classical-quantum mapping. Overall, we establish a standard detection method for uncovering topological phases that masquerade as ordinary states of matter.

Ultracold neutral atoms in optical lattices have become a powerful platform for the simulation of complex quantum systems. With our quantum gas microscope, we measure snapshots of the quantum many-body wavefunction by fully resolving the position and spin of each atom. I will present the application of this method to two quantum phases: The Haldane spin-1 phase is the prototype of a symmetry-protected topological phase, whose spin order is hidden in conventional two-point correlation functions. On our images, we can evaluate the characteristic string-correlator of this state and directly see the associated edge states of the system. In an antiferromagnetic background, holes get dressed by a surrounding cloud of ferromagnetic correlations. We study these magnetic polarons, which are a building block of the intricate physics of cuprates, by mapping out the spatial structure of the spin environment of individual holes. Upon increased doping, we observe the transition from this unusual polaronic metal to a Fermi Liquid and provide quantum-simulated results of the Fermi-Hubbard model as a benchmark for different theoretical approaches.

Symmetry-protected topological phases have fundamentally changed our understanding of quantum matter. An archetypal example of such a quantum phase of matter is the Haldane phase, containing the spin-1 Heisenberg chain. The intrinsic quantum nature of such phases, however, often makes it challenging to study them using classical means. Here, we use trapped-ion qutrits to natively engineer spin-1 chains within the Haldane phase. Using a scalable deterministic procedure to prepare the Affleck-Kennedy-Lieb-Tasaki (AKLT) state within the Haldane phase, we study the topological features of this system on a qudit quantum processor. Notably, we verify the long-range string order of the state, despite its short-range correlations, and observe spin fractionalization of the physical spin-1 particles into effective qubits at the chain edges, a defining feature of this system. The native realization of Haldane physics on a qudit quantum processor and the scalable preparation procedures open the door to the efficient exploration of a wide range of systems beyond spin-1/2.