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arXiv:2101.11176 · Chinese Physics B

Observation of photon recoil effects in single-beam absorption spectroscopy with an ultracold strontium gas

Fachao Hu, Canzhu Tan, Yuhai Jiang, Matthias Weidemüller, Bing Zhu

Published Sep 8, 2021• 4 citations
arXivHTMLPDF

Abstract

We report on observing photon recoil effects in the absorption of a single monochromatic light at 689 nm through an ultracold 88Sr gas, where the recoil frequency is comparable to natural linewidth of the narrow-line transition 5s2 1S0–5s5p 3P1 in strontium. In the regime of high-saturation, the absorption profile becomes asymmetric due to the photon-recoil shift, which is of the same order as the natural linewidth. The lineshape is described by an extension of the optical Bloch equations including the momentum transfers to atoms during emission and absorption of photons. Our work reveals the photon recoil effects in a simplest single-beam absorption setting, which is of significant relevance to other applications such as saturation spectroscopy, Ramsey interferometry, and absorption imaging.

DOI
10.1088/1674-1056/ac2486

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arXiv:2004.02959•Physical Review A•Jun 9, 2022•4 citations
We report on observing photon recoil effects in the absorption of a single monochromatic light at 689 nm through an ultracold 88Sr gas, where the recoil frequency is comparable to natural linewidth of the narrow-line transition 5s2 1S0–5s5p 3P1 in strontium. In the regime of high-saturation, the absorption profile becomes asymmetric due to the photon-recoil shift, which is of the same order as the natural linewidth. The lineshape is described by an extension of the optical Bloch equations including the momentum transfers to atoms during emission and absorption of photons. Our work reveals the photon recoil effects in a simplest single-beam absorption setting, which is of significant relevance to other applications such as saturation spectroscopy, Ramsey interferometry, and absorption imaging.
We analyse the spectrum on the narrow-line transition \narrow at 689 nm in an ultracold gas of 88^{88}88Sr via absorption imaging. In the low saturation regime, the Doppler effect dominates in the observed spectrum giving rise to a symmetric Voigt profile. The atomic temperature and atom number can accurately be deduced from these low-saturation imaging data. At high saturation, the absorption profile becomes asymmetric due to the photon-recoil shift, which is of the same order as the natural line width. The line shape can be described by an extension of the optical Bloch equations including the photon recoil. A lensing effect of the atomic cloud induced by the dispersion of the atoms is also observed at higher atomic densities in both the low and strong saturation regimes.
We present an extensive study of the unique thermal and mechanical dynamics for narrow-line cooling on the 1S0-3P1 88Sr transition. For negative detuning, trap dynamics reveal a transition from the semiclassical regime to the photon-recoil-dominated quantum regime, yielding an absolute minima in the equilibrium temperature below the single-photon-recoil limit. For positive detuning, the cloud divides into discrete momentum packets whose alignment mimics lattice points on a face-centered-cubic crystal. This novel behavior arises from velocity selection and "positive feedback" acceleration due to a finite number of photon recoils. Cooling is also achieved with blue-detuned light around a velocity where gravity balances the radiative force.
A systematic shift of the photon recoil momentum due to the index of refraction of a dilute gas of atoms has been observed. The recoil frequency was determined with a two-pulse light grating interferometer using near-resonant laser light. The results show that the recoil momentum of atoms caused by the absorption of a photon is n variant Planck's k, where n is the index of refraction of the gas and k is the vacuum wave vector of the photon. This systematic effect must be accounted for in high-precision atom interferometry with light gratings.
We report on our progress toward the realization of an optical frequency standard referenced to strontium intercombination lines. While first frequency measurement of the weakly allowed 1S 0- 3P 1 transition was done with saturation spectroscopy on a thermal beam, we are preparing the experimental setup for high resolution spectroscopy on ultracold atoms of the doubly forbidden 1S 0- 3P 0 line. Our current setup allows the capture more than 10 7 atoms at 1 μK in 500 ms in two stages of magneto-optical trapping. We also demonstrated the dipole trapping of ultracold strontium isotopes for accurate spectroscopy and collisional measurements. A semiconductor laser source at 698 nm has already been locked to a pre-stabilization cavity obtaining a fast linewidth of less than 1 kHz. Second stage stabilization of the clock laser to ultra-high finesse cavity is in development. Recent measurement of elastic and inelastic cross-sections of the two most abundant 88Sr and 86Sr isotopes are also presented.
We observe the fluorescence and the saturated fluorescence spectra of (5s2)1S0(5s5p)3P1 intercombination transition of thermal strontium atomic beam. Experimental investigation of 88Sr(5s2)1S0(5s5p)3P1 intercombination transition is performed on the different experimental conditions. Our study indicates that experimental parameters affect spectra largely, including temperature, intensity of laser and scanning frequency of laser. Intensity of spectrum is reciprocal of scanning frequency of laser due to long lifetime of (5s5p)3P1 state of Sr atom. Owing to Doppler broadening, transit broadening and other experimental factors, the linewidth of (5s2)1S0(5s5p)3P1 fluorescence spectrum is far more than its natural linewidth and proportional scanning frequency of laser.
We reflect on the prospect of exploiting the recoil associated with absorption and emission of photons to perform spectroscopy of a single molecular ion. For this recoil to be detectable, the molecular ion is sympathetically cooled by a laser-cooled atomic ion to near their common quantum-mechanical ground state within a trapping potential. More specifically, we present a general framework for simulating the expected photon recoil spectra in regimes where either the natural transition linewidth ${\mathrm{\ensuremath{\Gamma}}}_{t}$ of the molecular ion or the spectral width ${\mathrm{\ensuremath{\Gamma}}}_{L}$ of the exciting light source exceeds the motional frequencies of the two-ion system. To exemplify the framework, we present two complementary cases: spectroscopy of the broad $3\mathrm{s} ^{2}\mathrm{S}_{1/2}\ensuremath{-}3\mathrm{p} ^{2}\mathrm{P}_{3/2}$ electronic transition (${\mathrm{\ensuremath{\Gamma}}}_{t}/2\ensuremath{\pi}=41.8\phantom{\rule{0.16em}{0ex}}\mathrm{M}\mathrm{Hz}$) of a single 24Mg+^{24}\mathrm{Mg}^{+}24Mg+ ion at $\ensuremath{\lambda}=279.6$ nm by a narrow laser source $({\mathrm{\ensuremath{\Gamma}}}_{L}/2\ensuremath{\pi}\ensuremath{\lesssim}1\phantom{\rule{0.16em}{0ex}}\mathrm{MHz})$ and mid-infrared vibrational spectroscopy of the very narrow $|v=0,J=1\ensuremath{\rangle}\ensuremath{-}|{v}^{\ensuremath{'}}=1,{J}^{\ensuremath{'}}=0\ensuremath{\rangle}$ transition $({\mathrm{\ensuremath{\Gamma}}}_{t}/2\ensuremath{\pi}=2.50\phantom{\rule{0.16em}{0ex}}\mathrm{Hz})$ at $\ensuremath{\lambda}=6.17\phantom{\rule{0.16em}{0ex}}\ensuremath{\mu}\mathrm{m}$ in the $^{1}\mathrm{\ensuremath{\Sigma}}^{+}$ electronic ground state of 24MgH+^{24}\mathrm{MgH}^{+}24MgH+ by a broadband laser source $({\mathrm{\ensuremath{\Gamma}}}_{L}/2\ensuremath{\pi}\ensuremath{\gtrsim}50\phantom{\rule{0.16em}{0ex}}\mathrm{MHz})$. The atomic ion 24Mg+^{24}\mathrm{Mg}^{+}24Mg+ has been picked to introduce a simple system to make comparisons with experimental results while still capturing most of the physics involved in electronic excitations of molecular ions.