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arXiv:1306.0699 · Physical Review A

Composite stimulated Raman adiabatic passage

Boyan T. Torosov, Nikolay V. Vitanov

Published Apr 17, 2013• 58 citations
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Abstract

We introduce a high-fidelity technique for coherent control of three-state quantum systems, which combines two popular control tools---stimulated Raman adiabatic passage (STIRAP) and composite pulses. By using composite sequences of pairs of partly delayed pulses with appropriate phases, the nonadiabatic transitions, which prevent STIRAP from reaching unit fidelity, can be canceled to an arbitrary order by destructive interference, and therefore, the technique can be made arbitrarily accurate. The composite phases are given by simple analytic formulas, and they are universal for they do not depend on the specific pulse shapes, the pulse delay, and the pulse areas.

DOI
10.1103/physreva.87.043418

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We introduce a high-fidelity technique for coherent control of three-state quantum systems, which combines two popular control tools---stimulated Raman adiabatic passage (STIRAP) and composite pulses. By using composite sequences of pairs of partly delayed pulses with appropriate phases, the nonadiabatic transitions, which prevent STIRAP from reaching unit fidelity, can be canceled to an arbitrary order by destructive interference, and therefore, the technique can be made arbitrarily accurate. The composite phases are given by simple analytic formulas, and they are universal for they do not depend on the specific pulse shapes, the pulse delay, and the pulse areas.
We present a method for optimization of the technique of adiabatic passage between two quantum states by composite sequences of frequency-chirped pulses with specific relative phases: composite adiabatic passage (CAP). By choosing the composite phases appropriately the nonadiabatic losses can be canceled to any desired order with sufficiently long sequences, regardless of the nonadiabatic coupling. The values of the composite phases are universal for they do not depend on the pulse shapes and the chirp. The accuracy of the CAP technique and its robustness against parameter variations make CAP suitable for high-fidelity quantum information processing.
Accurate control of a quantum system is a fundamental requirement in many areas of modern science ranging from quantum information processing to high-precision measurements. A significantly important goal in quantum control is to prepare a desired state as fast as possible with sufficiently high fidelity allowed by available resources and experimental constraints. Stimulated Raman adiabatic passage (STIRAP) is a robust way to realize high-fidelity state transfer but it requires a sufficiently long operation time to satisfy the adiabatic criteria. We here theoretically propose and then experimentally demonstrate a shortcut-to-adiabatic protocol to speed up the STIRAP. By modifying the shapes of the Raman pulses, we experimentally realize a fast and high-fidelity stimulated Raman shortcut-to-adiabatic passage that is robust against control parameter variations. The all-optical, robust, and fast protocol demonstrated here provides an efficient and practical way to control quantum systems.
Accurate control of a quantum system is a fundamental requirement in many areas of modern science ranging from quantum information processing to high-precision measurements. A significantly important goal in quantum control is preparing a desired state as fast as possible, with sufficiently high fidelity allowed by available resources and experimental constraints. Stimulated Raman adiabatic passage (STIRAP) is a robust way to realize high-fidelity state transfer but it requires a sufficiently long operation time to satisfy the adiabatic criteria. Here we theoretically propose and then experimentally demonstrate a shortcut-to-adiabatic protocol to speed-up the STIRAP. By modifying the shapes of the Raman pulses, we experimentally realize a fast and high-fidelity stimulated Raman shortcut-to-adiabatic passage that is robust against control parameter variations. The all-optical, robust and fast protocol demonstrated here provides an efficient and practical way to control quantum systems.
Multistate stimulated Raman adiabatic passage (STIRAP) is a process which allows for adiabatic population transfer between the two ends of a chainwise-connected quantum system. The process requires large temporal areas of the driving pulsed fields (pump and Stokes) in order to suppress the nonadiabatic couplings and thereby to make adiabatic evolution possible. To this end, in the present paper a variation of multistate STIRAP, which accelerates and improves the population transfer, is presented. In addition to the usual pump and Stokes fields it uses shortcut fields applied between the states, which form the dark state of the system. The shortcuts cancel the couplings between the dark state and the other adiabatic states thereby resulting (in the ideal case) in a unit transition probability between the two end states of the chain. Specific examples of five-state systems formed of the magnetic sublevels of the transitions between two degenerate levels with angular momenta Jg=2{J}_{g}=2Jg​=2 (of ground or lower level) and Je=1{J}_{e}=1Je​=1 or Je=2{J}_{e}=2Je​=2 (of excited or upper level) are considered in detail, for which the shortcut fields are derived analytically. The proposed method is simpler than the usual ``shortcuts to adiabaticity'' recipe, which prescribes shortcut fields between all states of the system, while the present proposal uses shortcut fields between the sublevels forming the dark state only. The results are of potential interest in applications where high-fidelity quantum control is essential, e.g., quantum information, atom optics, formation of ultracold molecules, cavity QED, etc.
Coherent manipulation of quantum states is of crucial importance in accurate control of a quantum system. A fundamental goal is coherently transferring the population of a desired state with near-unit fidelity. For this purpose, we theoretically demonstrate a novel coherent double-stimulated Raman adiabatic passage (STIRAP) in a three-level Λ-type system for realizing the switch of unequal initial preparations on two ground states. This operation uses a single optical pulse sequence accomplishing both bright-STIRAP and dark-STIRAP processes, in which the intermediate-level detuning and the pulse delay must be given an optimal adjustment. Besides, owing to the imperfection of double-STIRAP transition, the sensitivity of the switch fidelity with respect to the spontaneous loss from the intermediate state, to the pulse amplitude and to the population difference, is also discussed. This work suggests a simple and experimentally feasible all-optical approach to switch a superposition quantum state, serving as one-step closer to the goal of coherent manipulation of quantum systems.
We propose a non-Hermitian generalization of stimulated Raman adiabatic passage (STIRAP), which allows one to increase speed and fidelity of the adiabatic passage. This is done by adding balanced imaginary (gain and loss) terms in the diagonal (bare energy) terms of the Hamiltonian and choosing them such that they cancel exactly the nonadiabatic couplings, providing in this way an effective shortcut to adiabaticity. Remarkably, for a STIRAP using delayed Gaussian-shaped pulses in the counterintuitive scheme the imaginary terms of the Hamiltonian turn out to be time independent. A possible physical realization of non-Hermitian STIRAP, based on light transfer in three evanescently coupled optical waveguides, is proposed.