Rutherford scattering is usually described by treating the projectile either classically or as quantum mechanical plane waves. Here we treat them as wave packets and study their head-on collisions with the stationary target nuclei. We simulate the quantum dynamics of this one-dimensional system and study deviations of the average quantum solution from the classical one. These deviations are traced back to the convexity properties of Coulomb potential. Finally, we sketch how these theoretical findings could be tested in experiments looking for the onset of nuclear reactions.
Rutherford scattering is usually described by treating the projectile either classically or as quantum mechanical plane waves. Here we treat them as wave packets and study their head-on collisions with the stationary target nuclei. We simulate the quantum dynamics of this one-dimensional system and study deviations of the average quantum solution from the classical one. These deviations are traced back to the convexity properties of Coulomb potential. Finally, we sketch how these theoretical findings could be tested in experiments looking for the onset of nuclear reactions.
Figure 1.1 represents schematically a typical scattering experiment, in fact this is the sketch of E. Rutherford experiment in 1910 [ 1 ]. Projectiles (here, α -particles) from a source go through a collimator and collide with a target (gold foil in Rutherford’s experiment). Some projectiles are scattered by the target and reach the detector (here, a fluorescent screen). Rutherford expected them to go straight through with perhaps a minor deflection. Most did go straight through, but to his surprise some particles bounced directly off the gold sheet! What did this mean? Rutherford hypothesized that the positive alpha particles had hit a concentrated mass of positive particles, which he termed the nucleus. We shall describe the Rutherford scattering theoretically later in this chapter.
Non-relativistic quantum scattering theory informs our broad understanding of nuclear collision processes. However, detailed theoretical insights into the dynamics of fusion, whereby the colliding nuclei form a compound nucleus, remain elusive with conventional approaches. Fundamentally, understanding the complex dissipative processes inherent to compound nucleus formation and when they occur during the collision remains challenging. This, for example, prevents a consistent description of heavy-ion fusion over a wide range of collision energies and hinders searches for new super-heavy elements. To understand these dynamics, we need time-dependent approaches to nuclear collisions. In this thesis, a non-relativistic, time-dependent wave packet theory for potential scattering of charged quantum particles (such as nuclei) has been developed. It formally extends the application of Tannor and Weeks's (1993) formulation of the scattering matrix theory to systems containing the long-range Coulomb potential, by utilising Dollard's (1964) Møller operators. Using the asymptotic localisation of wave packets, analytical theorems have been formulated that allow convenient numerical application of this method. Numerical tests illustrating the theory mark the first rigorous application of this method in nuclear physics. Further insights are gained through a novel analysis of the wave packet time-correlation function (which underlies the theory) to understand how different dynamical processes, such as the formation of long-lived, quasi-bound states, during scattering contribute to the scattering matrix. This provides guidance on using the time-correlation function to obtain fusion observables, along with the associated challenges. Furthermore, this analysis showed that time-correlation functions can be obtained from static calculations, opening numerous new possibilities for studying the dynamics of nuclear reactions, in general, using this approach. This work opens new avenues for studying the dynamics of compound nucleus formation and other dissipative processes in nuclear reactions.
A previous paper [J. Phys. B: At. Mol. Opt. Phys. 50, 215302 (2017)] showed that partial wave analysis becomes applicable to nonrelativistic Coulomb scattering if wavepackets are used. The scattering geometry considered was special: that of a head-on collision between the wavepacket and the centre of the potential. Our results predicted, in this case, a shadow zone of low probability for small angles around the forward direction for the description of alpha scattering from a gold foil. In this paper we generalize the results to the case of a nonzero impact parameter, a displacement of the wavepacket centre perpendicular to the average momentum direction. We predict a large flux in the forward direction from events with large impact parameters. We find a significant probability of scattering into the deviation region for impact parameters of order the spatial width of the wavepacket. Averaging over impact parameters produces predictions in excellent agreement with the Rutherford formula down to lower angles than for the zero impact parameter prediction. We consider issues that would arise in a real experiment and discuss the possibility of measuring a deviation from the Rutherford formula.
Introduction We now move to considering the dynamics of a system of nuclei and electrons. Of course, both electrons and nuclei are subject to the laws of quantum mechanics, but since nuclei are 2000 to 200,000 times heavier than electrons, we expect that classical mechanics will be a much better approximation for the motion of nuclei than for the motion of electrons. This means that we expect a level of approximation to be valid, where some of the degrees of freedom (d.o.f.) of a system behave essentially classically and others behave essentially quantum-mechanically. The system then is of a mixed quantum/classical nature. Most often the quantum subsystem consists of system of electrons in a dynamical field of classical nuclei, but the quantum subsystem may also be a selection of generalized nuclear coordinates (e.g., corresponding to high-frequency vibrations) while other generalized coordinates are supposed to behave classically, or describe the motion of a proton in a classical environment. So, in this chapter we consider the dynamics of a quantum system in a non-stationary potential. In Section 5.2 we consider the time-dependent potential as externally given, without taking notice of the fact that the sources of the time-dependent potential are moving nuclei, which are quantum particles themselves, feeling the interaction with the quantum d.o.f. Thus we consider the time evolution of the quantum system, which now involves mixing-in of excited states, but we completely ignore the back reaction of the quantum system onto the d.o.f. that cause the time-dependent potential, i.e., the moving nuclei.
Quantum Rutherford scattering and scattering of classical waves off Coulomb-like potentials have similar formal structures and can be studied using the same mathematical techniques. In both contexts, the long-range nature of the interaction leads to a divergent total cross-section, which has been interpreted and regularized in various ways in the past literature. We review in detail the origin of this divergence, in both real and multipole spaces, and show that it arises from incorrectly using approximations out of their domain of validity. We also stress that although classical and quantum Rutherford scattering share the same formalism, the natures of the associated physical observables differ. We comment on the role of interference: while interference can be safely neglected in a quantum context (due to the fact that the observable quantity is a flux, and the incoming flux is collimated), in a classical context one expects to see a superposition of transmitted and scattered waves in a broad region downstream of the target, hence a cross-section is not connected to any physically observable quantity.