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arXiv:1004.4050 · Physical Review A

Controllability on relaxation-free subspaces: On the relationship between adiabatic population transfer and optimal control

Haidong Yuan, Christiane P. Koch, Peter Salamon, David J. Tannor

Published Mar 15, 2012• 27 citations
arXivHTMLPDF

Abstract

We consider the optimal control problem of transferring population between states of a quantum system where the coupling proceeds only via intermediate states that are subject to decay. We pose the question whether it is generally possible to carry out this transfer. For a single intermediate decaying state, we recover the stimulated Raman adiabatic passage process, which we identify as the global optimum in the limit of infinite control time. We also present analytical solutions for the case of transfer that has to proceed via two consecutive intermediate decaying states. We show that in this case, for finite power the optimal control does not approach perfect state transfer even in the infinite time limit. We generalize our findings to characterize the topologies of paths that can be achieved by coherent control under the assumption of finite power. If two or more consecutive states in an $N$-level chain are subject to decay, complete population transfer with finite-power controls is not possible.

DOI
10.1103/physreva.85.033417

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The stimulated Raman adiabatic passage shows an efficient technique that accurately transfers population between two discrete quantum states with the same parity in three-level quantum systems based on adiabatic evolution. This technique has widely theoretical and experimental applications in many fields of physics, chemistry, and beyond. Here, we present a general approach to robust stimulated Raman shortcut-to-adiabatic passage with invariant-based optimal control. By controlling the dynamical process, we inversely design a family of Hamiltonians with non-divergent Rabi frequencies that can realize fast and accurate population transfer from the first to the third level, while the systematic errors are largely suppressed in general. Furthermore, a detailed trade-off relation between the population of the intermediate state and the amplitudes of Rabi frequencies in the transfer process is illustrated. These results provide an optimal route toward manipulating the evolution of three-level quantum systems in future quantum information processing.
We study quantum population transfer via a common intermediate state initially in thermal equilibrium with a finite temperature TTT, exhibiting a multilevel stimulated Raman adiabatic passage structure. We consider two situations for the common intermediate state, namely a discrete two-level spin and a bosonic continuum. In both cases we show that the finite temperature strongly affects the efficiency of the population transfer. We also show in the discrete case that strong coupling with the intermediate state, or a longer duration of the controlled pulse, would suppress the effect of finite temperature. In the continuous case, we adapt the thermofield-based chain-mapping matrix product states algorithm to study the time evolution of the system plus the continuum under time-dependent controlled pulses, which shows great potential to be used to solve open quantum system problems in quantum optics.
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The stimulated Raman adiabatic passage (STIRAP) shows an efficient technique that accurately transfers population between two discrete quantum states with the same parity, in three-level quantum systems based on adiabatic evolution. This technique has widely theoretical and experimental applications in many fields of physics, chemistry, and beyond. Here, we present a generally robust approach to speed up STIRAP with invariant-based shortcut to adiabaticity. By controlling the dynamical process, we inversely design a family of Hamiltonians that can realize fast and accurate population transfer from the first to the third level, while the systematic error is largely suppressed in general. Furthermore, a detailed trade-off relation between the population of the intermediate state and the amplitudes of Rabi frequencies in the transfer process is illustrated. These results provide an optimal route toward manipulating the evolution of three-level quantum systems in future quantum information processing.
We use optimal control theory to obtain shortcuts to adiabaticity which maximize population transfer in a three-level stimulated Raman adiabatic passage system, for a given finite duration of the process and a specified dissipation rate at the intermediate state. We fix the sum of the intensities of the pump and Stokes pulses and use the mixing angle of the fields as the sole control variable. We determine the optimal variation of this angle and reveal the role of the singular arc in the optimal trajectory, in order to minimize the effect of dissipation. This article is part of the theme issue 'Shortcuts to adiabaticity: theoretical, experimental and interdisciplinary perspectives'.