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arXiv:2007.09113 · Journal of Statistical Mechanics Theory and Experiment

Free energy fluxes and the Kubo–Martin–Schwinger relation

Benjamin Doyon, Joseph Durnin

Published Apr 1, 2021• 16 citations
arXivHTMLPDF

Abstract

Abstract A general, multi-component Eulerian fluid theory is a set of nonlinear, hyperbolic partial differential equations. However, if the fluid is to be the large-scale description of a short-range many-body system, further constraints arise on the structure of these equations. Here we derive one such constraint, pertaining to the free energy fluxes. The free energy fluxes generate expectation values of currents, akin to the specific free energy generating conserved densities. They fix the equations of state and the Euler-scale hydrodynamics, and are simply related to the entropy currents. Using the Kubo–Martin–Schwinger relations associated to many conserved quantities, in quantum and classical systems, we show that the associated free energy fluxes are perpendicular to the vector of inverse temperatures characterising the state. This implies that all entropy currents can be expressed as averages of local observables. In few-component fluids, it implies that the averages of currents follow from the specific free energy alone, without the use of Galilean or relativistic invariance. In integrable models, in implies that the thermodynamic Bethe ansatz must satisfy a unitarity condition. The relation also guarantees physical consistency of the Euler hydrodynamics in spatially-inhomogeneous, macroscopic external fields, as it implies conservation of entropy, and the local-density approximated Gibbs form of stationarity states. The main result on free energy fluxes is based on general properties such as clustering, and we show that it is mathematically rigorous in quantum spin chains.

DOI
10.1088/1742-5468/abefe3

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Abstract Hydrodynamics is a powerful emergent theory for the large-scale behaviours in many-body systems, quantum or classical. It is a gradient series expansion, where different orders of spatial derivatives provide an effective description on different length scales. We report the first fully general derivation of third-order, or ‘dispersive’, terms in the hydrodynamic expansion. Our derivation is based on general principles of statistical mechanics, along with the assumption that the complete set of local and quasi-local conserved densities constitutes a good set of emergent degrees of freedom. We obtain fully general Kubo-like expressions for the associated hydrodynamic coefficients (also known as Burnett coefficients), and we determine their exact form in quantum integrable models, introducing in this way purely quantum higher-order terms into generalised hydrodynamics. We emphasise the importance of hydrodynamic gauge fixing at diffusive order, where we claim that it is parity-time-reversal, and not time-reversal, invariance that is at the source of Einstein’s relation, Onsager’s reciprocal relations, the Kubo formula and entropy production. At higher hydrodynamic orders we introduce a more general, nth order ‘symmetric’ gauge, which we show implies the validity of the higher-order hydrodynamic description.
The macroscopic hydrodynamic equations are derived for many-body systems in the local-equilibrium approach, using the Schrödinger picture of quantum mechanics. In this approach, statistical operators are defined in terms of microscopic densities associated with the fundamentally conserved quantities and other slow modes possibly emerging from continuous symmetry breaking, as well as macrofields conjugated to these densities. Functional identities can be deduced, allowing us to identify the reversible and dissipative parts of the mean current densities, to obtain general equations for the time evolution of the conjugate macrofields, and to establish the relationship to projection-operator methods. The entropy production is shown to be nonnegative by applying the Peierls-Bogoliubov inequality to a quantum integral fluctuation theorem. Using the expansion in the gradients of the conjugate macrofields, the transport coefficients are given by Green-Kubo formulas and the entropy production rate can be expressed in terms of quantum Einstein-Helfand formulas, implying its nonnegativity in agreement with the second law of thermodynamics. The results apply to multicomponent fluids and can be extended to condensed matter phases with broken continuous symmetries.
Using the theory of generalized hydrodynamics (GHD), we derive exact Euler-scale dynamical two-point correlation functions of conserved densities and currents in inhomogeneous, non-stationary states of many-body integrable systems with weak space-time variations. This extends previous works to inhomogeneous and non-stationary situations. Using GHD projection operators, we further derive formulae for Euler-scale two-point functions of arbitrary local fields, purely from the data of their homogeneous one-point functions. These are new also in homogeneous generalized Gibbs ensembles. The technique is based on combining a fluctuation-dissipation principle along with the exact solution by characteristics of GHD, and gives a recursive procedure able to generate n n -point correlation functions. Owing to the universality of GHD, the results are expected to apply to quantum and classical integrable field theory such as the sinh-Gordon model and the Lieb-Liniger model, spin chains such as the XXZ and Hubbard models, and solvable classical gases such as the hard rod gas and soliton gases. In particular, we find Leclair-Mussardo-type infinite form-factor series in integrable quantum field theory, and exact Euler-scale two-point functions of exponential fields in the sinh-Gordon model and of powers of the density field in the Lieb-Liniger model. We also analyse correlations in the partitioning protocol, extract large-time asymptotics, and, in free models, derive all Euler-scale n n -point functions.
The problem considered here is motivated by a work by B. Nachtergaele and H.T. Yau where the Euler equations of fluid dynamics are derived from manybody quantum mechanics, see [10]. A crucial concept in their work is that of local quantum Gibbs states, which are quantum statistical equilibria with prescribed particle, current, and energy densities at each point of space (here R d , d ≥\ge≥ 1). They assume that such local Gibbs states exist, and show that if the quantum system is initially in a local Gibbs state, then the system stays, in an appropriate asymptotic limit, in a Gibbs state with particle, current, and energy densities now solutions to the Euler equations. Our main contribution in this work is to prove that such local quantum Gibbs states can be constructed from prescribed densities under mild hypotheses, in both the fermionic and bosonic cases. The problem consists in minimizing the von Neumann entropy in the quantum grand canonical picture under constraints of local particle, current, and energy densities. The main mathematical difficulty is the lack of compactness of the minimizing sequences to pass to the limit in the constraints. The issue is solved by defining auxiliary constrained optimization problems, and by using some monotonicity properties of equilibrium entropies.
Abstract We propose a general formalism, within large-deviation theory, giving access to the exact statistics of fluctuations of ballistically transported conserved quantities in homogeneous, stationary states. The formalism is expected to apply to any system with an Euler hydrodynamic description, classical or quantum, integrable or not, in or out of equilibrium. We express the exact scaled cumulant generating function (or full counting statistics) for any (quasi-)local conserved quantity in terms of the flux Jacobian. We show that the “extended fluctuation relations” of Bernard and Doyon follow from the linearity of the hydrodynamic equations, forming a marker of “freeness” much like the absence of hydrodynamic diffusion does. We show how an extension of the formalism gives exact exponential behaviours of spatio-temporal two-point functions of twist fields, with applications to order-parameter dynamical correlations in arbitrary homogeneous, stationary state. We explain in what situations the large-deviation principle at the basis of the results fail, and discuss how this connects with nonlinear fluctuating hydrodynamics. Applying the formalism to conformal hydrodynamics, we evaluate the exact cumulants of energy transport in quantum critical systems of arbitrary dimension at low but nonzero temperatures, observing a phase transition for Lorentz boosts at the sound velocity.