We revisit a phenomenological model of fermions coupled to fluctuating bosons that emerges from finite-momentum particle-particle pairs for describing the strange metal phase in the cuprates. The incoherent bosons dominate the transport properties for the resistivity and optical conductivity in the non-Fermi-liquid phase. Within the Kubo formalism, the resistivity is approximately linear in temperature with a Drude form for the optical conductivity, such that the Drude lifetime is inversely proportional to the temperature. Here, we compute the transport properties of such bosons within the memory-matrix approach that successfully captures the hydrodynamic regime. This technique emerges as the appropriate framework for describing the transport coefficients of the strange metal phase. Our analysis confirms the
T-linear resistivity due to the umklapp scattering that we obtained for this effective model. Finally, we provide new predictions regarding the variation of the thermal conductivity with temperature and examine the validity of the Wiedemann-Franz law.
Fermi liquid theory forms the basis for our understanding of the majority of metals, which is manifested in the description of transport properties that the electrical resistivity goes as temperature squared in the limit of zero temperature. However, the observations of strange metal states in various quantum materials, notably high-temperature superconductors, bring this spectacularly successful theoretical framework into crisis. When electron scattering rate 1/τ hits its limit, kBT/{\hbar} where {\hbar} is the reduced Planck's constant, T represents absolute temperature and kB denotes Boltzmann's constant, Planckian dissipation occurs and lends strange metals a surprising link to black holes, gravity, and quantum information theory. Here, we show the characteristic signature of strange metallicity arising unprecedentedly in a bosonic system. Our nanopatterned YBa2Cu3O7-δ(YBCO) film arrays reveal T-linear resistance as well as B-linear magnetoresistance over an extended temperature and magnetic field range in a quantum critical region in the phase diagram. Moreover, the slope of the T-linear resistance α_cp appears bounded by α_cp {\approx} h/2e^2 [1/T]_c^onset where T_c^onset is the temperature at which Cooper pairs form, intimating a common scale-invariant transport mechanism corresponding to Planckian dissipation.In contrast to fermionic systems where the temperature and magnetic field dependent scattering rates combine in quadrature of {\hbar}/τ {\approx} {\sqrt} (((k_B T)^2+(μ_B B)^2)), both terms linearly combine in the present bosonic system, i.e. {\hbar}/τ {\approx} (k_B T+[γμ]_B B), where γ is a constant. By extending the reach of strange metal phenomenology to a bosonic system, our results suggest that there is a fundamental principle governing their transport which transcends particle statistics.
The strange metallic regime across a number of high-temperature superconducting materials presents numerous challenges to the classic theory of Fermi liquid metals. Recent measurements of the dynamical charge response of strange metals, including optimally doped cuprates, have revealed a broad, featureless continuum of excitations, extending over much of the Brillouin zone. The collective density oscillations of this strange metal decay into the continuum in a manner that is at odds with the expectations of Fermi liquid theory. Inspired by these observations, we investigate the phenomenology of bosonic collective modes and the particle-hole excitations in a class of strange metals by making an analogy to the phonons of classical lattices falling apart across an unconventional jamming-like transition associated with the onset of rigidity. By making comparisons to the experimentally measured dynamical response functions, we reproduce many of the qualitative features using the above framework. We conjecture that the dynamics of electronic charge density over an intermediate range of energy scales in a class of strongly correlated metals can be at the brink of a jamming-like transition.
Despite much theoretical effort, there is no complete theory of the "strange" metal state of the high temperature superconductors, and its linear-in-temperature T resistivity.Recent experiments showing an unexpected linear-in-field B magnetoresistivity have deepened the puzzle.We propose a simple model of itinerant electrons, interacting via random couplings, with electrons localized on a lattice of "quantum dots" or "islands."This model is solvable in a particular large-N limit and can reproduce observed behavior.The key feature of our model is that the electrons in each quantum dot are described by a Sachdev-Ye-Kitaev model describing electrons without quasiparticle excitations.For a particular choice of the interaction between the itinerant and localized electrons, this model realizes a controlled description of a diffusive marginal-Fermi liquid (MFL) without momentum conservation, which has a linear-in-T resistivity and a T ln T specific heat as T → 0. By tuning the strength of this interaction relative to the bandwidth of the itinerant electrons, we can additionally obtain a finite-T crossover to a fully incoherent regime that also has a linear-in-T resistivity.We describe the magnetotransport properties of this model and show that the MFL regime has conductivities that scale as a function of B=T; however, the magnetoresistance saturates at large B. We then consider a macroscopically disordered sample with domains of such MFLs with varying densities of electrons and islands.Using an effective-medium approximation, we obtain a macroscopic electrical resistance that scales linearly in the magnetic field B applied perpendicular to the plane of the sample, at large B. The resistance also scales linearly in T at small B, and as TfðB=TÞ at intermediate B. We consider implications for recent experiments reporting linear transverse magnetoresistance in the strange metal phases of the pnictides and cuprates.
The strange metal is an enigma within the field of many-body quantum physics, as it defies the standard Fermi liquid theory of metals due to the absence of well-defined, electron-like quasiparticles. It has been presumed that strange metal behavior arises due to strong correlations between electrons that are not present in ordinary Fermi liquids, but the exact nature of these correlations is unknown. To this end, this thesis aims to address the fundamental question: What, precisely, is so strongly correlated about charge in the strange metal? This question is tackled by experimentally measuring the dynamic charge response function, which directly encodes charge correlations in momentum and energy, using the technique of Momentum-resolved Electron Energy-loss Spectroscopy (M-EELS). In particular, two prototypical members of the cuprate and ruthenate strange metal families are studied: Bi-2212 and Sr
2RuO
4. By studying Bi-2212 at optimal doping, it is found that the charge response of the strange metal is characterized by a broad continuum of fluctuations that are momentum and energy independent over a large range of parameter space, unlike Fermi liquid charge correlations which exhibit propagating density waves of charge with well defined energy and momentum (i.e. plasmons). We argue that, in essence, the charge correlations of the strange metal are highly localized in both space and time, unlike the Fermi Liquid where they are localized in momentum and energy instead. To understand how charge correlations change as one leaves the strange metal regime, the M-EELS response of Bi-2212 is mapped out as a function of doping and temperature. At high temperature, it is found that the continuum is largely doping independent. However, upon cooling, very large changes in spectral weight are observed over a range of energy scales nearly two orders of magnitude larger than the thermal scale
kBT. Moreover, this change in spectral weight undergoes a sign reversal as a function of doping, with spectral weight enhancement on the underdoped side, suppression in the overdoped regime, and no change at optimal doping. These changes in spectral weight are completely unlike the case of the Fermi liquid, where doping only acts to rigidly shift the plasmon energy and no significant changes occur as a function of temperature. Finally, we venture further and ask whether strange metal and Fermi liquid charge correlations can simultaneously coexist in a material. To explore this possibility, we measured the M-EELS response of Sr
2RuO
4, a material which exhibits strange and bad metal behavior at high temperature, but transitions to a well-defined Fermi liquid at low temperature. Surprisingly, in the strange metal regime, Sr
2RuO
4 exhibits both a broad continuum similar to Bi-2212 and a propagating Fermi liquid collective mode at low-energies and momentum. Upon cooling, low-energy spectral weight is suppressed in the strange metal continuum and the Fermi liquid collective mode velocity is strongly renormalized. These findings confirm the strange metal and Fermi liquid can coexist and demonstrate that Sr
2RuO
4 exhibits charge correlations with strange metal character at high energies and short length scales and Fermi liquid character at low energies and long wavelengths.
Abstract The mysterious metallic phase showing T-linear resistivity and a universal scattering rate 1 / τ = α P k B T / ℏ with a universal prefactor α P ∼ 1 and logarithmic-in-temperature singular specific heat coefficient, the so-called ‘Planckian metal phase’ was observed in various overdoped high- T c cuprate superconductors over a finite range in doping. Revealing the mystery of the Planckian metal state is believed to be the key to understanding the mechanism for high- T c superconductivity. Here, we propose a generic microscopic mechanism for this state based on quantum-critical local bosonic charge Kondo fluctuations coupled to both spinon and a heavy conduction-electron Fermi surface within the heavy-fermion formulation of the slave-boson t–J model. By a controlled perturbative renormalization group analysis, we examine the competition between the pseudogap phase, characterized by Anderson’s Resonating-Valence-Bond spin-liquid, and the Fermi-liquid state, modeled by the electron hopping (effective charge Kondo effect). We find a quantum-critical metallic phase with a universal Planckian ℏ ω / k B T scaling in scattering rate near an extended localized-delocalized (pseudogap-to-Fermi liquid) charge-Kondo breakdown transition. The d-wave superconducting ground state emerges near the transition. Unprecedented qualitative and quantitative agreements are reached between our theoretical predictions and various experiments, including optical conductivity, universal doping-independent field-to-temperature scaling in magnetoresistance, specific heat coefficient, marginal Fermi-liquid spectral function observed in ARPES, and Fermi surface reconstruction observed in Hall coefficients in various overdoped cuprates. Our mechanism offers a microscopic understanding of the quantum-critical Planckian metal phase observed in cuprates and its link to the pseudogap, d-wave superconducting, and Fermi liquid phases. It offers a promising route for understanding how d-wave superconductivity emerges from such a strange metal phase in cuprates–one of the long-standing open problems in condensed matter physics since 1990s–as well as shows a broader implication for the Planckian strange metal states observed in other correlated unconventional superconductors.