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arXiv:2004.11885 · Physical Review A

Tuning photon statistics with coherent fields

Eduardo Zubizarreta Casalengua, Juan Camilo López Carreño, Fabrice P. Laussy, Elena del Valle

Published Jun 18, 2020• 35 citations
arXivHTMLPDF

Abstract

Photon correlations, as measured by Glauber's $n\mathrm{th}$-order coherence functions ${g}^{(n)}$, are highly sought to be minimized and/or maximized. In systems that are coherently driven, so-called blockades can give rise to strong correlations according to two scenarios based on level repulsion (conventional blockade) or interferences (unconventional blockade). Here, we show how these two approaches relate to the admixing of a coherent state with a quantum state such as a squeezed state for the simplest and most recurrent case. The emission from a variety of systems, such as resonance fluorescence, the Jaynes-Cummings model, or microcavity polaritons, as a few examples of a large family of quantum optical sources, are shown to be particular cases of such admixtures, that can further be doctored up externally by adding an amplitude- and phase-controlled coherent field with the effect of tuning the photon statistics from exactly zero to infinity. We show how such an understanding also allows to classify photon statistics throughout platforms according to conventional and unconventional features, with the effect of optimizing the correlations and with possible spectroscopic applications. In particular, we show how configurations that can realize simultaneously conventional and unconventional antibunching bring the best of both worlds: huge antibunching (unconventional) with large populations and being robust to dephasing (conventional).

DOI
10.1103/physreva.101.063824

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Photon correlations, as measured by Glauber's nthn\mathrm{th}nth-order coherence functions g(n){g}^{(n)}g(n), are highly sought to be minimized and/or maximized. In systems that are coherently driven, so-called blockades can give rise to strong correlations according to two scenarios based on level repulsion (conventional blockade) or interferences (unconventional blockade). Here, we show how these two approaches relate to the admixing of a coherent state with a quantum state such as a squeezed state for the simplest and most recurrent case. The emission from a variety of systems, such as resonance fluorescence, the Jaynes-Cummings model, or microcavity polaritons, as a few examples of a large family of quantum optical sources, are shown to be particular cases of such admixtures, that can further be doctored up externally by adding an amplitude- and phase-controlled coherent field with the effect of tuning the photon statistics from exactly zero to infinity. We show how such an understanding also allows to classify photon statistics throughout platforms according to conventional and unconventional features, with the effect of optimizing the correlations and with possible spectroscopic applications. In particular, we show how configurations that can realize simultaneously conventional and unconventional antibunching bring the best of both worlds: huge antibunching (unconventional) with large populations and being robust to dephasing (conventional).
Abstract The photon statistics emitted by a large variety of light‐matter systems under weak coherent driving can be understood, to lowest order in the driving, in the framework of an admixture of (or interference between) a squeezed state and a coherent state, with the resulting state accounting for all bunching and antibunching features. One can further identify two mechanisms that produce resonances for the photon correlations: i) conventional photon blockade describes cases that involve a particular quantum level or set of levels in the excitation/emission processes with interferences occurring to all orders in the photon numbers, while ii) unconventional photon blockade describes cases where the driving laser is far from resonance with any level and the interference occurs for a particular number of photons only, yielding stronger correlations but only for a definite number of photons. Such an understanding and classification allows for a comprehensive and transparent description of the photon statistics from a wide range of disparate systems, where optimum conditions for various types of photon correlations can be found and realized.
Photon antibunching is a quantum phenomenon typically observed in strongly nonlinear systems where photon blockade suppresses the probability of detecting two photons at the same time. Antibunching has also been reported with Gaussian states, where optimized amplitude squeezing yields classically forbidden values of the intensity correlation, g(2)(0)<1{g}^{(2)}(0)<1g(2)(0)<1. As a consequence, observation of antibunching is not necessarily a signature of photon-photon interactions. To clarify the significance of the intensity correlations, we derive a sufficient condition for deducing whether a field is non-Gaussian based on a g(2)(0){g}^{(2)}(0)g(2)(0) measurement. We then show that the Gaussian antibunching obtained with a degenerate parametric amplifier is close to the ideal case reached using dissipative squeezing protocols. We finally shed light on the so-called unconventional photon blockade effect predicted in a driven two-cavity setup with surprisingly weak Kerr nonlinearities, stressing that it is a particular realization of optimized Gaussian amplitude squeezing.
Similar to interferences in classical optics that can combine two waves to produce no output or more output than input, multiphoton interferences can produce, for instance, anti-bunched light by admixing squeezed (bunched) and laser (uncorrelated) light. The general case of quantum-field interferences, that can be self- or externally realized in coherently driven quantum sources, leads to a classification of conventional and unconventional photon statistics, as discussed by Elena del Valle and co-workers in article number 1900279.
Photon blockades are traditionally classified into conventional and unconventional types, depending on distinct physical mechanisms. Regarding the cavity decay rate κ, the conventional photon blockade takes place under strong nonlinearity condition (g>κ), whereas the unconventional photon blockade occurs in the regime of weak nonlinearity (g<κ). We here propose how to derive an optimal condition for photon blockade utilizing a two-photon Jaynes-Cummings model. Under this condition, the equal-time second-order correlation function reaches its minimum, leading to photon antibunching in both conventional and unconventional photon blockade regimes (g>κ and g<κ), even in g∼κ. This characteristic is termed universal photon blockade. By comparing it with the conventional and the unconventional photon blockades in the weak-driving limit, the advantages of universal photon blockade are revealed. Our proposal paves an avenue towards the future study of photon blockades and has potential applications in generating antibunched photons.
The photon blockade phenomenon, a promising tool for realizing efficient single-photon sources, is the central focus of our work. We study this phenomenon within the context of the multimode extension of the Jaynes-Cummings model, incorporating two-photon dissipation and external coherent driving. Operating in the weak-driving regime, we confine our analysis to the two-excitation sector of the Hilbert space, initially exploring the single-mode case and then focusing on the corresponding multimode problem. Our study calculates the second-order correlation function (both numerically and analytically) for zero- and nonzero time delays in single- and multimode cases, to pinpoint and validate the conditions that lead to conventional and unconventional photon blockade. Our zero delay findings reveal that photon antibunching is comparable in both cases; however, the multimode case offers a greater degree of control and applicability. Furthermore, for non-zero delay operation, we find that when one of the multiple modes is set at the optimal conventional photon blockade conditions, the behavior of the curve mimics the single-mode problem with an overall slower rate of reaching the g(2)(τ)=1g^{(2)}(τ)=1g(2)(τ)=1 value. These results highlight the practical implications of our findings for building useful single-photon sources.
Herein, we propose a coupled Jaynes-Cummings model for the preparation of strong antibunched single photons and antibunched correlated photon pairs. Using the effective Hamiltonian method, we obtained the expression for the correlation function and then presented the optimal conditions for conventional/unconventional photon blockade. The results showed that on one hand, an intersection point exists between conventional photon blockade and unconventional photon blockade and that the performance of the single photon at the intersection point is better. On the other hand, under the condition of unconventional photon blockade, the photons produced by each Jaynes-Cummings system are strongly correlated with each other.