The time-frequency degree of freedom of the electromagnetic field is the final frontier for single-photon measurements. The temporal and spectral distribution a measurement retrodicts (that is, the state it projects onto) is determined by the detector's intrinsic resonance structure. In this paper, we construct ideal and more realistic positive operator-valued measures (POVMs) that project onto arbitrary single-photon wave packets with high efficiency and low noise. We discuss applications to super-resolved measurements and quantum communication. In doing so we will give a fully quantum description of the entire photodetection process, give prescriptions for (in principle) performing single-shot Heisenberg-limited time-frequency measurements of single photons, and discuss fundamental limits and trade-offs inherent to single-photon detection.
The time-frequency degree of freedom of the electromagnetic field is the final frontier for single-photon measurements. The temporal and spectral distribution a measurement retrodicts (that is, the state it projects onto) is determined by the detector's intrinsic resonance structure. In this paper, we construct ideal and more realistic positive operator-valued measures (POVMs) that project onto arbitrary single-photon wave packets with high efficiency and low noise. We discuss applications to super-resolved measurements and quantum communication. In doing so we will give a fully quantum description of the entire photodetection process, give prescriptions for (in principle) performing single-shot Heisenberg-limited time-frequency measurements of single photons, and discuss fundamental limits and trade-offs inherent to single-photon detection.
Quantum mechanics cements the intimate relationship between the nature of light and its detection. Historically, quantum theories of photodetection have generally fallen into two categories: the first tries to determine what quantum field observable is measured when photoelectrons are detected, laying the theoretical groundwork for photodetection being possible. The second type are phenomenological theories, which take great care to model the details of specific photodetectors. In this dissertation, we fill in the gap between these two models in the modern literature on photodetection by constructing a fully quantum-mechanical and sufficiently realistic model that includes all stages of the photodetection process. We accomplish this within the framework of quantum information theory using the language of positive operator valued measures (POVMs). \n\nA POVM provides the most general description of a quantum measurement. In the context of single-photon detection, the photodetector POVM provides a complete characterization of the single-photon detector (SPD) from which all figures of merit can be calculated. Each element of the POVM is comprised of a weighted sum over single-photon state projectors. To construct SPD POVMs, we identify the states projected onto by a measurement and the associated weights. We first accomplish this for a simple time-dependent system, laying out how to efficiently project onto arbitrary single-photon states. Then, we describe the three stages of a realistic SPD: transmission, amplification, and measurement.\n\nIn the transmission stage of photodetection a photon enters a network of discrete energy levels, its energy propagating through that network and finally exiting into another output continuum of modes, a process entirely described by a single complex function. In the amplification stage of photodetection, a single excitation is amplified into a macroscopic signal via a nonlinear amplification mechanism. In the final stage, an inefficient ``classical'' measurement is made on the macroscopic signal. By combining these three stages we form a chain of inference from the final ``click'' to the input photon and construct a POVM projecting onto the input Hilbert space. Lastly, we discuss limits and tradeoffs that arise at each stage and implications for photodetection applications.\n\nThis dissertation contains previously published and unpublished material.
Quantum mechanics cements the intimate relationship between the nature of light and its detection. Historically, quantum theories of photodetection have generally fallen into two categories: the first tries to determine what quantum field observable is measured when photoelectrons are detected, laying the theoretical groundwork for photodetection being possible. The second type are phenomenological theories, which take great care to model the details of specific photodetectors. In this dissertation, we fill in the gap between these two models in the modern literature on photodetection by constructing a fully quantum mechanical and sufficiently realistic model that includes all stages of the photodetection process: transmission, amplification, and a final classical measurement. We accomplish this within the framework of quantum information theory using the language of positive operator valued measures (POVMs). This dissertation contains material previously published in three papers: Propp, Tz. B & van Enk, S. J. (2019). On nonlinear amplification: improved quantum limits for photon counting. Optics Express 27, 16, 23454-23463. Propp, Tz. B & van Enk, S. J. (2019). Quantum networks for single photon detection. Physical Review A, 100, 033836. Propp, Tz. B & van Enk, S. J. (2020). How to project onto an arbitrary single-photon wavepacket. Physical Review A, 102, 053707.
Suppose we measure the time-dependent spectrum of a single photon. That is, we first send the photon through a set of frequency filters (which we assume to have different filter frequencies but the same finite bandwidth $\mathrm{\ensuremath{\Gamma}}$) and then record at what time (with some finite precision $\mathrm{\ensuremath{\Delta}}t$ and some finite efficiency $\ensuremath{\eta}$) and after passing what filter the photon is detected. What is the positive-operator-valued measure (POVM), the most general description of a quantum measurement, corresponding to such a measurement? We show how to construct the POVM in various cases, with special interest in the case $\mathrm{\ensuremath{\Gamma}}\mathrm{\ensuremath{\Delta}}t\ensuremath{\ll}1$ (time-frequency uncertainty still holds, even in that limit). One application of the formalism is to heralding single photons. We also find a Hong-Ou-Mandel type of interference effect with two photons entering a frequency filter.
We propose a procedure for defining all single-photon observables in terms of Positive-Operator Valued Measures (POVMs), in particular spin and position. We identify the suppression of 0-helicity photon states as a projection from an extended Hilbert space onto the photon Hilbert space. We show that all single-photon observables are in general described by POVMs, obtained by applying this projection to opportune Projection-Valued Measures (PVMs), defined on the extended Hilbert space. The POVMs associated to momentum and helicity reduce to PVMs, unlike those associated to position and spin, this fact reflecting the intrinsic unsharpness of these observables. We finally extensively study the preparation uncertainty relations for position and momentum and the probability distribution of spin, exploring single photon Gaussian states for several choices of spin and polarization.
We present a method for measuring quantum states encoded in the temporal modes of photons. The basis for the multilevel quantum states is defined by the use of modes propagating in a dispersive medium, which is a fiber in this case. The propagation and time-resolved single-photon detection allow us to define a positive-operator valued measure (POVM). The POVM depends on the amount of dispersion and the characteristics of a detector. This framework is numerically tested by performing quantum state tomography on a large number of states for a set of realistic experimental settings. Finally, the average fidelity between the expected and reconstructed states is computed for qubits, qutrits, and entangled qubits.
Photon counting is a cornerstone of quantum optics. Here, we demonstrate precisely counting from 0 to over 9000 photons, beating the Poisson noise limit by at least 4.1dB across this range. We achieve sub-single-photon precision up to 276 photons per pulse. To do so, we multiplex eight intrinsically photon-number-resolving superconducting nanowire single-photon detectors across 128 temporal modes. We use a model-informed characterization of each of the 1024 detection bins, for optimal precision. We perform quantum detector tomography to reconstruct the positive operator valued measures (POVMs) of the complete device, which consists of 1.38⋅108 matrix elements. At the repetition rate of our experiment of 80kHz, we can precisely count photons corresponding to an optical power of approximately 71pW, bridging the gap from single-photon measurements to high-sensitivity optical power meters. A photon-number-resolving detector of this size, and the tools used to analyze it, will become increasingly important to characterize large quantum states, as well as tasks in precision metrology and optical power standards.