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arXiv:2003.09885 · Physical Review A

Dynamics of Rydberg excitations and quantum correlations in an atomic array coupled to a photonic crystal waveguide

Yashwant Chougale, Jugal Talukdar, Tomás Ramos, Rejish Nath

Published Aug 25, 2020• 19 citations
arXivHTMLPDF

Abstract

We study the dynamics of up to two Rydberg excitations and the correlation growth in a chain of atoms coupled to a photonic crystal waveguide. In this setup, an excitation can hop from one atom to another via exponentially decaying exchange interactions mediated by the waveguide. An initially localized excitation undergoes a continuous-time quantum walk for short-range hopping, and for long-range hopping, it experiences quasilocalization. In addition, the inverse participation ratio reveals a superballistic diffusion of the excitation in short times, whereas, at a long time, it becomes ballistic. For two initially localized excitations, intriguing and complex dynamical scenarios emerge for different initial separations due to the competition between the Rydberg-Rydberg and exchange interactions. In particular, the two-point correlation reveals a light-cone behavior even for sufficiently long-range exchange interactions. Additionally, we characterize the growth of bipartite entanglement entropy, which exhibits a global bound if only one excitation is present in the dynamics. Finally, we analyze the effect of imperfections due to spontaneous emission from the Rydberg state into photons outside the waveguide and show that all of the physical phenomena we predict are well within experimental reach.

DOI
10.1103/physreva.102.022816

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We study the dynamics of up to two Rydberg excitations and the correlation growth in a chain of atoms coupled to a photonic crystal waveguide. In this setup, an excitation can hop from one atom to another via exponentially decaying exchange interactions mediated by the waveguide. An initially localized excitation undergoes a continuous-time quantum walk for short-range hopping, and for long-range hopping, it experiences quasilocalization. In addition, the inverse participation ratio reveals a superballistic diffusion of the excitation in short times, whereas, at a long time, it becomes ballistic. For two initially localized excitations, intriguing and complex dynamical scenarios emerge for different initial separations due to the competition between the Rydberg-Rydberg and exchange interactions. In particular, the two-point correlation reveals a light-cone behavior even for sufficiently long-range exchange interactions. Additionally, we characterize the growth of bipartite entanglement entropy, which exhibits a global bound if only one excitation is present in the dynamics. Finally, we analyze the effect of imperfections due to spontaneous emission from the Rydberg state into photons outside the waveguide and show that all of the physical phenomena we predict are well within experimental reach.
Giant atoms are attracting interest as an emerging paradigm in the quantum optics of engineered waveguides. Here we propose to realize a synthetic giant atom working in the optical regime starting from a pair of interacting Rydberg atoms driven by a coherent field and coupled to a photonic crystal waveguide. Giant-atom effects can be observed as a phase-dependent decay of the double Rydberg excitation during the initial evolution of this atomic pair while (internal) atomic entanglement is exhibited at later times. Such an intriguing entanglement onset occurs in the presence of intrinsic atomic decay toward non-guided vacuum modes and is accompanied by an anti-bunching correlation of the emitted photons. Our findings may be relevant to quantum information processing, besides broadening the giant-atom waveguide physics with optically driven natural atoms.
Abstract We study the population dynamics in a two-atom setup in which each atom is driven independently by different light fields, but coupling the same Rydberg state. In particular, we look at how an offset in the Rabi frequencies between two atoms affects the dynamics. We find novel features such as amplifying the Rabi frequency of one atom, together with strong Rydberg-Rydberg interactions freezes the dynamics in the second atom. We analyze this Rydberg-biased freezing phenomenon in detail, with effective Hamiltonians obtained for various limits of the system parameters. In the absence of Rabi-offset, the doubly excited state population exhibits a Lorentzian profile as a function of interaction, whereas for very small offsets it shows splitting and thus peaks. Using an effective Hamiltonian, as well as the perturbation theory in the weak interaction limit, we show that the peak arises from a competition between Rabi-offset and Rydberg-Rydberg interactions when both are sufficiently small, together with the Rydberg blockade at large interactions. The effective Hamiltonians provide us with analytical results for long time dynamics, which are in an excellent agreement with exact numerical solutions. Also, we analyze the growth and the dynamics of quantum correlations such as entanglement entropy/quantum discord for the coherent dynamics. Finally, we extend our studies to the dissipative case in which the spontaneous emission from the Rydberg state is taken into account and in particular, we look at how the Rabi-offset modifies the purity and quantum discord in the steady states. We conclude that the local manipulation of an atom by introducing a Rabi-offset can be a useful tool to control the quantum correlations and in general, the quantum states of the composite two-qubit systems.
The atom-waveguide interface mediates significant and long-range light-matter interactions through guided modes. In this one-dimensional system, we theoretically investigate the excitation localization of multiple atomic excitations under strong position disorder. Deep in the localization side, we obtain the time evolutions of quantum correlations via Kubo cumulant expansions, which arise initially and become finite and leveled afterward, overtaking those without disorder. This indicates two distinct regimes in time: before the onset of excitation localization, the disorder engage the disturbance of quantum correlations, which is followed by disorder-assisted buildup of quantum correlations that maintain at a later stage owing to the absence of excitations diffusion. The crossing of distinct regimes is pushed further in time for longer-range correlations, which indicates a characteristic timescale needed for disorder to sustain them. We also explore the effect of directionality of couplings and resonant dipole-dipole interactions, which can drive the system toward the delocalized side when it is under chiral couplings or large dipole-dipole interaction strengths. The time-evolved quantum correlations can give insights into the studies of few-body localization phenomenon and nonequilibrium dynamics in open quantum systems.
An atomic array coupled to a one-dimensional nanophotonic waveguide allows photon-mediated dipole-dipole interactions and nonreciprocal decay channels. Such an array possesses many intriguing quantum phenomena due to its distinctive and emergent quantum correlations. In this atom-waveguide quantum system, we theoretically investigate the atomic excitation dynamics and its transport property, specifically at an interface of dissimilar atomic arrays with different interparticle distances. We find that the atomic excitation dynamics is highly dependent on the interparticle distances of dissimilar arrays and the directionality of nonreciprocal couplings. By tuning these parameters, a dominant excitation reflection can be achieved at the interface of the arrays in the single excitation case. We further study two effects on the transport property—of external drive and of single excitation delocalization over multiple atoms—where we manifest a rich interplay between multisite excitation and the relative phase in determining the transport properties. Finally, we present an intriguing trapping effect of atomic excitation by designing multiple zones of dissimilar arrays. Similar to the single excitations, multiple excitations are reflected from the array interfaces and trapped as well, although complete trapping of many excitations together is relatively challenging at long time due to a faster combined decay rate. Our results can provide insights into nonequilibrium quantum dynamics in dissimilar arrays, and they can shed light on confining and controlling quantum registers useful for quantum information processing. Published by the American Physical Society 2024
Quantum correlations are essential to the emergent behaviors of quantum systems, supporting key phenomena such as localization or delocalization of particles, quantum avalanches in many-body localized systems, and quantum information transfer. In open atom-nanophotonic systems characterized by long-range spin-exchange interactions, we examine the influence of clean system size on high-order quantum correlations among a clean-disordered atomic array with multiple atomic excitations. By initializing the system far from equilibrium, we observe a suppression of quantum correlations for localized atomic excitations in the disordered zone as the clean system size increases, showcasing the delocalization behavior in the high-order spin-exchange processes. The calculation of the entanglement entropy at the interface further substantiates this thermalizing effect. Our results manifest distinct quantum correlations enabled by long-range interactions mediated by the waveguide, enhance the theoretical comprehension of clean-disordered systems, and provide insights to nonequilibrium quantum dynamics in an atom-nanophotonic platform.
We investigate the transport of excitations through a chain of atoms with nonlocal dissipation introduced through coupling to additional short-lived states. The system is described by an effective spin-1/2 model where the ratio of the exchange interaction strength to the reservoir coupling strength determines the type of transport, including coherent exciton motion, incoherent hopping, and a regime in which an emergent length scale leads to a preferred hopping distance far beyond nearest neighbors. For multiple impurities, the dissipation gives rise to strong nearest-neighbor correlations and entanglement. These results highlight the importance of nontrivial dissipation, correlations, and many-body effects in recent experiments on the dipole-mediated transport of Rydberg excitations.