We use quantum Monte Carlo simulations to study an S = 1/2 spin model with competing multi-spin interactions. We find a quantum phase transition between a columnar valence-bond solid (cVBS) and a Néel antiferromagnet (AFM), as in the scenario of deconfined quantum-critical points, as well as a transition between the AFM and a staggered valence-bond solid (sVBS). By continuously varying a parameter, the sVBS–AFM and AFM–cVBS boundaries merge into a direct sVBS–cVBS transition. Unlike previous models with putative deconfined AFM–cVBS transitions, e.g., the standard J–Q model, in our extended J–Q model with competing cVBS and sVBS inducing terms the transition can be tuned from continuous to first-order. We find the expected emergent U(1) symmetry of the microscopically Z 4 symmetric cVBS order parameter when the transition is continuous. In contrast, when the transition changes to first-order, the clock-like Z 4 fluctuations are absent and there is no emergent higher symmetry. We argue that the confined spinons in the sVBS phase are fracton-like. We also present results for an SU(3) symmetric model with a similar phase diagram. The new family of models can serve as a useful tool for further investigating open questions related to deconfined quantum criticality and its associated emergent symmetries.
We use quantum Monte Carlo simulations to study an S = 1/2 spin model with competing multi-spin interactions. We find a quantum phase transition between a columnar valence-bond solid (cVBS) and a Néel antiferromagnet (AFM), as in the scenario of deconfined quantum-critical points, as well as a transition between the AFM and a staggered valence-bond solid (sVBS). By continuously varying a parameter, the sVBS–AFM and AFM–cVBS boundaries merge into a direct sVBS–cVBS transition. Unlike previous models with putative deconfined AFM–cVBS transitions, e.g., the standard J–Q model, in our extended J–Q model with competing cVBS and sVBS inducing terms the transition can be tuned from continuous to first-order. We find the expected emergent U(1) symmetry of the microscopically Z 4 symmetric cVBS order parameter when the transition is continuous. In contrast, when the transition changes to first-order, the clock-like Z 4 fluctuations are absent and there is no emergent higher symmetry. We argue that the confined spinons in the sVBS phase are fracton-like. We also present results for an SU(3) symmetric model with a similar phase diagram. The new family of models can serve as a useful tool for further investigating open questions related to deconfined quantum criticality and its associated emergent symmetries.
Abstract Berry phase interference arguments that underlie the theory of deconfined quantum criticality (DQC) for S = 1 / 2 antiferromagnets have also been invoked to allow for continuous transitions in S = 1 magnets including a Néel to (columnar) valence bond solid (cVBS) transition. We provide a microscopic model realization of this transition on the square lattice consisting of Heisenberg exchange ( J H ) and biquadratic exchange ( J B ) that favor a Néel phase, and a designed Q -term ( Q B ) interaction which favors a cVBS through large-scale quantum Monte Carlo (QMC) simulations. For J H = 0 , this model is equivalent to the SU(3) JQ model with a Néel-cVBS transition that has been argued to be DQC through QMC. Upon turning on J H which brings down the symmetry to SU(2), we find multiple signatures—a single critical point, high quality collapse of correlation ratios and order parameters, ‘U(1)-symmetric’ cVBS histograms and lack of double-peak in order parameter histograms for largest sizes studied near the critical point—that are highly suggestive of a continuous transition scenario. However, Binder analysis finds negative dips that grow sub-extensively that we interpret as these transitions rather being pseudocritical. This, along with recent results on spin- 1 2 models, suggests that deconfined pseudocriticality is the more generic scenario.
We study the N\'eel to fourfold columnar valence bond solid (cVBS) quantum phase transition in a sign-free S=1 square-lattice model. This is the same kind of transition that for S=1/2 has been argued to realize the prototypical deconfined critical point. Extensive numerical simulations of the square-lattice S=1/2 N\'eel-VBS transition have found consistency with the deconfined critical point scenario with no direct evidence for first-order behavior. In contrast to the S=1/2 case, in our quantum Monte Carlo simulations for the S=1 model, we present unambiguous evidence for a direct conventional first-order quantum phase transition. Classic signs of a first-order transition demonstrating coexistence including double-peaked histograms and switching behavior are observed. The sharp contrast from the S=1/2 case is remarkable; we hypothesize that this is a striking demonstration of the role of the size of the quantum spin in the phase diagram of two-dimensional lattice models.
We introduce a quantum spin-1/2 model with many-body correlated Heisenberg-type interactions on the two-dimensional square lattice, designed so that the system can host a fourfold degenerate plaquette valencebond solid (PVBS) ground state that spontaneously breaks Z 4 symmetry.The system is sign-problem free and amenable to large-scale quantum Monte Carlo simulations, thus allowing us to carry out a detailed study of the quantum phase transition between the standard Néel antiferromagnetic (AFM) and PVBS states.We find a first-order transition, in contrast to previously studied continuous transitions from the AFM phase into a columnar valence-bond solid (CVBS) phase.The theory of deconfined quantum criticality predicts generic continuous AFM-CVBS and AFM-PVBS transitions, and, in one version of the theory, the two critical order parameters transform under SO(5) symmetry.Emergent SO(5) symmetry has indeed been observed in studies of the AFM-CVBS transition, and here we show that the first-order AFM-PVBS transition also exhibits SO(5) symmetry at the transition point.Such unexpected symmetry of the coexistence state, which implies a lack of energy barriers between the coexisting phases, has recently been observed at other first-order transitions, but the case presented here is the first example with SO(5) symmetry.The extended symmetry may indicate that the transition is connected to a deconfined critical point.We also discuss the first-order transition in the context of a recent proposal of spinons with fracton properties in the PVBS state, concluding that the fracton scenario is unlikely.Furthermore, we discover a novel type of eightfold degenerate VBS phase, arising when the PVBS state breaks a remaining Z 2 symmetry.This second phase transition, which is continuous, implies that the PVBS phase can be regarded as an intermediate "vestigial" phase, a concept recently introduced to describe multistage phase transitions involving a continuous symmetry.Here we construct a six-dimensional order parameter and also introduce a general graph-theoretic approach to describe the two-stage discrete symmetry breaking.We discuss different ways of breaking the symmetries in one or two stages at zero and finite temperatures.In the latter case, we observe fluctuation-induced first-order transitions, which are hallmarks of vestigial phase transitions.We also mention possible connections of the AFM-PVBS transition to the SO(5) theory of high-T c superconductivity.
We study the transition between N\'eel and columnar valence-bond solid ordering in two-dimensional S=3/2 square lattice quantum antiferromagnets with SO(3) symmetry. According to the deconfined criticality scenario, this transition can be direct and continuous like the well-studied S=1/2 case. To study the global phase diagram, we work with four multi-spin couplings with full rotational symmetry, that are free of the sign-problem of quantum Monte Carlo. Exploring the phase diagram with quantum Monte Carlo simulations, we find that the phase transition between N\'eel and valence-bond solid is strongly first-order in the parts of the phase diagram that we have accessed.
Open quantum spin systems offer a previously unexplored route to realizing deconfined quantum criticality. We consider a spin-1/2 J-Q3 chain, consisting of an antiferromagnetic (AFM) Heisenberg exchange and a competing multi-spin interaction favoring a valence-bond solid (VBS) state, with each spin component coupled to a bosonic bath. Using non-Abelian bosonization and renormalization-group (RG) analysis, combined with large-scale quantum Monte Carlo (QMC) simulations, we determine the phase diagram and the associated phase transitions of the model. We show that strong dissipation stabilizes an AFM phase for sub-Ohmic, Ohmic, and super-Ohmic baths. Continuous AFM-VBS transitions at finite dissipation are found upon increasing the multi-spin interaction in both the sub-Ohmic and Ohmic regimes. Critical properties are obtained through perturbative RG analysis and QMC simulations. In the Ohmic case, the critical point features spinon deconfinement and emergent O(4) symmetry. In the sub-Ohmic regime, the transition may also involve spinon deconfinement, provided that spinons remain deconfined in the dissipative VBS phase. In addition, in the super-Ohmic regime, we propose a transition from AFM phase to a quasi-long-range ordered phase.
We study spin-1/2 chains with long-range power-law decaying unfrustrated (bipartite) Heisenberg exchange Jr∝r−α and multi-spin interactions Q favoring a valence-bond solid (VBS) ground state. Employing quantum Monte Carlo techniques and Lanczos diagonalization, we analyze order parameters and excited-state level crossings to characterize quantum states and phase transitions in the (α,Q) plane. For weak Q and sufficiently slowly decaying Heisenberg interactions (small α), the system has a long-range-ordered antiferromagnetic (AFM) ground state, and upon increasing α there is a continuous transition into a quasi long-range ordered (QLRO) critical state of the type in the standard Heisenberg chain. For rapidly decaying long-range interactions, there is transition between QLRO and VBS ground states of the same kind as in the frustrated J1-J2 Heisenberg chain. Our most important finding is a direct continuous quantum phase transition between the AFM and VBS states - a close analogy to the 2D deconfined quantum-critical point. In previous 1D analogies the ordered phases both have gapped fractional excitations, and the critical point is a conventional Luttinger Liquid. In our model the excitations fractionalize upon transitioning from the AFM state, changing from spin waves to deconfined spinons. We extract critical exponents at the AFM-VBS transition and use order-parameter distributions to study emergent symmetries. We find emergent O(4) symmetry of the O(3) AFM and scalar VBS order parameters. Thus, the order parameter fluctuations exhibit the covariance of a uniaxially deformed O(4) sphere (an "elliptical" symmetry). This unusual quantum phase transition does not yet have any known field theory description, and our detailed results can serve to guide its construction. We discuss possible experimental realizations.