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arXiv:2103.04305 · Optics Express

Bright correlated twin-beam generation and radiation shaping in high-gain parametric down-conversion with anisotropy

Matvei Riabinin, Polina R. Sharapova, T. Meier

Published May 25, 2021• 0 citations
arXivHTMLPDF

Abstract

Uniaxial anisotropy in nonlinear birefringent crystals limits the efficiency of nonlinear optical interactions and breaks the spatial symmetry of light generated in the parametric down-conversion (PDC) process. Therefore, this effect is usually undesirable and must be compensated for. However, high gain may be used to overcome the destructive role of anisotropy in order to generate bright two-mode correlated twin-beams. In this work, we provide a rigorous theoretical description of the spatial properties of bright squeezed light in the presence of strong anisotropy. We investigate a single crystal and a system of two crystals with an air gap (corresponding to a nonlinear SU(1,1) interferometer) and demonstrate the generation of bright correlated twin-beams in such configurations at high gain due to anisotropy. We explore the mode structure of the generated light and show how anisotropy, together with crystal spacing, can be used for radiation shaping.

DOI
10.1364/oe.424977

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•Jun 8, 2017•0 citations
Uniaxial anisotropy in nonlinear birefringent crystals limits the efficiency of nonlinear optical interactions and breaks the spatial symmetry of light generated in the parametric down-conversion (PDC) process. Therefore, this effect is usually undesirable and must be compensated for. However, high gain may be used to overcome the destructive role of anisotropy in order to generate bright two-mode correlated twin-beams. In this work, we provide a rigorous theoretical description of the spatial properties of bright squeezed light in the presence of strong anisotropy. We investigate a single crystal and a system of two crystals with an air gap (corresponding to a nonlinear SU(1,1) interferometer) and demonstrate the generation of bright correlated twin-beams in such configurations at high gain due to anisotropy. We explore the mode structure of the generated light and show how anisotropy, together with crystal spacing, can be used for radiation shaping.
Parametric down-conversion (PDC) is mostly known in the low-gain (spontaneous) regime, in which the correlated photon pairs are produced. Spontaneous PDC (SPDC) plays a very important role for quantum optics as a variety of quantum states is produced via SPDC. In the high-gain case PDC leads to generation of bright states having up to hundreds mW mean power. With such states almost any nonlinear optical interaction or light-matter interaction becomes more efficient. Even being macroscopically bright, the produced states maintain nonclassical properties as, for example, the fluctuations of electric field quadratures are squeezed below the shot-noise level. The high-gain PDC could be used not only in the same applications as SPDC, it also can provide new ones. Apart from that the high-gain PDC has many remarkable spectral and statistical properties, which are in the focus of this work. The description starts from the PDC generation in normal and anomalous group velocity dispersion ranges. The spectrum and mode content of high-gain PDC is considered as well as their change with the parametric gain are demonstrated. Then, there are the interference effects emerging from the PDC correlations presented, namely the macroscopic analogue of the Hong-Ou-Mandel interference. In addition, it is shown how spatial and temporal walk-off matching could be used for the generation of giant narrowband twin beams. Finally, the statistical properties of high-gain PDC are reviewed as well as their use for multiphoton effects is demonstrated. Photon-number fluctuations of PDC are studied via normalized correlation functions and probability distributions. These fluctuations enhance the generation efficiency for multiphoton effects by orders of magnitude and lead to tremendously fluctuating light described by heavy-tailed photon-number probability distributions.
Abstract Light beams with orbital angular momentum (OAM) are convenient carriers of quantum information. They can also be used for imparting rotational motion to particles and providing high resolution in imaging. Due to the conservation of OAM in parametric down-conversion (PDC), signal and idler photons generated at low gain have perfectly anti-correlated OAM values. It is interesting to study the OAM properties of high-gain PDC, where the same OAM modes can be populated with large, but correlated, numbers of photons. Here we investigate the OAM spectrum of high-gain PDC and show that the OAM mode content can be controlled by varying the pump power and the configuration of the source. In our experiment, we use a source consisting of two nonlinear crystals separated by an air gap. We discuss the OAM properties of PDC radiation emitted by this source and suggest possible modifications.
We present a parametric down-conversion (PDC) process in a nonlinear ß-barium borate (BBO) crystal, driven by two non-collinear pump beams, obtained from a Mach-Zehnder type interferometer. We show the possibility to reproduce in a bulk crystal a phenomenology analogue to that previously observed in a PDC process inside a χ 2 2D nonlinear photonic crystal (NPC) [1] , [2] . Each pump mode generates a family of cones of parametric radiation collinear with its direction. The intersection zones define an ensemble of modes shared by the two pumps, indistinguishably populated by the photons generated by pump 1 or by pump 2. As in [1] , in the high-gain regime these two possibilities sum up coherently, leading to a local increase of the parametric gain. Indeed we observe an unusual far-field distribution of the down-converted light, in the form of three bright branches of hot-spots against a more diffuse background [3] .
We analyse a method to compensate for anisotropy effects in the spatial distribution of parametric down-conversion (PDC) radiation in bulk crystals. In this method, a single nonlinear crystal is replaced by two consecutive crystals with opposite transverse walk-off directions. We implement a simple numerical model to calculate the spatial distribution of intensity and correlations, as well as the Schmidt mode structure, with an account for the anisotropy. Experimental results are presented which prove the validity of both the model and the method.
The effect of the quantum properties of light on nonlinear processes has been well studied theoretically. It has been shown that the efficiency of n-photon nonlinear processes in many cases scales as the normalized n-th order correlation function. For light with high intensity correlation function, the efficiency of the n-th harmonic generation will be considerably higher than for coherent light. The experimental observation of this effect remained difficult until recently, because of the absence of bright sources with strong and fast intensity fluctuations. For the experimental demonstration of statistical effects in optical harmonic generation we use as a pump the radiation of high-gain parametric down conversion. Such light shows quantum properties (e.g. quadrature or two-mode squeezing) and has large number of photons in one mode. The normalized n-th order correlation function for this light is (2n - 1)!!, which makes it more attractive for nonlinear processes than both coherent and thermal light. For the generation of optical harmonics we used broadband parametric down conversion around frequency-degeneracy (1600 nm) produced in 1cm BBO crystal from Ti:Sapphire laser (800 nm, 1.6ps, 5kHz, 3W mean intensity). Due to spectral filtering and post-selection technique we could vary the statistics of light from coherent to super-bunched, which allowed us to demonstrate the efficiency enhancement for second-, third-, and fourth-harmonic generation. The obtained experimental results show a good agreement with the theory.