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arXiv:2007.13774 · Physical Review Research

Universal relations for dipolar quantum gases

Johannes Hofmann, W. Zwerger

Published Jan 28, 2021• 13 citations
arXivHTMLPDF

Abstract

We establish that two-dimensional dipolar quantum gases admit a universal description, i.e., their thermodynamic properties are independent of details of the interaction at short distances.The only relevant parameters are the dipole length as well as the scattering length of the combined short-range plus dipolar interaction potential.We derive adiabatic relations that link the change in the thermodynamic potentials with respect to the scattering length and the dipole length to a generalized Tan contact parameter and a new dipolar contact, which involves an integral of a short-distance regularized pair distribution function.These two quantities determine the scale anomaly in the difference between pressure and energy density and also the internal energy in the presence of a harmonic confinement.For a weak transverse confinement, configurations with attractive interactions appear, which lead to a density-wave instability beyond a critical strength of the dipolar interaction.We show that this instability essentially coincides with the onset of a roton minimum in the excitation spectrum and may be understood in terms of a quantum analog of the Hansen-Verlet criterion for freezing of a classical fluid.

DOI
10.1103/physrevresearch.3.013088

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We establish that two-dimensional dipolar quantum gases admit a universal description, i.e., their thermodynamic properties are independent of details of the interaction at short distances.The only relevant parameters are the dipole length as well as the scattering length of the combined short-range plus dipolar interaction potential.We derive adiabatic relations that link the change in the thermodynamic potentials with respect to the scattering length and the dipole length to a generalized Tan contact parameter and a new dipolar contact, which involves an integral of a short-distance regularized pair distribution function.These two quantities determine the scale anomaly in the difference between pressure and energy density and also the internal energy in the presence of a harmonic confinement.For a weak transverse confinement, configurations with attractive interactions appear, which lead to a density-wave instability beyond a critical strength of the dipolar interaction.We show that this instability essentially coincides with the onset of a roton minimum in the excitation spectrum and may be understood in terms of a quantum analog of the Hansen-Verlet criterion for freezing of a classical fluid.
The low-density expansions for the energy, chemical potential, and condensate depletion of the homogeneous dilute dipolar Bose gas are obtained by regularizing the dipole-dipole interaction at long distances. It is shown that the leading term, proportional to the density, allows a simple physical interpretation and consistently describes the thermodynamic stability of the system. The long-range asymptotics are obtained analytically for the normal and anomalous one-particle correlation functions and the pair distribution function. We discuss the properties of the two-body scattering with zero relative momentum for the dipole-dipole interaction; in particular, we derive the asymptotics of the wave function and a correction to the scattering length for small values of the dipolar range. We show how the density expansions can be derived within the Bogoliubov model of weakly interacting particles without any divergence from the assumption of universality of the expansions at low densities.
We present a thermodynamic description of ultracold gases with dipolar interactions which properly accounts for the long-range nature and broken rotation invariance of the interactions. It involves an additional thermodynamic field conjugate to the linear extension of the gas along the direction of the dipoles. The associated uniaxial pressure shows up as a deviation from the Gibbs–Duhem relation in the density profile of a trapped gas. It has to vanish in self-bound droplets, a condition which determines the observed dependence of the aspect ratio on particle number. A tensorial generalization of the virial theorem and a number of further exact thermodynamic relations are derived. Finally, extending a model due to Nozières, a simple criterion for the freezing transition to a superfluid mass density wave is given.
In quasi-one- or quasi-two-dimensional traps with strong transverse confinements, quantum gases behave like strictly one- or two-dimensional systems at large length scales. However, at short distance, the two-body scattering intrinsically has three-dimensional characteristics such that an exact description of any universal thermodynamic relation requires three-dimensional contacts since the range of interaction (a few nm) is orders of magnitude smaller than the harmonic-oscillator length of the transverse confinement ($\ensuremath{\sim}{10}^{2}\phantom{\rule{0.28em}{0ex}}\mathrm{nm}$ for a 100 kHz trap). A fundamental question arises as to whether one- or two-dimensional contacts, which were originally defined for strictly one or two dimensions, are capable of describing quantum gases in quasi-one- or quasi-two-dimensional traps. Here, we point out an exact relation between the three- and low-dimensional contacts in these highly anisotropic traps. Such relation allows us to directly connect physical quantities at different length scales and to characterize the quasi-one- or quasi-two-dimensional traps using universal thermodynamic relations that were derived for strict one or two dimensions.
The energy of ultra-dilute quantum many-body systems is known to exhibit a universal dependence on the gas parameter x=n a_0^d x = n a 0 d , with n n the density, d d the dimensionality of the space ( d=1,2,3 d = 1 , 2 , 3 ) and a_0 a 0 the s s -wave scattering length. The universal regime typically extends up to x\approx 0.001 x ≈ 0.001 , while at larger values specific details of the interaction start to be relevant and different model potentials lead to different results. Dipolar systems are peculiar in this regard since the anisotropy of the interaction makes a_0 a 0 depend on the polarization angle \alpha α , so different combinations of n and \alpha α can lead to the same value of the gas parameter x. In this work we analyze the scaling properties of dipolar bosons in two dimensions as a function of the density and polarization dependent scattering length up to very large gas parameter values. Using Quantum Monte Carlo (QMC) methods we study the energy and the main structural and coherence properties of the ground state of a gas of dipolar bosons by varying the density and scattering length for a fixed gas parameter. We find that the dipolar interaction shows relevant scaling laws up to unusually large values of x x that hold almost to the boundaries in the phase diagram where a transition to a stripe phase takes place.
A microscopic description of the zero-energy two-body ground state and many-body static properties of anisotropic homogeneous gases of bosonic dipoles in two dimensions at low densities is presented and discussed. By changing the polarization angle with respect to the plane, we study the impact of the anisotropy, present in the dipole-dipole interaction, on the energy per particle, comparing the results with mean-field predictions. We restrict the analysis to the regime where the interaction is always repulsive, although the strength of the repulsion depends on the orientation with respect to the polarization field. We present a series expansion of the solution of the zero-energy two-body problem, which allows us to find the scattering length of the interaction and to build a suitable Jastrow factor that we use as a trial wave function for both a variational and diffusion Monte Carlo simulation of the infinite system. We find that the anisotropy has an almost negligible impact on the ground-state properties of the many-body system in the universal regime where the scattering length governs the physics of the system. We also show that scaling in the gas parameter persists in the dipolar case up to values where other isotropic interactions with the same scattering length yield different predictions.
We derive universal relations between thermodynamic quantities and the pair distribution function for bosons interacting via power-law interactions in three and two dimensions. We find beyond mean-field expressions for Tan's contact and establish new connections between the chemical potential and potential energy per particle, characteristic of systems with finite-range interactions. The obtained results are relevant for dipoles, quadrupoles, Rydberg atoms, excitons, van der Waals atoms, and other systems in the dilute limit.