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arXiv:2006.02730 · Physical Review A

Spectral Green's-function method in driven open quantum dynamics

Alexander A. Karabanov, Walter Köckenberger

Published Jan 27, 2021• 1 citation
arXivHTMLPDF

Abstract

A method based on spectral Green's functions is presented for the simulation of driven open quantum dynamics that can be described by the Lindblad master equation in Liouville density operator space. The method extends the Hilbert space formalism and provides simple algebraic connections between the driven and nondriven dynamics in the spectral frequency domain. The formalism shows remarkable analogies to the use of Green's functions in quantum field theory, such as the elementary excitation energies and the Dyson self-energy equation. To demonstrate its potential, we apply the method to a coherently driven dissipative ensemble of two-level systems comprising a single ``active'' subsystem interacting with $N$ ``passive'' subsystems---a generic model with important applications in quantum optics and dynamic nuclear polarization. The method dramatically reduces the computational cost compared with simulations based on solving the full master equation, thus making it possible to study and optimize many-body correlated states up to the physically realistic limit of an arbitrarily large $N$.

DOI
10.1103/physreva.103.012224

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A method based on spectral Green's functions is presented for the simulation of driven open quantum dynamics that can be described by the Lindblad master equation in Liouville density operator space. The method extends the Hilbert space formalism and provides simple algebraic connections between the driven and nondriven dynamics in the spectral frequency domain. The formalism shows remarkable analogies to the use of Green's functions in quantum field theory, such as the elementary excitation energies and the Dyson self-energy equation. To demonstrate its potential, we apply the method to a coherently driven dissipative ensemble of two-level systems comprising a single active'' subsystem interacting with $N$ passive'' subsystems---a generic model with important applications in quantum optics and dynamic nuclear polarization. The method dramatically reduces the computational cost compared with simulations based on solving the full master equation, thus making it possible to study and optimize many-body correlated states up to the physically realistic limit of an arbitrarily large NNN.
We study driven and open quantum systems described by a time-periodic Lindblad master equation. In closed systems, the stroboscopic dynamics can always be described by an effective time-independent Floquet Hamiltonian; this idea is the basis of Floquet engineering. However, in the presence of dissipation, the existence of an effective time-independent Floquet Lindbladian is not guaranteed due to the non-unitary nature of the evolution. Using Floquet theory, we construct a well-defined time-independent Floquet Lindbladian in an extended Sambe-Liouville space, transforming the initial time-dependent problem to a static and non-Hermitian eigenvalue problem. For harmonic driving, we introduce a matrix continued fraction method to nonperturbatively resum multiphoton processes and construct an effective Floquet Lindbladian acting only on the physical Liouville space. Compared to other high-frequency expansions, this method has the advantage of providing the whole infinite series expansion at once. Using a resolvent formalism, we show how to obtain a spectral Floquet representation of correlation functions of an open quantum system. As an application, we consider a dissipating two-level system in a linearly polarized field and calculate its resonance fluorescence spectrum. Furthermore, we consider a parametrically driven quantum dot with pump and loss for which we calculate its spectral function and current-voltage characteristics.
We develop an exact analytical framework for studying the nonequilibrium dynamics of interacting quantum harmonic oscillators coupled to a modelled thermal reservoir and driven by external classical fields. The total Hamiltonian is diagonalized via successive Bogoliubov transformations, enabling a nonperturbative treatment of dissipation and driving. For two coupled oscillators with an external source applied to the first, we derive explicit energy expressions and analyze their dependence on coupling and bath parameters. The phase-space structure is characterized through Husimi QQQ-functions for initial separable coherent and number states. We obtain the reduced density matrix elements in the number-state basis and demonstrate that, in the absence of driving and at zero temperature, the reduced density matrix of the main system satisfies the Lindblad master equation. A generating function for the Husimi function is introduced to facilitate computation of higher-order correlations. The analysis is then generalized to nnn interacting oscillators, with analytical energy expressions provided and the case n=3n=3n=3 examined in detail. Our results establish a versatile and exact framework for driven-dissipative quantum systems, with potential applications in quantum thermodynamics, open quantum systems, and many-body physics.
We develop an exact framework for describing the non-Markovian dynamics of an open quantum system interacting with an environment modeled by a generalized spectral density function.The approach relies on mapping the initial system onto an auxiliary configuration, comprising the original open system coupled to a small number of discrete modes, which in turn are each coupled to an independent Markovian reservoir.Based on the connection between the discrete modes and the poles of the spectral density function, we show how expanding the system using the discrete modes allows for the full inclusion non-Markovian effects within an enlarged open system whose dynamics is governed by an exact Lindblad master equation.Initially we apply this result to obtain a generalization of the pseudomode method [B.M. Garraway, Phys. Rev. A. 55, 2290 (1997)] in cases where the spectral density function has a Lorentzian structure.For many other types of spectral density function, we extend our proof to show that an open system dynamics may be modeled physically using discrete modes which admit a non-Hermitian coupling to the system and for such cases determine the equivalent master equation to no longer be of Lindblad form.For applications involving two discrete modes, we demonstrate how to convert between pathological and Lindblad forms of the master equation using the techniques of the pseudomode method.
In this paper, we investigate periodically driven open quantum systems within the framework of Floquet-Lindblad master equations. Specifically, we discuss Lindblad master equations in the presence of a coherent, time-periodic driving and establish their general spectral features. We also clarify the notions of transient and nondecaying solutions from this spectral perspective, and then prove that any physical system described by a Floquet-Lindblad equation must have at least one physical nonequilibrium steady state (NESS), corresponding to an eigenoperator of the Floquet-Lindblad evolution superoperator UF{\mathcal{U}}_{F}UF​ with unit eigenvalue. Since the Floquet-Lindblad formalism encapsulates the entire information regarding the NESS, it in principle enables us to obtain nonlinear effects to all orders at once. The Floquet-Lindblad formalism thus provides a powerful tool for studying driven-dissipative solid-state systems, which we illustrate by deriving the nonlinear optical response of a simple two-band model of an insulating solid and comparing it with prior results established through Keldysh techniques.
The Markovian dynamics of open quantum many-body systems are typically governed by the Lindblad master equation, yet obtaining the reduced density matrix for bosonic and fermionic systems remains a formidable numerical challenge due to the exponential growth of the Hilbert space. Here, we introduce a computationally efficient framework for constructing the reduced density matrix by modeling the environment as a copy of the primary system with a monotonically decaying coupling that enforces unidirectional energy flow. Our method directly yields exact solutions that rigorously satisfy the Lindblad master equation for both bosonic and fermionic cases, bypassing the need for costly Liouvillian diagonalization. We validate our approach through applications to paradigmatic models, demonstrating accurate reproduction of dissipative dynamics across a broad parameter regime. This work provides a straightforward and powerful tool for simulating Markovian open-system evolution, with immediate applicability to quantum transport and control problems in many-body physics.
Driven-dissipative quantum devices are routinely operated with time-dependent drives and exposed to temporally correlated classical noise. When these perturbations vary on timescales comparable to the system's intrinsic dynamics, rotating-wave and Markovian approximations can fail, making effective static descriptions unreliable. As a result, accurately modeling systems in this regime often relies on simulating the full time-dependent master equation. This is particularly demanding for processes requiring long integration times, such as rare switching between metastable states, or for stochastic perturbations requiring averaging over many noise realizations. To address these challenges, we introduce Liouvillian spectral snapshots (LSS), a reduced-basis method that enables efficient simulation of such systems by projecting the master equation onto a low-dimensional subspace capturing their coarse-grained dynamics. LSS constructs this subspace by computing the slowly decaying, low-frequency eigenoperators of the Liouvillian at a few adaptively sampled perturbation values and compressing them into a common basis. This basis is built once and can be reused across noise realizations and perturbation parameters, reducing the cost of ensemble averages and parameter sweeps.