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arXiv:2003.09060 · Journal of the Optical Society of America B

VECSEL systems for quantum information processing with trapped beryllium ions

S. C. Burd, Jussi-Pekka Penttinen, Pan‐Yu Hou, H. M. Knaack, Sanna Ranta, Mika Maki, Emmi L. Kantola, Mircea D. Guina, D. H. Slichter, Dietrich G. Leibfried, A. C. Wilson

Published Nov 29, 2022• 16 citations
arXivHTMLPDF

Abstract

We demonstrate two systems based on vertical-external-cavity surface-emitting lasers (VECSELs) for producing ultraviolet laser light at wavelengths of 235 and 313 nm. The systems are suitable for quantum information processing with trapped beryllium ions. Each system consists of a compact, single-frequency, continuous-wave VECSEL producing high-power near-infrared light, tunable over tens of nanometers. One system generates 2.4 W at 940 nm, using a gain mirror based on GaInAs/GaAs quantum wells, which is converted to 54 mW of 235 nm light for photoionization of neutral beryllium atoms. The other system uses a gain mirror based on GaInNAs/GaAs quantum wells, enabling wavelength extension above 1200 nm with manageable strain in the GaAs lattice. This system generates 1.6 W at 1252 nm, which is converted to 41 mW of 313 nm light that is used to laser cool trapped 9Be+ ions and quantum state preparation and detection. The 313 nm system is also suitable for implementing high-fidelity quantum gates.

DOI
10.1364/josab.475467

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APL Photonics•Feb 1, 2026•0 citations
We demonstrate two systems based on vertical-external-cavity surface-emitting lasers (VECSELs) for producing ultraviolet laser light at wavelengths of 235 and 313 nm. The systems are suitable for quantum information processing with trapped beryllium ions. Each system consists of a compact, single-frequency, continuous-wave VECSEL producing high-power near-infrared light, tunable over tens of nanometers. One system generates 2.4 W at 940 nm, using a gain mirror based on GaInAs/GaAs quantum wells, which is converted to 54 mW of 235 nm light for photoionization of neutral beryllium atoms. The other system uses a gain mirror based on GaInNAs/GaAs quantum wells, enabling wavelength extension above 1200 nm with manageable strain in the GaAs lattice. This system generates 1.6 W at 1252 nm, which is converted to 41 mW of 313 nm light that is used to laser cool trapped 9Be+ ions and quantum state preparation and detection. The 313 nm system is also suitable for implementing high-fidelity quantum gates.
Experiments in atomic, molecular, and optical (AMO) physics rely on lasers at many different wavelengths and with varying requirements on spectral linewidth, power, and intensity stability. Vertical external-cavity surface-emitting lasers (VECSELs), when combined with nonlinear frequency conversion, can potentially replace many of the laser systems currently in use. Here we present and characterize VECSEL systems that can perform all laser-based tasks for quantum information processing experiments with trapped magnesium ions. For photoionization of neutral magnesium, 570.6 \,nm light is generated with an intracavity frequency-doubled VECSEL containing a lithium triborate (LBO) crystal for second harmonic generation. External frequency doubling produces 285.3 \,nm light for resonant interaction with the 1S0↔^{1}S_{0}\leftrightarrow1S0​↔ 1P1^{1}P_{1}1P1​ transition of neutral Mg. Using an externally frequency-quadrupled VECSEL, we implement Doppler cooling of 25^{25}25Mg+^{+}+ on the 279.6 \,nm 2S1/2↔^{2}S_{1/2}\leftrightarrow2S1/2​↔ 2P3/2^{2}P_{3/2}2P3/2​ cycling transition, repumping on the 280.4 \,nm 2S1/2↔^{2}S_{1/2}\leftrightarrow2S1/2​↔ 2P1/2^{2}P_{1/2}2P1/2​ transition, coherent state manipulation, and resolved sideband cooling close to the motional ground state. Our systems serve as prototypes for applications in AMO requiring single-frequency, power-scalable laser sources at multiple wavelengths.
We generate coherent ultraviolet radiation at 313 nm as the third harmonic of an external-cavity diode laser. We use this radiation for laser cooling of trapped beryllium atomic ions and sympathetic cooling of co-trapped beryllium-hydride molecular ions. An LBO crystal in an enhancement cavity generates the second harmonic, and a BBO crystal in a doubly resonant enhancement cavity mixes this second harmonic with the fundamental to produce the third harmonic. Each enhancement cavity is preceded by a tapered amplifier to increase the fundamental light. The 36-mW output power of this all-semiconductor-gain system will enable quantum control of the beryllium ions' motion.
Quantum information processing (QIP) approach based on trapped ions is a promising technology that exploits different ion species as individual qubits and qubit gates, while featuring long coherence times, high fidelity of operations, fast readout, and ion-ion gate entanglement. The practical usefulness of trapped-ion quantum computer depends on its further scaling to a large number of qubits. Meanwhile, trapped-ion quantum computer relies on a set of single-frequency lasers, utilizing them for different functions such as photoionization, atom cooling, optical pumping and qubit operations. Thus, a combination of narrow linewidth lasers is required, with the emission wavelengths precisely defined by the corresponding electronic transitions of the selected ion species. Further development, scalability and commercialization of quantum information technologies is interwind with the availability of affordable and robust single-frequency lasers on a variety of application-specific wavelengths. QIP manifests strict requirements posed to lasers in terms of central wavelength, linewidth, long-term stability, beam quality, polarization extinction ratio, side-mode suppression ratio, etc. In this work we present the development and characterization of multiwavelength narrow linewidth system designed for the Ba+ trapped ion computing. The laser system emits single-frequency, sub-MHz emission at 553 nm, 493 nm and 614 nm based on second-harmonic generation of two separate semiconductor laser platforms. Two-step photoionization of neutral Ba is implemented resonantly through 6s2 1S0 → 6s6p 1P1 transition corresponding to 553 nm wavelength, whereas Ba ion is Doppler cooled on 6S1/2 →6P1/2 transition corresponding to 493 nm. Such single-frequency greenyellow and cyan lasers are based on intracavity frequency doubled vertical-external-cavity surface-emitting laser (VECSEL), serving as an effective replacement of the legacy dye laser, previously used to address these Ba transition. On the other hand, frequency doubled external cavity diode laser (ECDL) is employed to generate 614 nm orange emission needed for 5D5/2→ 6P3/2 transition. The laser system incorporates modular laser engines together with low-noise driving electronics, mechanical and acoustic concealment and provide laser locking interfaces to high-finesse optical cavity or a wavemeter.
High-power, narrow-linewidth light sources in the visible and UV spectra are in growing demand, particularly as quantum information and sensing research proliferates. Vertical external-cavity surface-emitting lasers (VECSELs) with intra-cavity frequency conversion are emerging as an attractive platform to fill these needs. Using such a device, we demonstrate 3.5 MHz full-width half-maximum Rydberg-state spectroscopy via electromagnetically induced transparency (EIT). The laser's 690 mW of output power at a wavelength of 475 nm enables large Rabi frequencies and strong signal-to-noise ratio in shorter measurement times. In addition, we characterize the frequency stability of the VECSEL using the delayed self-heterodyne technique and direct comparison with a commercial external-cavity diode laser (ECDL). We measure the pre-doubled light's Lorentzian linewidth to be 2π × 5.3(2) kHz, and the total linewidth to be 2π × 23(2) kHz. These measurements provide evidence that intra-cavity frequency-doubled VECSELs can perform precision spectroscopy at and below the MHz level, and are a promising tool for contemporary, and future, quantum technologies.
We demonstrate laser cooling of trapped beryllium ions at 313 nm using a frequency-doubled extended cavity diode laser operated at 626 nm, obtained by cooling a ridge waveguide diode laser chip to -31°C. Up to 32 mW of narrowband 626 nm laser radiation is obtained. After passage through an optical isolator and beam shaping optics, 14 mW of 626 nm power remains of which 70% is coupled into an external enhancement cavity containing a nonlinear crystal for second-harmonic generation. We produce up to 35 μW of 313 nm radiation, which is subsequently used to laser cool and detect 6×10(2) beryllium ions, stored in a linear Paul trap, to a temperature of about 10 mK, as evidenced by the formation of Coulomb crystals. Our setup offers a simple and affordable alternative for Doppler cooling, optical pumping, and detection to presently used laser systems.
We report low noise and narrow linewidth performance of an actively stabilized optical parametric oscillator, intracavity-pumped by a visible AlGaInP-based vertical-external-cavity surface-emitting laser (VECSEL). Under dual-locking conditions, where the VECSEL and intracavity resonant idler are stabilized using the Pound–Drever–Hall and side-of-fringe locking techniques, respectively, narrow linewidths of 6.21(1) kHz (VECSEL) and 151(1) Hz (idler) are achieved for integration times as long as 4 s, illustrating the transfer of noise from the VECSEL fundamental to the OPO non-resonant signal. In this regime, the relative intensity noise of all three interacting waves is <−120 dBc/Hz for all frequencies above 1 kHz, indicating that this coherent laser system is well-suited for quantum optics experiments, potentially those involving squeezed light generation.