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arXiv:2012.15120 · Physical Review A

Coherent control techniques for two-state quantum systems: A comparative study

Boyan T. Torosov, Bruce W. Shore, Nikolay V. Vitanov

Published Mar 17, 2021• 30 citations
arXivHTMLPDF

Abstract

We evaluate various sources of errors that occur when attempting to produce a specified coherent change of a two-state quantum system using six popular coherent control techniques: resonant excitation, adiabatic following, composite adiabatic passage, universal composite pulses, shortcut to adiabaticity, and single-shot shaped pulses. As error sources, we consider spatial intensity distribution, transit time variation, inhomogeneous broadening, Doppler broadening, unwanted chirp, and shape errors, as well as errors generated by counter-rotating terms. For the various error types, different techniques emerge as the best performers, but overall we find that universal composite pulses perform most consistently and are most resilient to errors compared to all other procedures.

DOI
10.1103/physreva.103.033110

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We evaluate various sources of errors that occur when attempting to produce a specified coherent change of a two-state quantum system using six popular coherent control techniques: resonant excitation, adiabatic following, composite adiabatic passage, universal composite pulses, shortcut to adiabaticity, and single-shot shaped pulses. As error sources, we consider spatial intensity distribution, transit time variation, inhomogeneous broadening, Doppler broadening, unwanted chirp, and shape errors, as well as errors generated by counter-rotating terms. For the various error types, different techniques emerge as the best performers, but overall we find that universal composite pulses perform most consistently and are most resilient to errors compared to all other procedures.
We introduce a high-fidelity technique for coherent control of three-state quantum systems, which combines two popular control tools---stimulated Raman adiabatic passage (STIRAP) and composite pulses. By using composite sequences of pairs of partly delayed pulses with appropriate phases, the nonadiabatic transitions, which prevent STIRAP from reaching unit fidelity, can be canceled to an arbitrary order by destructive interference, and therefore, the technique can be made arbitrarily accurate. The composite phases are given by simple analytic formulas, and they are universal for they do not depend on the specific pulse shapes, the pulse delay, and the pulse areas.
Composite pulses---sequences of pulses with well-defined relative phases---are an efficient, robust, and flexible technique for coherent control of quantum systems. Composite sequences can compensate for a variety of experimental errors in the driving field (e.g., in the pulse amplitude, duration, detuning, chirp, etc.) or in the quantum system and its environment (e.g., inhomogeneous broadening, stray electric or magnetic fields, unwanted couplings, etc.). The control parameters are the relative phases between the constituent pulses in the composite sequence, an accurate control over which is required in all composite sequences reported hitherto. In this paper, we introduce two types of composite pulse sequences which, in addition to error compensation in the basic experimental parameters, compensate for systematic errors in the composite phases. In the first type of such composite sequences, which compensate for pulse area errors, relative phase errors of over 10% can be tolerated with reasonably short sequences while maintaining the fidelity above the 99.99% quantum computing benchmark. In the second type of composite sequences, which compensate for simultaneous pulse area and detuning errors, relative phase errors of over 5% can be compensated.
Here, we focus on using composite pulses to realize high-robustness and high-fidelity coherent control in three-level quantum systems. We design the dynamic parameters (Rabi frequency and detuning) for three-level Hamiltonians for high-fidelity quantum state control using five well-known coherent control techniques including a composite adiabatic passage (CAP). Furthermore, we compare their performance against the Rabi frequency and systematic errors, and accordingly show that the CAP is the most robust against them. It features a broad range of high efficiencies above 99.9%. Thus, it provides an accurate approach for manipulating the evolution of quantum states in three-level quantum systems.
Population inversion from an initial quantum state to a desired quantum state represents an exciting new frontier for quantum manipulation; that frontier is endowed with a strong interdisciplinary character and connections to other scientific fields, including atomic, molecular, and optical physics, as well as in solid-state devices, for fundamental studies, nuclear magnetic resonance and other spectroscopic techniques, metrology, interferometry, optical control of chemical reactions or quantum-information applications. Two-level systems are ubiquitous in these areas, and the driving of a population inversion is an important operation. So far various schemes for population transfer to a target state from an initial state have been proposed in theory and implemented in experiment. To be useful, such methods must, of course, be reliable, fast, and robust. Most literatures on two-level models investigated population inversion, which could be modelled by infinite-time processes. In this paper, by using a composite adiabatic passage (CAP) technique—in which the single pulse driving the quantum transition is replaced by a sequence of pulses with well-defined control phases, we investigate the population inversion problem of two-level quantum system with a finite duration. We take a sinusoidally varying pulse model that continuously vanishes at the beginning and the end of the finite duration as an example. The high-fidelity population inversion of the two-level system with finite duration is achieved. We discuss the effects of both coupling strength and detuning strength on the transition probability. It is found that this protocol could suppress the oscillations in the transition probability and reduce the admissible error bellow the 10 -4 quantum computation benchmark. The fidelity can arrive at 1, even with simple three- and five-composite pulse sequences. The protocol combines the advantages of adiabatic passage and composite pulses techniques. By choosing the composite phases appropriately, a high-fidelity, fast, stable and extremely robust complete population inversion is achieved for the finite-time two-level model. The values of the composite phases are universal for they do not depend on the pulse shapes and the chirp as long as the latter satisfy the symmetry property. Furthermore, the classical Hamiltonian is applied to describe the dynamic properties of the quantum system and further verify the effectiveness and feasibility of the proposed CAP technique. The results we present here are general and in principle apply to any two- and multi-level quantum systems. The accuracy of the CAP technique and its robustness against parameter variations make the protocol suitable for ultrahigh-fidelity quantum manipulation. We believe that the protocol can be widely used in many different areas of science, ranging from the quantum information, the quantum chemical, and the quantum optics to the ultracold atomic and molecular physics.
We derive composite pulse sequences that achieve high-fidelity excitation of two-state systems in an optically dense, inhomogeneously broadened ensemble. The composite pulses are resistant to distortions due to the backaction of the medium they propagate in and are able to create high-fidelity inversion to optical depths $\ensuremath{\alpha}z>10$. They function well with smooth pulse shapes used for coherent control of optical atomic transitions in quantum computation and communication. They are an intermediary solution between single $\ensuremath{\pi}$-pulse excitation schemes and adiabatic passage schemes, being far more error tolerant than the former but still considerably faster than the latter.