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arXiv:2006.12750 · Optics Letters

Strongly confined atomic localization by Rydberg coherent population trapping

Teodora Kirova, Ning Jia, Seyyed Hossein Asadpour, Jing Qian, Gediminas Juzeliūnas, Hamid Reza Hamedi

Published Aug 14, 2020• 17 citations
arXivHTMLPDF

Abstract

We investigate the possibility to attain strongly confined atomic localization using interacting Rydberg atoms in a coherent population trapping ladder configuration, where a standing-wave is used as a coupling field in the second leg of the ladder. Depending on the degree of compensation for the Rydberg level energy shift induced by the van der Waals interaction, by the coupling field detuning, we distinguish between two antiblockade regimes, i.e., a partial antiblockade (PA) and a full antiblockade. While a periodic pattern of tightly localized regions can be achieved for both regimes, the PA allows much faster convergence of spatial confinement, yielding a high-resolution Rydberg state-selective superlocalization regime for higher-lying Rydberg levels. In comparison, for lower-lying Rydberg levels, the PA leads to an anomalous change of spectra linewidth, confirming the importance of using a stable uppermost state to achieve a superlocalization regime.

DOI
10.1364/ol.400849

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We investigate the possibility to attain strongly confined atomic localization using interacting Rydberg atoms in a coherent population trapping ladder configuration, where a standing-wave is used as a coupling field in the second leg of the ladder. Depending on the degree of compensation for the Rydberg level energy shift induced by the van der Waals interaction, by the coupling field detuning, we distinguish between two antiblockade regimes, i.e., a partial antiblockade (PA) and a full antiblockade. While a periodic pattern of tightly localized regions can be achieved for both regimes, the PA allows much faster convergence of spatial confinement, yielding a high-resolution Rydberg state-selective superlocalization regime for higher-lying Rydberg levels. In comparison, for lower-lying Rydberg levels, the PA leads to an anomalous change of spectra linewidth, confirming the importance of using a stable uppermost state to achieve a superlocalization regime.
We propose a robust localization of the highly-excited Rydberg atoms, interacting with doughnut-shaped optical vortices. Compared with the earlier standing-wave (SW)-based localization methods, a vortex beam can provide an ultrahigh-precision two-dimensional localization solely in the zero-intensity center, within a confined excitation region down to the nanometer scale. We show that the presence of the Rydberg-Rydberg interaction permits counter-intuitively much stronger confinement towards a high spatial resolution when it is partially compensated by a suitable detuning. In addition, applying an auxiliary SW modulation to the two-photon detuning allows a three-dimensional confinement of Rydberg atoms. In this case, the vortex field provides a transverse confinement while the SW modulation of the two-photon detuning localizes the Rydberg atoms longitudinally. To develop a new subwavelength localization technique, our results pave one-step closer to reduce excitation volumes to the level of a few nanometers, representing a feasible implementation for the future experimental applications.
We propose a robust localization of the highly-excited Rydberg atoms interacting with doughnut-shaped optical vortices. Compared with the earlier standing-wave (SW)-based localization methods, a vortex beam can provide an ultraprecise two-dimensional localization solely in the zero-intensity center, within a confined excitation region down to the nanometer scale. We show that the presence of the Rydberg-Rydberg interaction permits counter-intuitively much stronger confinement towards a high spatial resolution when it is partially compensated by a suitable detuning. In addition, applying an auxiliary SW modulation to the two-photon detuning allows a three-dimensional confinement of Rydberg atoms. In this case, the vortex field provides a transverse confinement, while the SW modulation of the two-photon detuning localizes the Rydberg atoms longitudinally. To develop a new subwavelength localization technique, our results pave a path one step closer to reducing excitation volumes to the level of a few nanometers, representing a feasible implementation for the future experimental applications.
Resonant laser excitation of multiple Rydberg atoms are prohibited, leading to Rydberg blockade, when the long-range van der Waals interactions are stronger than the laser-atom coupling. Rydberg blockade can be violated, i.e., simultaneous excitation of more than one Rydberg atom, by off-resonant laser excitation, causing an excitation antiblockade. Rydberg antiblockade gives rise to strongly correlated many-body dynamics and spin-orbit coupling and also finds quantum computation applications. Instead of commonly used van der Waals interactions, we investigate antiblockade dynamics of two Rydberg atoms interacting via dipole-dipole exchange interactions. We study typical situations in current Rydberg atom experiments, where different types of dipole-dipole interactions can be achieved by varying Rydberg state couplings. An effective Hamiltonian governing underlying antiblockade dynamics is derived. We illustrate that geometric gates can be realized with the Rydberg antiblockade which is robust against the decay of Rydberg states. Our study may stimulate new experimental and theoretical exploration of quantum optics and strongly interacting many-body dynamics with Rydberg antiblockade driven by dipole-dipole interactions.
We study the Rydberg blockade in a system of three atoms arranged in different two-dimensional geometries (linear and triangular configurations). In the strong blockade regime, we observe high-contrast, coherent collective oscillations of the single excitation probability and an almost perfect van der Waals blockade. Our data are consistent with a total population in doubly and triply excited states below 2%. In the partial blockade regime, we directly observe the anisotropy of the van der Waals interactions between |nD> Rydberg states in the triangular configuration. A simple model that only uses independently measured two-body van der Waals interactions fully reproduces the dynamics of the system without any adjustable parameter. These results are extremely promising for scalable quantum information processing and quantum simulation with neutral atoms.
We report the direct measurement of the van der Waals interaction between two isolated, single Rydberg atoms separated by a controlled distance of a few micrometers.Working in a regime where the single-atom Rabi frequency for excitation to the Rydberg state is comparable to the interaction, we observe partial Rydberg blockade, whereby the time-dependent populations of the various two-atom states exhibit coherent oscillations with several frequencies.Quantitative comparison of the data with a simple model based on the optical Bloch equations allows us to extract the van der Waals energy, and observe its characteristic C 6 =R 6 dependence.The measured C 6 coefficients agree well with ab initio calculations, and we observe their dramatic increase with the principal quantum number n of the Rydberg state.
Rydberg antiblockade (RAB) allows more than one Rydberg atom to be excited in the presence of Rydberg-Rydberg interaction (RRI) and has many potential applications in quantum optics, many-body physics and quantum information. In this paper, we would review the conditions and possible applications of different types of RAB regimes under weak, intermediate and strong RRIs, respectively. Both van der Waals (vdW) and dipole-dipole (DD) interactions are considered for each interaction strength. This work displays the layout of RAB and provides a reference for further study of RAB-regime-based quantum optics and quantum information processing tasks.