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arXiv:2008.05334 · Physical Review Letters

Electrical Access to Ising Anyons in Kitaev Spin Liquids

Rodrigo G. Pereira, Reinhold Egger

Published Nov 23, 2020• 42 citations
arXivHTMLPDF

Abstract

We show that spin-spin correlations in a non-Abelian Kitaev spin liquid are associated with a characteristic inhomogeneous charge density distribution in the vicinity of Z_{2} vortices. This density profile and the corresponding local electric fields are observable, e.g., by means of surface probe techniques. Conversely, by applying bias voltages to several probe tips, one can stabilize Ising anyons (Z_{2} vortices harboring a Majorana zero mode) at designated positions, where we predict a clear Majorana signature in energy absorption spectroscopy.

DOI
10.1103/physrevlett.125.227202

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We show that spin-spin correlations in a non-Abelian Kitaev spin liquid are associated with a characteristic inhomogeneous charge density distribution in the vicinity of Z_{2} vortices. This density profile and the corresponding local electric fields are observable, e.g., by means of surface probe techniques. Conversely, by applying bias voltages to several probe tips, one can stabilize Ising anyons (Z_{2} vortices harboring a Majorana zero mode) at designated positions, where we predict a clear Majorana signature in energy absorption spectroscopy.
Abstract We formulate a Majorana mean-field theory for the extended J-K-Gamma Kitaev model in a magnetic Zeeman field of arbitrary direction, and apply it for studying spatially inhomogeneous states harboring vortices. This mean-field theory is exact in the pure Kitaev limit and captures the essential physics throughout the Kitaev spin liquid phase. We determine the charge profile around vortices and the corresponding quadrupole tensor. The quadrupole-quadrupole interaction between distant vortices is shown to be either repulsive or attractive, depending on parameters. We predict that electrically biased scanning probe tips enable the creation of vortices at preselected positions. Our results open new perspectives for the electric manipulation of Ising anyons in Kitaev spin liquids.
The Kitaev honeycomb model realizes a quantum spin liquid where spin degrees of freedom are fractionalized into itinerant Majorana fermions and localized vortices. The entanglement among these particles holds promise for executing fault-tolerant topological quantum computation. While several materials have been proposed to host a quantum spin liquid phase, concrete evidence confirming its existence remains elusive. To aid in identifying this phase, we propose an electrical test using the charge profile, offering a signature for the Z2 vortices in Kitaev materials. This study explores the electric charge response in Kitaev materials, considering a generalized spin model including Heisenberg, off-diagonal exchange interactions, and magnetic Zeeman field. Majorana mean-field theory is employed to analyze spin correlations around vortices, revealing spatial anisotropy in the charge distribution, quantified by the electric quadrupole moment. This mean-field approach remains exact in the pure Kitaev limit and captures the fundamental physics across the Kitaev spin liquid phase. The quadrupole-quadrupole interaction between distant vortices is shown to be either repulsive or attractive, depending on the parameters. We predict that electrically biased scanning probe tips can help create vortices at predetermined locations. The findings of our study pave the way for electrically manipulating Ising anyons in Kitaev spin liquids, offering a promising path for technological applications of Kitaev materials.
In the Kitaev chiral spin liquid, Ising anyons are realized as Z_{2} fluxes binding Majorana zero modes, which, however, are thermal excitations with finite decay rates. On the other hand, a lattice vacancy traps a Z_{2} flux even in the ground state, resulting in the stable realization of a Majorana zero mode in a vacancy. We demonstrate that spin-spin correlation functions between two vacancy sites exhibit long-range correlation arising from the fractionalized character of Majorana zero modes, in spite of the strong decay of bulk spin correlations. Remarkably, this nonlocal spin correlation does not decrease as the distance between two vacancy sites increases, signaling Majorana teleportation. Furthermore, we clarify that the nonlocal correlation can be detected electrically via the measurement of nonlocal conductance between two vacancy sites, which is straightforwardly utilized for the readout of Majorana qubits. These findings pave the way to the measurement-based quantum computation with Ising anyons trapped in vacancies of the Kitaev spin liquid.
We study the temperature (T) dependence of the dynamical structure factor of the chiral spin liquid phase of Kitaev's honeycomb model. We find, using a recently developed analytical approach, direct signatures of the Majorana modes associated with the non-Abelian Z_2 vortices (visons). In particular, a characteristic multiplet of discrete peaks at low but nonzero-T and its field dependence reflect the existence of thermally activated visons whose varying separation yields different splittings of the Majorana `zero' modes. The resonant processes involved are specific to the Majorana modes, and will persist even in the presence of weak non-integrable interactions.
The Kitaev model on a honeycomb lattice with bond-dependent Ising interactions offers an exactly solvable model of a quantum spin liquid (QSL) with fractionalized excitations: gapped Z2{Z}_{2}Z2​ fluxes and gapless linearly dispersing Majorana fermions in the isotropic limit (Kx=Ky=Kz{K}_{x}={K}_{y}={K}_{z}Kx​=Ky​=Kz​). We explore the phase diagram along two axes, an external magnetic field hhh, applied out of plane of the honeycomb, and anisotropic interactions Kz{K}_{z}Kz​ larger than the other two (${K}_{x}={K}_{y}\ensuremath{\equiv}K$). For ${K}_{z}/K\ensuremath{\gg}2$ and h=0h=0h=0, the matter Majorana fermions have the largest gap, and the system is described by a gapped Z2{Z}_{2}Z2​ toric code. One of the central questions we address is whether the fractionalized excitations in the different phases have sharp signatures that can be detected in experiments. We show that while the response to single-spin excitations is broad, the spectral function corresponding to two-spin excitations across a bond has sharp signatures that can be attributed to specific anyons. In the toric code regime, the $\ensuremath{\epsilon}=e\ifmmode\times\else\texttimes\fi{}m$ fermion, formed from the bosonic Ising electric (eee) and magnetic (mmm) charges, disperses along a specific one-dimensional direction that provides a fingerprint of fractionalization. At lower Kz{K}_{z}Kz​ in the center of the Abelian phase, in a regime we dub the primordial fractionalized regime, the field generates a hybridization between the $\ensuremath{\epsilon}$ fermion and the Majorana matter fermion, resulting in a $\ensuremath{\psi}$ fermion which too has a distinct quasi-one-dimensional dispersion. All the other phases in the field-anisotropy plane are naturally obtained from this primordial soup. These highly constrained fractonlike dispersions can be observable by inelastic light and neutron scattering, thereby providing ``smoking gun'' signatures of fractionalization in the QSL phase. Our analysis is based on calculations of susceptibilities, topological entanglement entropy, and excitation dynamics, obtained using exact diagonalization and density matrix renormalization group, and supported by perturbation theory.
We propose Majorana-assisted nonlocal spin correlation as a manifestation of Majorana nonlocality in quasi-one-dimensional (1D) Kitaev spin liquids. Focusing on the flux-free sector of the Kitaev honeycomb model in a quasi-1D geometry, we uncover its topological nature and show that it hosts Majorana zero modes localized at both ends, which are stabilized by finite-size-induced topology. We further show that the nonlocal Majorana fermion parity operator, PMF=iγLγRP_{\text{MF}}=iγ_{\text{L}}γ_{\text{R}}PMF​=iγL​γR​, is mapped to a nonlocal spin-string operator, producing an end-to-end spin correlation proportional to the product of PMFP_{\text{MF}}PMF​ and total fermion parity operators when local perturbations remove redundant ground-state degeneracies while preserving the Majorana and total fermion parities in the flux-free sector. Numerical calculations confirm a finite nonlocal spin correlation generated by these Majorana zero modes without any local magnetization. Our results establish a concrete signature of intrinsic Majorana nonlocality in quantum spin liquids.