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arXiv:2007.10680 · Physical Review A

Limit cycle phase and Goldstone mode in driven dissipative systems

Hadiseh Alaeian, G. Giedke, Iacopo Carusotto, R. Löw, Tilman Pfau

Published Jan 11, 2021• 16 citations
arXivHTMLPDF

Abstract

In this article, we theoretically investigate the first- and second-order quantum dissipative phase transitions of a three-mode cavity with a Hubbard interaction. In both types, there is a mean-field (MF) limit cycle phase where the local U(1) symmetry and the time-translational symmetry of the Liouvillian superoperator are spontaneously broken. In MF, this spontaneous symmetry breaking manifests itself through the appearance of an unconditionally and fully squeezed state at the cavity output, connected to the well-known Goldstone mode. By employing the Wigner function formalism, hence, properly including the quantum noise, we show that away from the thermodynamic limit and within the quantum regime, fluctuations notably limit the coherence time of the Goldstone mode due to the phase diffusion. Our theoretical predictions suggest that interacting multimode photonic systems are rich, versatile test beds for investigating the crossovers between the mean-field picture and quantum phase transitions, a problem that can be investigated in various platforms including superconducting circuits, semiconductor microcavities, atomic Rydberg polaritons, and cuprite excitons.

DOI
10.1103/physreva.103.013712

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In this article, we theoretically investigate the first- and second-order quantum dissipative phase transitions of a three-mode cavity with a Hubbard interaction. In both types, there is a mean-field (MF) limit cycle phase where the local U(1) symmetry and the time-translational symmetry of the Liouvillian superoperator are spontaneously broken. In MF, this spontaneous symmetry breaking manifests itself through the appearance of an unconditionally and fully squeezed state at the cavity output, connected to the well-known Goldstone mode. By employing the Wigner function formalism, hence, properly including the quantum noise, we show that away from the thermodynamic limit and within the quantum regime, fluctuations notably limit the coherence time of the Goldstone mode due to the phase diffusion. Our theoretical predictions suggest that interacting multimode photonic systems are rich, versatile test beds for investigating the crossovers between the mean-field picture and quantum phase transitions, a problem that can be investigated in various platforms including superconducting circuits, semiconductor microcavities, atomic Rydberg polaritons, and cuprite excitons.
We theoretically investigate the critical properties of a single driven-dissipative nonlinear photon mode. In a well-defined thermodynamical limit of large excitation numbers, the exact quantum solution describes a first-order phase transition in the regime where semiclassical theory predicts optical bistability. We study the behavior of the complex spectral gap associated with the Liouvillian superoperator of the corresponding master equation. We show that in this limit the Liouvillian gap vanishes exponentially and that the bimodality of the photon Wigner function disappears. The connection between the considered thermodynamical limit of large photon numbers for the single-mode cavity and the thermodynamical limit of many cavities for a driven-dissipative Bose-Hubbard system is discussed.
We investigate nonequilibrium criticality and chaos in a two-photon-driven optomechanical system. The parametric drive preserves a discrete Z2\mathbb{Z}_2Z2​ symmetry of the optical field, while radiation-pressure coupling transfers the resulting nonlinear dynamics to a mechanical oscillator. Combining semiclassical stability analysis, exact Liouvillian spectra, and stochastic quantum trajectories, we show that this driven-dissipative optomechanical model supports both first- and second-order dissipative phase transitions. At negative detuning a second-order transition yields spontaneous breaking of the cavity-parity symmetry in the thermodynamic limit. At positive detuning the same symmetry breaking coexists with a first-order transition, signaled by metastability and by an additional symmetric Liouvillian mode. At stronger pump power the mean-field dynamics loses all stable fixed points and develops limit cycles and chaotic attractors with positive Lyapunov exponent. Quantum trajectories in this regime display chaotic-like motion, enhanced steady-state entropy, and delocalization over many entropic Liouvillian modes. These results establish two-photon-driven optomechanics as a platform where dissipative criticality, symmetry breaking, and quantum signatures of chaos emerge within the same experimentally accessible setting.
Supersolids are characterized by the counterintuitive coexistence of superfluid and crystalline order. Here we study a supersolid phase emerging in the steady state of a driven-dissipative system. We consider a transversely pumped Bose-Einstein condensate trapped along the axis of a ring cavity and coherently coupled to a pair of degenerate counterpropagating cavity modes. Above a threshold pump strength the interference of photons scattered into the two cavity modes results in an emergent superradiant lattice, which spontaneously breaks the continuous translational symmetry towards a periodic atomic pattern. The crystalline steady state inherits the superfluidity of the Bose-Einstein condensate, thus exhibiting genuine properties of a supersolid. A gapless collective Goldstone mode correspondingly appears in the superradiant phase, which can be nondestructively monitored via the relative phase of the two cavity modes on the cavity output. Despite cavity-photon losses the Goldstone mode remains undamped, indicating the robustness of the supersolid phase.
The study of phase transitions and critical phenomena arising in quantum driven-dissipative systems, and whether a correspondence can be drawn to their equilibrium counterparts, is a pressing question in contemporary physics. The development of large-scale superconducting circuits provides an experimental platform for these theoretical models. We report an experimental study of a multimode dissipative first-order phase transition in a 1D Bose-Hubbard chain consisting of 21 superconducting resonators. This phase transition manifests itself as a simultaneous frequency jump in all resonator modes as the frequency or power of a pump tone is swept. By measuring the system’s emission spectrum through the transition, we characterize the dim-to-bright phase transition and construct the full phase diagram. We further perform time-dependent measurements of the switching between the two phases in the transition region, from which we corroborate the transition line and extract transition times ranging from a few ms up to 143 s. Our model, based on single-mode mean-field theory and cross-Kerr interactions, captures the features at moderate pump powers and quantitatively reproduces the transition line. Our results open a new window into nonequilibrium quantum many-body physics and mark a step toward realizing and understanding dissipative phase transitions in the thermodynamic limit using superconducting quantum circuits. In addition, our study opens new possibilities for sensing and cryo-switching applications.
In open quantum systems, dissipative phase transitions (DPTs) emerge from the interplay between unitary evolution, drive, and dissipation. While second-order DPTs have been predominantly investigated theoretically, first-order DPTs have been observed in single-photon-driven Kerr resonators. We present here an experimental and theoretical analysis of both first and second-order DPTs in a two-photon-driven superconducting Kerr resonator. We characterize the steady state at the critical points, showing squeezing below vacuum and the coexistence of phases with different photon numbers. Through time resolved measurements, we study the dynamics across the critical points and observe hysteresis cycles at the first-order DPT and spontaneous symmetry breaking at the second-order DPT. Extracting the timescales of the critical phenomena reveals slowing down across five orders of magnitude when scaling towards the thermodynamic limit. Our results showcase the engineering of criticality in superconducting circuits, advancing the use of parametric resonators for critically-enhanced quantum information applications.
Spontaneous breaking of a continuous symmetry produces a massless Goldstone mode that can evolve across a degenerate manifold at zero energy cost. Goldstone modes have been identified primarily through excitation spectra, mode softening or collective oscillations. However, their time-domain transport under intrinsic fluctuations and dissipation has remained largely unexplored. Here we directly track the stochastic transport of a Goldstone mode in a self-organized atomic crystal inside an optical ring cavity. The ring cavity maps the order-parameter phase onto the real-space position of the emergent crystal. Without any external perturbation, fundamental photon-scattering recoil drives the collective transport, while cavity dissipation generates friction. We monitor individual trajectories of the atoms and their self-generated optical lattice by measuring the cavity output phase. We find that the diffusion constant decreases as 1/N1/N1/N, indicating that all atoms move collectively as a rigid object rather than independently. By tuning the Langevin driving force and cavity-mediated damping, we show that the normalized diffusion constant collapses onto a single universal curve. This work extends the study of continuous symmetry breaking from excitation-frequency measurements to real-time tracking of transport, and opens routes for studying non-equilibrium collective transport, phonon dynamics, and defect formation in driven-dissipative quantum matter.