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arXiv:2006.02583 · Physical Review A

Population transfer via a finite temperature state

Wei Huang, Baohua Zhu, Wei Wu, Shan Yin, Wentao Zhang, Chu Guo

Published Oct 21, 2020• 7 citations
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Abstract

We study quantum population transfer via a common intermediate state initially in thermal equilibrium with a finite temperature $T$, exhibiting a multilevel stimulated Raman adiabatic passage structure. We consider two situations for the common intermediate state, namely a discrete two-level spin and a bosonic continuum. In both cases we show that the finite temperature strongly affects the efficiency of the population transfer. We also show in the discrete case that strong coupling with the intermediate state, or a longer duration of the controlled pulse, would suppress the effect of finite temperature. In the continuous case, we adapt the thermofield-based chain-mapping matrix product states algorithm to study the time evolution of the system plus the continuum under time-dependent controlled pulses, which shows great potential to be used to solve open quantum system problems in quantum optics.

DOI
10.1103/physreva.102.043714

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We study quantum population transfer via a common intermediate state initially in thermal equilibrium with a finite temperature TTT, exhibiting a multilevel stimulated Raman adiabatic passage structure. We consider two situations for the common intermediate state, namely a discrete two-level spin and a bosonic continuum. In both cases we show that the finite temperature strongly affects the efficiency of the population transfer. We also show in the discrete case that strong coupling with the intermediate state, or a longer duration of the controlled pulse, would suppress the effect of finite temperature. In the continuous case, we adapt the thermofield-based chain-mapping matrix product states algorithm to study the time evolution of the system plus the continuum under time-dependent controlled pulses, which shows great potential to be used to solve open quantum system problems in quantum optics.
We propose a model to study quantum population transfer via a structural continuum. The model is composed of two spins which are coupled to two bosonic modes separately by two control pulses, and the two bosonic modes are coupled to a common structural continuum. We show that efficient population transfer can be achieved between the two spins by using a multilevel stimulated Raman adiabatic passage (STIRAP) across the continuum, which we refer to as straddle STIRAP via continuum. We also consider the stability of this model against different control parameters and show that efficient population transfer can be achieved even in the presence of a moderate dissipation.
We consider the optimal control problem of transferring population between states of a quantum system where the coupling proceeds only via intermediate states that are subject to decay. We pose the question whether it is generally possible to carry out this transfer. For a single intermediate decaying state, we recover the stimulated Raman adiabatic passage process, which we identify as the global optimum in the limit of infinite control time. We also present analytical solutions for the case of transfer that has to proceed via two consecutive intermediate decaying states. We show that in this case, for finite power the optimal control does not approach perfect state transfer even in the infinite time limit. We generalize our findings to characterize the topologies of paths that can be achieved by coherent control under the assumption of finite power. If two or more consecutive states in an NNN-level chain are subject to decay, complete population transfer with finite-power controls is not possible.
Abstract Stimulated Raman adiabatic passage is a well-known technique for quantum population transfer due to its robustness again various sources of noises. Here we consider quantum population transfer from one spin to another via an intermediate spin which is under dephasing noise. We obtain an analytic expression for the transfer efficiency under a specific driving protocol, showing that dephasing could reduce the transfer efficiency, but the effect of dephasing could also be suppressed with a stronger laser coupling or a longer laser duration. We also consider another commonly used driving protocol, which shows that this analytic picture is still qualitatively correct.
This work investigates the effect of phonon coupling on the transfer of population and creation of coherence using variant of stimulated Raman adiabatic passage (STIRAP) known as \emph{fractional} stimulated Raman adiabatic passage (FSTIRAP). The study is based on the Liouville equation, which is solved numerically in the adiabatic limit. Although the phonon is assumed to be coupled only to the intermediate state, it is coupled to the other two states by dipolar system-environment interaction, inducing phonon coupling to the other states which are not directly in contact with the phonon. At zero temperature the STIRAP pulse protocol's efficiency of the transfer decreases exponentially with the electron-phonon coupling, until the coupling strength is strong enough to make the process fully incoherent, in which case the population transfer is 13\frac{1}{3}31​ in each level. For the FSTIRAP protocol we find that the transferred population to target state decreases, leaving some population on the intermediate state. Consequently, there is an increase in the magnitude of the coherences ρ01,ρ12ρ_{01}, ρ_{12}ρ01​,ρ12​, albeit small. Furthermore population transfer for non-zero temperature and effect of coupling strength is investigated, it is observed that while both parameters negatively influence the efficiency of transfer the former decrease the transfer exponentially, thereby equilibrating the system fast, while the latter seen to decrease the transfer monotonically, and hence equilibrates slowly.
We propose a technique which produces nearly complete ionization of the population of a discrete state coupled to a continuum by a two-photon transition via a lossy intermediate state whose lifetime is much shorter than the interaction duration. We show that using counterintuitively ordered pulses, as in stimulated Raman adiabatic passage (STIRAP), wherein the pulse coupling the intermediate state to the continuum precedes and partly overlaps the pulse coupling the initial and intermediate states, greatly increases the ionization signal and strongly reduces the population loss due to spontaneous emission through the lossy state. For strong spontaneous emission from that state, however, the ionization is never complete because the dark state required for STIRAP does not exist. We demonstrate that this drawback can be eliminated almost completely by creating a laser-induced continuum structure (LICS) by embedding a third discrete state into the continuum with a third control laser. This LICS introduces some coherence into the continuum, which enables a STIRAP-like population transfer into the continuum. A highly accurate analytic description is developed and numerical results are presented for Gaussian pulse shapes.
We use optimal control in order to find the optimal shapes of pulses maximizing the population transfer between two bound states which are coupled via a continuum of states. We find that the optimal bounded controls acquire the bang-interior and interior-bang form, with the bang part corresponding to the maximum allowed control value and the interior part to values between zero and the maximum. Then we use numerical optimal control to obtain the switching times and the interior control values. We compare our results with those obtained using Gaussian stimulated Raman adiabatic passage pulses and find that the optimal method performs better, with the extent of improvement depending on the effective two-photon detuning and the size of incoherent losses. When we consider effective two-photon resonance, the improvement is more dramatic for larger incoherent losses, while when we take into account the effective two-photon detuning, the improvement is better for smaller incoherent losses. We also obtain how the transfer efficiency increases with increasing absolute value of the Fano factor. The present work is expected to find application in areas where the population transfer between two bound states through a continuum structure plays an important role, for example coherence effects, like population trapping and electromagnetically induced transparency, optical analogs for light waves propagating in waveguide-based photonic structures, and qubits coupled via a continuum of bosonic or waveguide modes.