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arXiv:2002.01224 · Physical Review Letters

Radio-Frequency Response and Contact of Impurities in a Quantum Gas

Weizhe Edward Liu, Zhe-Yu Shi, Jesper Levinsen, Meera M. Parish

Published Aug 5, 2020• 20 citations
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Abstract

We investigate the radio-frequency spectroscopy of impurities interacting with a quantum gas at finite temperature. In the limit of a single impurity, we show using Fermi's golden rule that introducing (or injecting) an impurity into the medium is equivalent to ejecting an impurity that is initially interacting with the medium, since the "injection" and "ejection" spectral responses are simply related to each other by an exponential function of frequency. Thus, the full spectral information for the quantum impurity is contained in the injection spectral response, which can be determined using a range of theoretical methods, including variational approaches. We use this property to compute the finite-temperature equation of state and Tan contact of the Fermi polaron. Our results for the contact of a mobile impurity are in excellent agreement with recent experiments and we find that the finite-temperature behavior is qualitatively different compared to the case of infinite impurity mass.

DOI
10.1103/physrevlett.125.065301

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We investigate the radio-frequency spectroscopy of impurities interacting with a quantum gas at finite temperature. In the limit of a single impurity, we show using Fermi's golden rule that introducing (or injecting) an impurity into the medium is equivalent to ejecting an impurity that is initially interacting with the medium, since the "injection" and "ejection" spectral responses are simply related to each other by an exponential function of frequency. Thus, the full spectral information for the quantum impurity is contained in the injection spectral response, which can be determined using a range of theoretical methods, including variational approaches. We use this property to compute the finite-temperature equation of state and Tan contact of the Fermi polaron. Our results for the contact of a mobile impurity are in excellent agreement with recent experiments and we find that the finite-temperature behavior is qualitatively different compared to the case of infinite impurity mass.
We present a theory of radio-frequency spectroscopy of impurities interacting with a quantum gas at finite temperature. By working in the canonical ensemble of a single impurity, we show that the impurity spectral response is directly connected to the finite-temperature equation of state (free energy) of the impurity. We consider two different response protocols: injection, where the impurity is introduced into the medium from an initially noninteracting state, and ejection, where the impurity is ejected from an initially interacting state with the medium. We show that there is a simple mapping between injection and ejection spectra, which is connected to the detailed balance condition in thermal equilibrium. To illustrate the power of our approach, we specialize to the case of the Fermi polaron, corresponding to an impurity atom that is immersed in a noninteracting Fermi gas. For a mobile impurity with a mass equal to the fermion mass, we employ a finite-temperature variational approach to obtain the impurity spectral response. We find a striking nonmonotonic dependence on temperature in the impurity free energy, the contact, and the radio-frequency spectra. For the case of an infinitely heavy Fermi polaron, we derive exact results for the finite-temperature free energy, thus generalizing Fumi's theorem to arbitrary temperature. We also determine the exact dynamics of the contact after a quench of the impurity-fermion interactions. Finally, we show that the injection and ejection spectra obtained from the variational approach compare well with the exact spectra, thus demonstrating the accuracy of our approximation method.
We present a systematic study of a mobile impurity immersed in a three-dimensional Fermi sea of fermions at finite temperature, by using the standard non-self-consistent many-body TTT-matrix theory that is equivalent to a finite-temperature variational approach with the inclusion of one-particle-hole excitation. The impurity spectral function is determined in the real-frequency domain, avoiding any potential errors due to the numerical analytic continuation in previous TTT-matrix calculations and the small spectral broadening parameter used in variational calculations. In the weak-coupling limit, we find that the quasiparticle decay rate of both attractive and repulsive polarons does not increase significantly with increasing temperature, and therefore Fermi polarons may remain well defined far above Fermi degeneracy. In contrast, near the unitary limit with strong coupling, the decay rate of Fermi polarons rapidly increases and the quasiparticle picture breaks down close to the Fermi temperature. We analyze in detail the recent ejection and injection radio-frequency (rf) spectroscopy measurements, performed at Massachusetts Institute of Technology (MIT) and at the European Laboratory for Non-Linear Spectroscopy (LENS), respectively. We show that the momentum average of the spectral function, which is necessary to account for the observed rf spectroscopy, has a sizable contribution to the width of the quasiparticle peak in spectroscopy. As a result, the measured decay rate of Fermi polarons could be significantly larger than the calculated quasiparticle decay rate at zero momentum. By taking this crucial contribution into account, we find that there is a reasonable agreement between theory and experiment for the lifetime of Fermi polarons in the strong-coupling regime, as long as they remain well defined.
In this report we discuss the dynamical response of heavy quantum impurities immersed in a Fermi gas at zero and at finite temperature. Studying both the frequency and the time domain allows one to identify interaction regimes that are characterized by distinct many-body dynamics. From this theoretical study a picture emerges in which impurity dynamics is universal on essentially all time scales, and where the high-frequency few-body response is related to the long-time dynamics of the Anderson orthogonality catastrophe by Tan relations. Our theoretical description relies on different and complementary approaches: functional determinants give an exact numerical solution for time- and frequency-resolved responses, bosonization provides accurate analytical expressions at low temperatures, and the theory of Toeplitz determinants allows one to analytically predict response up to high temperatures. Using these approaches we predict the thermal decoherence rate of the fermionic system and prove that within the considered model the fastest rate of long-time decoherence is given by [Formula: see text]. We show that Feshbach resonances in cold atomic systems give access to new interaction regimes where quantum effects can prevail even in the thermal regime of many-body dynamics. The key signature of this phenomenon is a crossover between different exponential decay rates of the real-time Ramsey signal. It is shown that the physics of the orthogonality catastrophe is experimentally observable up to temperatures [Formula: see text] where it leaves its fingerprint in a power-law temperature dependence of thermal spectral weight and we review how this phenomenon is related to the physics of heavy ions in liquid [Formula: see text]He and the formation of Fermi polarons. The presented results are in excellent agreement with recent experiments on LiK mixtures, and we predict several new phenomena that can be tested using currently available experimental technology.
Recent experimental advances enabled the realization of mobile impurities immersed in a Bose-Einstein condensate (BEC) of ultracold atoms. Here, we consider impurities with two or more internal hyperfine states, and study their radio-frequency (rf) absorption spectra, which correspond to transitions between two different hyperfine states. We calculate rf spectra for the case when one of the hyperfine states involved interacts with the BEC, while the other state is noninteracting, by performing a nonperturbative resummation of the probabilities of exciting different numbers of phonon modes. In the presence of interactions, the impurity gets dressed by Bogoliubov excitations of the BEC, and forms a polaron. The rf signal contains a $\ensuremath{\delta}$-function peak centered at the energy of the polaron measured relative to the bare impurity transition frequency with a weight equal to the amount of bare impurity character in the polaron state. The rf spectrum also has a broad incoherent part arising from the background excitations of the BEC, with a characteristic power-law tail that appears as a consequence of the universal physics of contact interactions. We discuss both the direct rf measurement, in which the impurity is initially in an interacting state, and the inverse rf measurement, in which the impurity is initially in a noninteracting state. In the latter case, in order to calculate the rf spectrum, we solve the problem of polaron formation: a mobile impurity is suddenly introduced in a BEC, and dynamically gets dressed by Bogoliubov phonons. Our solution is based on a time-dependent variational ansatz of coherent states of Bogoliubov phonons, which becomes exact when the impurity is localized. Moreover, we show that such an ansatz compares well with a semiclassical estimate of the propagation amplitude of a mobile impurity in the BEC. Our technique can be extended to cases when both initial and final impurity states are interacting with the BEC.
The radio-frequency spectrum of the fermions in the unitary limit at finite temperatures is characterized by the sum-rule relations. We consider a simple picture where the atoms are removed by radio-frequency excitations from the strongly interacting states into a state of negligible interaction. We calculate the moments of the response function in the range of temperature 0.08ϵF<T<0.8ϵF0.08{ϵ}_{F}<T<0.8{ϵ}_{F}0.08ϵF​<T<0.8ϵF​ using auxiliary field Monte Carlo technique in which continuum auxiliary fields with a density-dependent shift are used. We estimate the effects of superfluid pairing from the clock shift. We find a qualitative agreement with the pairing gap--pseudogap transition behavior. We also find within the quasiparticle picture that in order for the gap to come into quantitative agreement with the previously known value at T=0T=0T=0, the effective mass has to be ${m}^{\ensuremath{\ast}}\ensuremath{\sim}1.43m$. Finally, we discuss implications for the adiabatic sweep of the resonant magnetic field.
We consider the McGuire model of a one-dimensional gas of free fermions interacting with a single impurity. We compute the static one-body function and momentum distribution of the impurity at finite temperatures. The results involve averages over Fredholm determinants that we further analyze using the effective form factors approach. With this approach, we derive the large-distance behavior of the one-body function, which takes the form of an averaged exponential decay. This method allows us to study an experimentally important regime of small momenta of the impurity's momentum distribution. We also consider the one-body function at short distances and compute finite-temperature Tan's contact.