Estimating the quality of a single-photon source is crucial for its use in quantum technologies. The standard test for semiconductor sources is a value of the second-order correlation function of the emitted field below $1/2$ at zero time delay. This criterion alone provides no information regarding the amplitude of the single-photon contribution for general quantum states. Addressing this question requires the knowledge of additional observables. We derive an effective second-order correlation function, strongly connected to the Mandel-$Q$ parameter and given in terms of both the second-order correlation and the average photon number, that provides a lower bound on the single-to-multiphoton projection ratio. Using both observables individually allows for lower and upper bounds for the single-photon projection. Comparing the tightness of our bounds with those in the literature, we find that relative bounds may be better described using the average photon number, while absolute bounds for low excitation states are tighter using the vacuum projection. Our results show that estimating the quality of a single-photon source based on additional information is very much dependent on what aspect of the quantum state of light one is interested in.
Estimating the quality of a single-photon source is crucial for its use in quantum technologies. The standard test for semiconductor sources is a value of the second-order correlation function of the emitted field below 1/2 at zero time delay. This criterion alone provides no information regarding the amplitude of the single-photon contribution for general quantum states. Addressing this question requires the knowledge of additional observables. We derive an effective second-order correlation function, strongly connected to the Mandel-Q parameter and given in terms of both the second-order correlation and the average photon number, that provides a lower bound on the single-to-multiphoton projection ratio. Using both observables individually allows for lower and upper bounds for the single-photon projection. Comparing the tightness of our bounds with those in the literature, we find that relative bounds may be better described using the average photon number, while absolute bounds for low excitation states are tighter using the vacuum projection. Our results show that estimating the quality of a single-photon source based on additional information is very much dependent on what aspect of the quantum state of light one is interested in.
Abstract Quantum-optical research on semiconductor single-photon sources puts special emphasis on the measurement of the second-order correlation function g (2) ( τ ), arguing that g (2) (0) < 1/2 implies the source field represents a good single-photon light source. We analyze the gain of information from g (2) (0) with respect to single photons. Any quantum state, for which the second-order correlation function falls below 1/2, has a nonzero projection on the single-photon Fock state. The amplitude p of this projection is arbitrary, independent of g (2) (0). However, one can extract a lower bound on the single-to-multi-photon-projection ratio. A vacuum contribution in the quantum state of light artificially increases the value of g (2) (0), cloaking actual single-photon projection. Thus, we propose an effective second-order correlation function g ˜ ( 2 ) ( 0 ) , which takes the influence of vacuum into account and also yields lower and upper bounds on p . We consider the single-photon purity as a standard figure of merit in experiments, reinterpret it within our results and provide an effective version of that physical quantity. Besides comparing different experimental and theoretical results, we also provide a possible measurement scheme for determining g ˜ ( 2 ) ( 0 ) .
What g(2)(0)<1/2 tells you - and what it does not
Quantum-optical research on semiconductor quantum dots puts special emphasis on the measurement of the second-order correlation function g(2)(τ), arguing that g(2)(0)<1/2 implies the source field represents a good single-photon light source. We analyze this claim theoretically. A quantum state of light having no projection on the single-photon Fock state can not give a value of g(2)(0)<1/2. However, with solely the value of g(2)(0), the amplitude of this single-photon projection can be arbitrarily small, owing to vacuum contributions. Yet, one can determine a lower bound on the ratio of single-to-multi-photon emission from g(2)(0). For a fixed ratio of single-to-multi-photon emission, g(2)(0) is artificially enhanced by the vacuum contributions. We derive an effective second-order correlation function, which corrects this enhancement, substantially improving the lower bound. The results are applied to theoretical and realized experimental setups and indicate that the quality of solid-state single-photon sources, at least with respect to this criterion, is often underestimated.
This thesis intends to familiarize the reader with the concepts of photon statistics and correlations in quantum optics. Developing light sources that emit quantum states is central for the realization of quantum technologies. One important step in characterizing these sources is the measurement of field fluctuations and correlations, by coincidence measurements. The expectation value of a coincidence measurement, a simultaneous measurement of two intensities (or, more general, four fields), is represented by the fourth-order correlation function. The value of the correlation function, at zero delay between the detection of two photons, reveals important properties of the state to which they belonged, for example the fluctuations of the photon number. Since predictability is important for many applications, light sources emitting single photons are also characterized by the indistinguishability of consecutively emitted photons, or of two photons from separate emitters. In paper I we investigate blinking behaviour in quantum emitters, and its effect on the interference pattern and photon statistics with photons from two separate emitters. Blinking refers to an emitters transition into a non-emitting state, and subsequent transition back to an emitting state. We show that blinking can not be treated as linear loss, when measuring the fourth-order correlation function for two emitters in a Hong-Ou-Mandel setup. In general, a measurement of the fourth-order correlation function is robust to loss, which makes it a very practical tool. However, the relation between recorded coincidence counts and the correlation function is only direct in the limit of zero detection efficiency, and depends on the detection system. In paper II, we show that by adding a variable attenuation in the beam path, we can trace back to the ''true'' value of the correlation function at zero quantum efficiency. This method improves accuracy in correlation measurements by decreasing a systematic error at the expense of an increased statistical error, which is easier to handle, extending the use of coincidence methods to classical and non-classical multi-photon states.
Low-photon-number sources can exhibit non-classical, counterintuitive behavior that can be exploited in the developing field of quantum technology. Single photons play a special role in this arena since they represent the ultimate lowphoton- number source. They are considered an important element in various applications such as quantum key distribution, optical quantum information processing, quantum computing, intensity measurement standards, and others yet to be discovered in this developing field. True deterministic sources of single photons on demand are currently an area of intensive research, but have not been demonstrated in a practical setting. As a result, researchers commonly default to the well-established workhorse: spontaneous parametric down-conversion generating entangled signal-idler pairs. Since this source is thermal-statistical in nature, it is common to use a detected idler photon to herald the production of a signal photon. The need exists to determine the quality of the single photons generated in the heralded signal beam. Quite often, the literature reports a "heralded second-order coherence function" of the signal photons conditioned on the idler photons using readily available single-photon detectors. In this work, we examine the applicability of this technique to single-photon characterization and the consequences of the fact that the most commonly used single-photon detectors are not photon-number resolving. Our results show that this method using non-photonresolving detectors can only be used to characterize the signal-idler correlations rather than the nature of the signalphoton state alone.
The development of linear quantum computing within integrated circuits demands high quality semiconductor single photon sources. In particular, for a reliable single photon source it is not sufficient to have a low multi-photon component, but also to possess high efficiency. We investigate the photon statistics of the emission from a single quantum dot with a method that is able to sensitively detect the trade-off between the efficiency and the multi-photon contribution. Our measurements show, that the light emitted from the quantum dot when it is resonantly excited possess a very low multi-photon content. Additionally, we demonstrated, for the first time, the non-Gaussian nature of the quantum state emitted from a single quantum dot.
A variety of quantum emitters compete in the quest for the best single-photon source for photonic quantum technologies. Consequently, only a consistent approach to analyze the second-order auto correlation function allows comparison of the multi-photon contribution (g(2)(0)) of different sources. However, the community employs different and inconsistent methods for blinking sources, leading to incomparable benchmarks of source quality. Here, we use the emission of an inherently non-blinking quantum dot (QD) and apply artificial blinking through two different mechanisms: masking the recorded raw data in post-processing and emulation of a blinking system by gating the laser excitation pulses. We then compare the g(2)(0) values with the non-blinking result. For the analysis, we investigate five estimators of g(2)(0) actively used in the literature. While fitting the envelope of the correlations on long-time scales with the correct blinking model is the best choice, normalizing to the Poisson level gives by far the worst proximity. Furthermore, we test our predictive model to identify the underlying blinking mechanism of a QD in a circular Bragg grating cavity.