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arXiv:2012.11591 · Physical Review A

Dynamical formation of polarons in a Bose-Einstein condensate: A variational approach

Luis A. Peña Ardila

Published Mar 23, 2021• 20 citations
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Abstract

We investigate the nonequilibrium dynamics of an impurity coupled to a Bose-Einstein condensate, systematically compared with recent experimental results [M. G. Skou et al., Nat. Phys. (2021)]. The dynamics of the impurity is tracked down by using a time-dependent variational coherent ansatz. For weak coupling between the impurity and the bath, analytical expressions for the time-dependent contrast are derived, matching quite well with previous findings obtained within a master equation approach. For strong coupling instead, the variational ansatz provides a good quantitative description of the polaron dynamics, in particular, in signaling the transition from the few- to the many-body correlated regime where polarons are expected to form.

DOI
10.1103/physreva.103.033323

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We investigate the nonequilibrium dynamics of an impurity coupled to a Bose-Einstein condensate, systematically compared with recent experimental results [M. G. Skou et al., Nat. Phys. (2021)]. The dynamics of the impurity is tracked down by using a time-dependent variational coherent ansatz. For weak coupling between the impurity and the bath, analytical expressions for the time-dependent contrast are derived, matching quite well with previous findings obtained within a master equation approach. For strong coupling instead, the variational ansatz provides a good quantitative description of the polaron dynamics, in particular, in signaling the transition from the few- to the many-body correlated regime where polarons are expected to form.
We study the quantum dynamics of a single impurity following its sudden immersion into a Bose–Einstein condensate. The ensuing formation of the Bose polaron in this general setting can be seen as impurity decoherence driven by the condensate, which we describe within a master equation approach. We derive rigorous analytical results for this decoherence dynamics, and thereby reveal distinct stages of its evolution from a universal stretched exponential initial relaxation to the final approach to equilibrium. The associated polaron formation time exhibits a strong dependence on the impurity speed and is found to undergo a critical slowdown around the speed of sound of the condensate. This rich non-equilibrium behavior of quantum impurities is of direct relevance to recent cold atom experiments, in which Bose polarons are created by a sudden quench of the impurity-bath interaction.
We study the quantum dynamics of a single impurity following its sudden immersion into a Bose-Einstein condensate. The formation of the Bose polaron after such a quench stems from decoherence of the impurity, driven by collisions with the condensate. Using a master equation approach, we derive rigorous analytical results for the decoherence dynamics of the impurity, which reveals different stages of its evolution from a universal non-exponential initial relaxation to the final approach of the equilibrium state of the Bose polaron. The associated polaron formation time exhibit a strong dependence of the impurity momentum and is found to undergo a critical slowdown around the Landau critical velocity of the condensate. The rich non-equilibrium behavior of quantum impurities in a Bose gas revealed in this work is of direct relevance to recent cold-atom experiments, in which Bose polarons are created by a sudden quench of the impurity-bath interaction.
An impurity particle interacting with a Bose-Einstein condensate (BEC) leads to the formation of a quasiparticle known as the Bose polaron. We investigate the properties of the two-dimensional Bose polaron, applying a variational ansatz that contains up to three Bogoliubov excitations of the BEC. Similar to its three-dimensional counterpart, we observe the existence of two quasiparticle branches, namely, the attractive and the repulsive polarons, at different coupling strengths. We find that their energies agree well with recent quantum Monte Carlo calculations. In particular, we observe that the inclusion of three excitations is crucial to capture the attractive polaron energy towards the regime of strong attraction, where the quasiparticle properties are dominated by few-body correlations. We also calculate the attractive polaron effective mass and residue, where we find significant differences between considering a weakly interacting Bose medium and taking the noninteracting limit, signaling enhanced impurity dressing by excitations in the latter case. By contrast, the spectral weight of the metastable repulsive polaron is largely insensitive to the interactions in the BEC and the number of Bogoliubov excitations. Our model may be experimentally realized in dilute atomic vapors and atomically thin semiconductors.
Important properties of complex quantum many-body systems and their phase diagrams can often already be inferred from the impurity limit. The Bose polaron problem describing an impurity atom immersed in a Bose-Einstein condensate is a paradigmatic example. The interplay between the impurity-mediated attraction between the bosons and their intrinsic repulsion makes this model rich and interesting, but also complex to describe theoretically. To tackle this challenge, we develop a quantum chemistry-inspired computational technique and compare two variational methods that fully include both the boson-impurity and interboson interactions. We find one regime where the impurity-mediated interactions overcome the repulsion between the bosons, so that a sweep of the boson-impurity interaction strength leads to an instability of the polaron due to the formation of many-body clusters. If instead the interboson interactions dominate, the impurity will experience a crossover from a polaron into a few-body bound state. We achieve a unified understanding incorporating both of these regimes and show that they are experimentally accessible. Moreover, we develop an analytical model that allows us to interpret these phenomena in the Landau framework of phase transitions, revealing a deep connection of the Bose polaron model to both few- and many-body physics.
Advancing our understanding of non-equilibrium phenomena in quantum many-body systems remains one of the greatest challenges in physics. Here we report on the experimental observation of a paradigmatic many-body problem, namely the non-equilibrium dynamics of a quantum impurity immersed in a bosonic environment1,2. We use an interferometric technique to prepare coherent superposition states of atoms in a Bose–Einstein condensate with a small impurity-state component, and monitor the evolution of such quantum superpositions into polaronic quasiparticles. These results offer a systematic picture of polaron formation3–7 from weak to strong impurity interactions. They reveal three distinct regimes of evolution with dynamical transitions that provide a link between few-body processes and many-body dynamics. Our measurements reveal universal dynamical behaviour in interacting many-body systems and demonstrate new pathways to study non-equilibrium quantum phenomena. Quantum impurities immersed in a bosonic environment can evolve into polaronic quasiparticles, so-called polarons. Interferometric measurement reveals this transition, which involves three different regimes dominated by few-body and many-body dynamics.
When a mobile impurity interacts with a surrounding bath of bosons, it forms a polaron. Numerous methods have been developed to calculate how the energy and the effective mass of the polaron are renormalized by the medium for equilibrium situations. Here, we address the much less studied nonequilibrium regime and investigate how polarons form dynamically in time. To this end, we develop a time-dependent renormalization-group approach which allows calculations of all dynamical properties of the system and takes into account the effects of quantum fluctuations in the polaron cloud. We apply this method to calculate trajectories of polarons following a sudden quench of the impurity-boson interaction strength, revealing how the polaronic cloud around the impurity forms in time. Such trajectories provide additional information about the polaron's properties which are challenging to extract directly from the spectral function measured experimentally using ultracold atoms. At strong couplings, our calculations predict the appearance of trajectories where the impurity wavers back at intermediate times as a result of quantum fluctuations. Our method is applicable to a broader class of nonequilibrium problems. As a check, we also apply it to calculate the spectral function and find good agreement with experimental results. At very strong couplings, we predict that quantum fluctuations lead to the appearance of a dark continuum with strongly suppressed spectral weight at low energies. While our calculations start from an effective Fr\"ohlich Hamiltonian describing impurities in a three-dimensional Bose-Einstein condensate, we also calculate the effects of additional terms in the Hamiltonian beyond the Fr\"ohlich paradigm. We demonstrate that the main effect of these additional terms on the attractive side of a Feshbach resonance is to renormalize the coupling strength of the effective Fr\"ohlich model.