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arXiv:2004.01948

Time development of a driven three-level lambda system: A case study

James P. Lavine

Published Apr 4, 2020• 0 citations
arXivHTMLPDF

Abstract

How does a driven system with many energy levels approach its steady state? Insights are gained by studying a system with three energy levels when the ground state is excited by a laser. The time-dependent occupation probabilities of the three energy levels show students how the system develops in time. The occupation probabilities come from the numerical solution of the Liouville-von Neumann equations for the density operator matrix elements when relaxation is included. A combination of the Interaction Picture, the Rotating Wave Approximation, and the assumption of resonance permit the eigenvalues of the Liouville-von Neumann equations to be found numerically and in closed-form in certain limits. The two methods are complementary and help students understand time-dependent systems. In addition, the eigenvalues allow the short-time and the long-time occupation probabilities to be connected to the relaxation parameters and the magnitude of the laser's electric field. Thus, this model three-level system illuminates how a driven system behaves over time and provides guidance for students studying time-dependent systems.

DOI
10.48550/arxiv.2004.01948

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How does a driven system with many energy levels approach its steady state? Insights are gained by studying a system with three energy levels when the ground state is excited by a laser. The time-dependent occupation probabilities of the three energy levels show students how the system develops in time. The occupation probabilities come from the numerical solution of the Liouville-von Neumann equations for the density operator matrix elements when relaxation is included. A combination of the Interaction Picture, the Rotating Wave Approximation, and the assumption of resonance permit the eigenvalues of the Liouville-von Neumann equations to be found numerically and in closed-form in certain limits. The two methods are complementary and help students understand time-dependent systems. In addition, the eigenvalues allow the short-time and the long-time occupation probabilities to be connected to the relaxation parameters and the magnitude of the laser's electric field. Thus, this model three-level system illuminates how a driven system behaves over time and provides guidance for students studying time-dependent systems.
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Summary form only given.A three-level atom in the V-configuration is treated under two coherent laser fields at resonance with the two allowed transitions. The master equation for the system and full quantum mechanical Hamiltonian are derived, and equations of motion for the elements of the density matrix are obtained by projecting into the bare- and dressed-states schemes. Analysis of light amplification without population inversion in this V-type system is accomplished within the framework of the dressed-state basis. The physical content of the equations of motion for the density matrix elements, namely the coherences and the populations is provided by identifying effective decay and relaxation rates and gain/absorption constants with the appropriate composite coefficients. These depend on the Rabi frequencies of both the drive and probe coherent fields. Time-dependent solutions for both the coherences and the populations are obtained both numerically and analytically under the secular approximation. We have shown how to construct these analytical approximate time-dependent solutions for dressed-state populations and coherences. These approximate solutions, as well as the full numerical calculation quantities, exhibit oscillations at the generalized Rabi frequency.
We show that the time-averaged density matrix which involves the solution of any Liouville equation with a specified initial condition is also the steady-state solution of an appropriately constructed Bloch equation taken in the weak-damping limit. This leads to new explicit expressions for the time-averaged density matrix which, unlike expressions in general use, give a completely analytic relation between the time average and the initial condition and contain no numerically determined eigenvector components. We apply this approach to driven multilevel systems to find new expressions for the time-averaged level populations in a three-level system. A strong initial-condition dependence is exhibited even for an equally spaced resonantly driven system. Analytic forms specifically showing a Stark-shifted multiphoton resonance and the associated line shape are also derived.
For an atom or molecule in which two transitions are driven by laser beams, a three-state model is used. Transitions among the three states are caused only by the oscillating electric fields of the laser beams. The amplitudes and detunings of the two laser beams, which are various functions of the time, appear in the Schrödinger equation for the atom or molecule. In certain cases, the Schrödinger equation can be solved analytically, to find transition probabilities and the probability of no transition. This is done by using Clausen’s special function, or by assuming that the sum of the two detunings is zero at all times. Conditions for complete transfer of the population from the ground state to an excited state are obtained from the analytic solutions.
We study the dynamics of three-level $\ensuremath{\Lambda}$-type atoms driven by a coherent train of short, nonoverlapping laser pulses. We derive analytical nonperturbative expressions for the density matrix by approximating the pulses by a $\ensuremath{\delta}$ function. We demonstrate that, depending on the train parameters, several scenarios of system dynamics can be realized. We show the possibility of driving Raman transitions between the two ground states of the $\ensuremath{\Lambda}$ system, avoiding populating excited states by using pulses with effective area equal to $2\ensuremath{\pi}$. The number of $2\ensuremath{\pi}$ pulses needed to transfer the entire population from one ground state to another depends on the ratio between the Rabi frequencies of two allowed transitions. In the case of equal Rabi frequencies, the system can be transferred from one ground state to another with a single $2\ensuremath{\pi}$ pulse. When the total pulse area differs from $2\ensuremath{\pi}$ and the two-photon resonance condition is fulfilled, the system evolves into a ``dark'' state and becomes transparent to subsequent pulses. The third possible scenario is the quasi-steady-state regime when neither the total single-pulse area is equal to $2\ensuremath{\pi}$ nor is the two-photon resonance condition fulfilled. In this regime the radiative-decay-induced drop in the population following a given pulse is fully restored by the subsequent pulse. We derive an analytical expression for the density matrix in the quasi-steady-state regime. We analyze the dependence of the postpulse excited-state population in the quasi-steady-state regime on the train parameters. We find the optimal values for the train parameters corresponding to the maximum of the excited-state population. The maximum of the excited-state population in the steady-state regime is reached at an effective single-pulse area equal to $\ensuremath{\pi}$ and is equal to 2/32/32/3 in the limiting case when its radiative lifetime is much shorter than the pulse repetition period.
Dissipation and decoherence, and the evolution from pure to mixed states in quantum physics, are handled through master equations for the density matrix. Master equations such as the Lindblad equation preserve the trace of this matrix. Viewing them as first-order time-dependent operator equations for the elements of the density matrix, a unitary integration procedure can be adapted to solve for these elements. A simple model for decoherence preserves the Hermiticity of the density matrix. A single, classical Riccati equation is the only one requiring numerical handling to obtain a full solution of the quantum evolution. The procedure is general, valid for any number of levels, but is illustrated here for a three-level system with two driving fields. For various choices of the initial state, we study the evolution of the system as a function of the amplitudes, relative frequencies, and phases of the driven fields and of the strength of the decoherence. The monotonic growth of the entropy is followed as the system evolves from a pure to a mixed state. An example is provided by the n=3n=3n=3 states of the hydrogen atom in a time-dependent electric field, such degenerate manifolds affording an analytical solution.