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arXiv:2009.11687 · Physical Review A

Radiation eigenmodes of Dicke superradiance

B. Lemberger, Klaus Mølmer

Published Mar 26, 2021• 15 citations
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Abstract

We calculate the field eigenmodes of the superradiant emission from an ensemble of $N$ two-level atoms and confirm the results of other authors that Dicke superradiant emission is restricted to a small number of modes, with more than 90% of the photons emitted in a single dominant mode. While numerical techniques are effective due to the symmetry of the problem, we develop also an analytical method to approximate the modes in the limit of a large number of emitters.

DOI
10.1103/physreva.103.033713

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We calculate the field eigenmodes of the superradiant emission from an ensemble of NNN two-level atoms and confirm the results of other authors that Dicke superradiant emission is restricted to a small number of modes, with more than 90% of the photons emitted in a single dominant mode. While numerical techniques are effective due to the symmetry of the problem, we develop also an analytical method to approximate the modes in the limit of a large number of emitters.
Previous numerical work on the spatiotemporal distributions of the atomic polarization and of the difference in levels population of a one-dimensional system of two-level atoms initially inverted strongly suggested that the dynamics of the slab atomic ensemble in the linear regime of superradiance may best be treated by an eigenmode analysis. This method proved effective in obtaining both the time dependence of the atomic polarization and the spectral distribution of the emitted radiation from the slab in a number of physically interesting problems in the linear regime. In the present paper, I use the eigenfunction expansion technique to reduce the Maxwell-Bloch system of partial differential equations into a system of coupled first-order ordinary differential equations whose solutions clearly detail the contributions of the different modes to the system dynamics in the nonlinear regime of superradiant emission. I compute also the delay in time of the peak of the superradiant burst and its magnitude as functions of the ratio of the longitudinal decay rate to the transverse decay rate of the system.
In order to study the cooperative emission of radiation from an extended system of NNN two-level atoms, we use the master-equation approach within the Born and Markov approximations. All the properties of the emission of radiation can be deduced from the diagonalization of the coupling matrix $\ensuremath{\Gamma}$, where an element ${\ensuremath{\Gamma}}_{\mathrm{jk}}$ gives the coupling between the atoms labeled jjj and kkk via the electromagnetic field. We choose a pencil-shaped volume and study analytically the coupling matrix in the limit for small and large Fresnel numbers. For Fresnel numbers of order unity numerical methods are used. Thus we prove that, for the pencil-shaped geometry, any elaborated model must take into account the interaction of the atoms with the infinity of electromagnetic field modes lying inside two small solid angles about the axis of the largest linear dimension, which we label the zzz axis. In other words, the intensity of radiation emitted by any atom of the system depends on its position with respect to the others and this "propagation effect" cannot be neglected when interpreting superradiance experiments. For small Fresnel numbers the zzz dependence predominates, in the opposite case the (x,yx, yx,y) dependence does, while for Fresnel numbers of order unity the dependence of all three components must be taken into account. Preliminary calculations are given for which only the zzz dependence is considered; for Fresnel numbers of magnitude of order unity or smaller, the effect of propagation along the zzz axis displays large delays for the appearance of superradiance with respect to the time at which the superradiant pulse is maximum when the "propagation effects" are neglected (one-mode model).
We study the quantum statistics of single-mode radiation emitted by an atomic ensemble when the ensemble is initially prepared in a superradiant Dicke state. We show that while the radiation is well approximated by the Glauber coherent state at early times in the evolution, the emission can be truly quantum at later times. In particular, one can observe a large amount of photon-number squeezing in the emission under certain conditions; even a Fock state can be produced. We discuss the quantum statistics of the emission for various parameters, including different initial conditions for the atomic ensemble. To obtain these results, we have developed a formalism where we are able to calculate the quantum statistics of the emission over long time scales even when the number of atoms in the ensemble is quite large.
We introduce a straightforward quantum-electrodynamic approach to the problem of superradiant spontaneous emission from a system of two-level atoms, and also discuss two classical superradiant systems. The same physical concepts underlie our treatment of both the quantum and classical cases. Explicit expressions are found which describe the time evolution and directional character of the radiated power. Our approach applies to an arbitrary number of atoms which are confined to a region with linear dimensions which may be large compared with the mean wavelength of the emitted radiation. The radiative decay half-life of a large many-atom system is found to be much shorter than the natural lifetime of a single atom, but not as short as the half-life of a small atomic system with the same number of atoms. The far-field radiation pattern appropriate to the case of a circular cylinder of emitters which have been excited by a plane-wave pulse is considered in detail. Polar plots are presented of the radiation patterns produced when the atoms are excited by a plane-wave pulse. Exciting pulses traveling in directions both parallel and at an angle of 10\ifmmode^\circ\else\textdegree\fi{} to the axis of the cylinder are considered. A discussion and generalization of Dicke's "coherence-brightening" criterion is given.
Dicke superradiance, a single-mode burst of radiation emitted by an ensemble of two-level atoms, has garnered tremendous attention within the physics community. Its extension to multi-level systems introduces additional degrees of freedom, such as mode-selective control over well-known Dicke superradiant behaviors. However, previous work on the extension to two-mode superradiance in three-level atoms has been largely overlooked for over five decades. In this study, we revisit the two-mode superradiance model for a Λ-type three-level system, where two modes couple to a common excited state and two separate lower levels, offering new insights. For the first time, we obtain exact numerical solutions of the two-mode rate equations for this model. We analyze the temporal evolution of two-mode intensities, superradiance time delays, and quantum noise in the time domain as the number of atoms varies. We believe this work will enable external mode-selective control over superradiance processes—a capability unattainable in the single-mode case.